Publication Information

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108, 121, 140, 153, 164, 166, 180, 191, 193, 207, 226, 239, 247, 272, 285, 293], '100190': [50, 63, 82, 109, 122, 141, 154, 181, 208, 227, 240, 273, 286], 'Biopharmaceutical': [54, 113, 145, 231, 277], 'Preparation': [55, 114, 146, 232, 278], 'Delivery,': [57, 116, 148, 234, 280], ',': [64, 91, 123, 155, 182, 209], 'Li': [66], 'University': [83, 158, 185, 241, 287], '100049': [90, 165, 192, 248, 294], 'Zhao': [93, 125], 'Zhang': [157], 'National': [167, 194], 'Condensed': [170, 197], 'Matter': [171, 198], 'Physics,': [172, 175, 199, 202], 'Gu': [184], '*Corresponding': [252], 'author:': [253], 'E-mail': [254], 'Address:': [255], '[email': [256], 'protected]': [257], 'https://doi.org/10.31635/ccschem.024.202303604': [295], 'SectionsSupplemental': [296], 'MaterialAboutAbstractPDF': [297], 'ToolsAdd': [298], 'to': [299, 313, 363, 401, 421, 462, 520, 628, 652, 791, 816, 848, 961, 1003, 1345, 1404, 1605, 1779, 1783, 1862, 2059, 2078, 2093, 2117, 2161, 2176, 2180, 2190, 2197, 2220, 2246, 2257, 2341, 2460, 2472, 2523, 2559, 2578, 2765, 2972, 3027, 3034, 3175, 3196, 3202, 3272, 3347, 3352, 3487, 3617, 3648, 3689, 3693, 3724, 3800, 3819, 3831, 3912, 4002], 'favoritesDownload': [300], 'CitationsTrack': [301], 'Citations': [302], 'ShareFacebookTwitterLinked': [303], 'InEmail': [304], 'The': [305, 414, 502, 897, 917, 946, 1138, 1261, 1297, 1596, 1640, 1711, 1804, 1853, 1874, 1897, 2037, 2104, 2288, 2492, 2514, 2799, 2829, 2853, 2875, 2909, 2929, 3002, 3047, 3186, 3374, 3438, 3450, 3478, 3510, 3667, 3735, 3771, 3867, 3935, 3965, 3995], 'ultimate': [306], 'goal': [307], 'photocatalytic': [309, 514, 583, 672, 716, 861, 1086, 3343, 3355, 3520, 3535, 3588], 'reduction': [311, 344, 674, 718, 749, 863, 2479, 3022, 3344, 3357, 3491, 3746, 3780, 3804], 'is': [312, 789, 1266, 1343, 1402, 1458, 1493, 1543, 1552, 1788, 1843, 1860, 2076, 2138, 2264, 2293, 2302, 2330, 2533, 2623, 2631, 2639, 2653, 2660, 2763, 2882, 2896, 2934, 2970, 3224, 3266, 3417, 3447, 3455, 3525, 3566, 3816, 3937, 4029, 4036, 4042, 4047, 4052, 4057], 'efficiently': [314], 'convert': [315], 'atmospheric': [316, 380, 472, 729, 743, 1117, 1185, 3744, 3802, 3904], 'into': [318, 509], 'value-added': [319, 510], 'products': [320, 2430, 3695, 3726], 'by': [321, 345, 536, 679, 775, 985, 1056, 1623, 1720, 1820, 2141, 2295, 2304, 2332, 2502, 2536, 2566, 2776, 2839, 2885, 2936, 3302, 3419, 3496, 3528, 3750, 3939], 'designing': [322], 'hierarchical': [323, 570, 915, 1399, 2250], 'photocatalysts': [324, 573, 3620], 'that': [325, 390, 614, 1228, 1350, 1664, 1692, 1786, 2266, 2761, 2768, 3073, 3226, 3774, 3793, 3917], 'combine': [326], 'effective': [327, 373, 734], 'harvesting': [328, 855, 1390, 3828, 4007], 'accelerate': [330], 'activation': [331, 3334], 'capabilities': [332], 'molecules.': [335, 436], 'In': [336, 2312, 3130, 3585, 3683], 'this': [337, 1310], 'work,': [338], 'we': [339, 969, 2383, 2444, 2753, 3350], 'demonstrated': [340], 'direct': [341, 505, 1444], 'air-level': [342, 506], 'hollow': [346, 588, 1569], 'multishell': [347], 'structure': [348, 1032, 1825, 1890, 1979, 2386, 2451, 2868, 2906, 3288, 3298, 3643], '(HoMS)': [349, 591], 'nanoreactors': [350, 482, 592, 1328, 3661], 'with': [351, 384, 446, 474, 543, 574, 593, 750, 781, 1033, 1048, 1105, 1107, 1130, 1179, 1375, 1398, 1431, 1540, 1557, 1762, 1764, 1998, 2324, 2433, 2707, 2869, 2878, 3111, 3219, 3387, 3434, 3551, 3609, 3706, 3730, 3846, 3889, 3927, 3962, 3977, 3989], 'zeolitic': [352, 973], 'imidazolate': [353, 974], 'framework-8': [354, 975], '(ZIF-8)-modified': [355], 'ZnO': [356, 1008, 1025, 1046, 1090, 1125, 1176, 1242, 1264, 1288, 1326, 1442, 1463, 1497, 1505, 1514, 1555, 1568, 1576, 1581, 1657, 1669, 1705, 1731, 1815, 1840, 1850, 1913, 1937, 1941, 1968, 1972, 2177, 2183, 2208, 2236, 2299, 2354, 2389, 2398, 2404, 2466, 2484, 2495, 2511, 2521, 2526, 2895, 2900, 2921, 2946, 2956, 2995, 3114, 3128, 3133, 3153, 3200, 3248, 3308, 3361, 3422, 3445, 3523, 3596, 3676, 3759, 3814, 3844, 3856, 3921, 3967, 3981, 3987], 'heteroshells,': [357], 'which': [358, 455, 549, 989, 1157, 1250, 1275, 1499, 1726, 1842, 1868, 2044, 2096, 2137, 2194, 2329, 2532, 2582, 2659, 2784, 3038, 3192, 3463, 3575, 3924], 'offers': [359, 516, 1417], 'a': [360, 484, 517, 726, 767, 776, 793, 924, 971, 1029, 1049, 1149, 1153, 1270, 1376, 1614, 1654, 1831, 1905, 1958, 2060, 2381, 2395, 2434, 2477, 2612, 2646, 2666, 2667, 2870, 2925, 3012, 3016, 3021, 3031, 3035, 3054, 3091, 3267, 3548, 3564, 3569, 3586, 3603, 3707, 3717, 3970, 3990], 'promising': [361, 518, 925], 'solution': [362, 519, 1492, 2314], 'optimize': [364], 'the': [365, 379, 396, 408, 419, 427, 438, 443, 458, 480, 489, 522, 538, 551, 578, 609, 616, 626, 629, 637, 688, 709, 715, 733, 764, 819, 834, 840, 872, 882, 903, 910, 931, 937, 940, 954, 962, 986, 1005, 1021, 1060, 1064, 1072, 1080, 1085, 1092, 1112, 1122, 1136, 1160, 1174, 1239, 1245, 1258, 1276, 1282, 1293, 1302, 1316, 1331, 1334, 1352, 1357, 1362, 1388, 1406, 1436, 1440, 1450, 1461, 1501, 1511, 1518, 1533, 1537, 1566, 1584, 1587, 1599, 1619, 1624, 1628, 1661, 1667, 1676, 1693, 1696, 1704, 1715, 1751, 1756, 1768, 1789, 1793, 1835, 1846, 1863, 1870, 1877, 1885, 1916, 1924, 1986, 1999, 2002, 2011, 2024, 2068, 2071, 2079, 2088, 2101, 2129, 2135, 2157, 2168, 2172, 2185, 2188, 2198, 2211, 2221, 2226, 2232, 2267, 2278, 2283, 2296, 2305, 2309, 2313, 2316, 2319, 2325, 2333, 2342, 2346, 2350, 2353, 2357, 2364, 2372, 2377, 2385, 2402, 2410, 2417, 2428, 2437, 2440, 2446, 2461, 2468, 2473, 2483, 2503, 2529, 2537, 2551, 2560, 2567, 2594, 2597, 2600, 2624, 2627, 2632, 2640, 2656, 2676, 2688, 2711, 2742, 2769, 2777, 2791, 2797, 2805, 2824, 2844, 2851, 2857, 2865, 2899, 2916, 2920, 2932, 2937, 2943, 2950, 2953, 2960, 2974, 2985, 2994, 3028, 3065, 3078, 3088, 3100, 3121, 3132, 3140, 3150, 3169, 3197, 3204, 3209, 3220, 3228, 3237, 3241, 3245, 3255, 3258, 3273, 3281, 3286, 3291, 3300, 3304, 3320, 3327, 3333, 3354, 3360, 3365, 3369, 3377, 3382, 3388, 3394, 3413, 3420, 3435, 3467, 3481, 3490, 3497, 3519, 3530, 3534, 3544, 3552, 3557, 3577, 3590, 3613, 3632, 3635, 3638, 3657, 3670, 3674, 3685, 3743, 3752, 3775, 3789, 3794, 3801, 3807, 3820, 3825, 3832, 3900, 3907, 3914, 3920, 3945, 3980, 4005, 4030, 4037, 4043, 4048, 4053, 4058], 'mass': [366, 620, 643, 711, 955, 1076, 1181, 2260, 2273, 2779, 3515], 'transfer': [367, 409, 451, 621, 646, 712, 803, 858, 956, 1077, 1083, 1146, 1182, 2261, 2274, 2780, 3125, 3516], 'process': [368, 515, 796, 3747], 'via': [369, 513, 1292], 'selective': [370, 1389, 4006], 'sieving': [371, 1385, 1424, 3916], 'enrichment': [374, 1074, 1140, 2792, 3795], 'molecules': [377, 425, 762, 3338], 'from': [378, 625, 763, 1439, 1666, 1681, 1777, 2087, 2517, 2702, 2734, 2741, 2756, 2790, 2814, 2856, 2898, 3030, 3053, 3160, 3489, 3727], 'environments.': [381, 3682], 'Specifically,': [382, 3254], 'heteroshells': [383, 1757, 1796, 3645], 'ZIF-8': [385, 1014, 1285, 1374, 1397, 1447, 1509, 1522, 1538, 1601, 1673, 1697, 1734, 1787, 2072, 2175, 2291, 2320, 2365, 2474, 2497, 2508, 3000, 3312, 3740, 3833, 3928], 'matrix': [386], 'act': [387], 'as': [388, 399, 979, 982, 1211, 1257, 2218, 2406, 2655, 3393, 3398, 3466, 3494, 3501, 3766], 'pumps': [389], 'effectively': [391, 422], 'capture': [392, 933], 'molecules,': [394, 404, 1341, 1373, 1427], 'while': [395], 'cavities': [397, 943, 1068], 'serve': [398], 'tanks': [400], 'hold': [402], 'these': [403, 707, 810, 2572, 3660], 'thus': [405, 430, 1516, 3715], 'significantly': [406, 635, 777, 880, 959, 3289, 3380, 3985], 'enhancing': [407, 3332], 'kinetics': [410, 713, 1183, 3517], 'photoreduction.': [413], 'periodic': [415, 887], 'shell-cavity': [416], 'configuration': [417], 'allows': [418, 1500], 'nanoreactor': [420, 1178], 'gather': [423], 'near': [426, 1510, 1823], 'catalytic': [428, 723, 995, 1155, 3324], 'sites,': [429], 'increasing': [431, 665, 703, 3529], 'conversion': [432, 508, 556, 666, 735, 795, 3592, 3686], 'opportunities': [433, 667], 'activated': [435], 'Simultaneously,': [437], 'surface': [439, 779, 806, 883, 1006, 1037, 1066, 1336, 1359, 1512, 1794, 2222, 2681, 2712, 2731, 2821, 2879, 2918, 2951, 2961, 3058, 3151], 'atomic': [440, 1038, 1769, 2682, 2725, 2732, 2848, 2880, 2910, 2939, 3085, 3177], 'steps': [441, 1039, 2733, 2849, 2881, 2911, 3086, 3167], 'on': [442, 560, 838, 1019, 1287, 1449, 1700, 1792, 2134, 2272, 2308, 2427, 2436, 2593, 2796, 2850, 2915, 2949, 2959, 2979, 3518], 'ZnO/ZIF-8': [444, 1034, 1041, 1633, 1925, 1946, 1961, 2254, 2378, 2580, 2689, 2699, 2770, 2802, 2825, 2927, 2997, 3141, 3170, 3276, 3284, 3378, 3931], 'heterointerfaces': [445, 837, 1042, 1630, 2281, 2803, 2826, 2978, 3932], 'staggered': [447, 3048, 3180], 'geometry': [448, 2877, 2930, 3049], 'expedite': [449], 'charge': [450, 658, 700, 802, 1082, 3075, 3124], 'adsorption': [453, 696, 1847, 2004, 3869, 3877], 'efficiency,': [454], 'synergistically': [456, 846], 'boosts': [457], 'CO2-CO': [459], 'yield': [460, 1095, 3416, 3441, 3546, 3811], 'up': [461], '3.7': [463, 1097, 3600], 'μmol/h': [464, 470, 1098, 1104, 3601, 3608], 'under': [465, 471, 725, 738, 1099, 1116, 1163, 2409, 3428, 3457, 3621, 3761, 3861], 'flow': [467], '0.7': [469, 1103, 2065], 'conditions': [473, 827, 3138, 3623], 'almost': [475, 1108], 'complete': [476, 1298], 'CO': [477, 1094, 1114, 1150, 3348, 3385, 3410, 3415, 3483, 3545, 3591, 3690, 3753, 3810, 3839, 3851], 'selectivity.': [478], 'Hopefully,': [479], 'HoMS': [481, 641, 685, 771, 843, 870, 885, 901, 1031, 1070, 1243, 1338, 1556, 1625, 1969, 2243, 2271, 2390, 2441, 3287, 3636, 3738, 3760, 3777, 3815, 3988], 'offer': [483, 923], 'potential': [485, 503, 1123, 3671, 4000], 'strategy': [486], 'solving': [488], '"last': [490], 'mile"': [491], 'challenge': [492], 'in': [493, 568, 605, 648, 693, 714, 852, 860, 909, 1028, 1040, 1045, 1127, 1135, 1224, 1234, 1249, 1269, 1274, 1309, 1315, 1410, 1420, 1563, 1631, 1650, 1688, 1708, 1746, 1814, 1834, 1876, 1884, 1892, 1908, 1911, 2100, 2107, 2152, 2167, 2187, 2207, 2231, 2480, 2482, 2540, 2553, 2574, 2745, 2786, 2804, 2808, 2832, 2924, 3008, 3023, 3117, 3145, 3168, 3217, 3269, 3318, 3372, 3400, 3533, 3539, 3581, 3602, 3678, 3742, 3768, 3788, 3809, 3960], 'practical': [494, 745, 1128], 'valorization.': [496], 'Download': [497, 499, 1188, 1190, 2006, 2008, 2748, 2750, 3894, 3896], 'figure': [498, 1189, 2007, 2749, 3895], 'PowerPoint': [500, 1191, 2009, 2751, 3897], 'Introduction': [501], 'solar': [511], 'fuels': [512], 'combat': [521], 'greenhouse': [523], 'effect': [524, 2269, 3796], 'achieve': [526, 1435], 'carbon': [527, 2124], 'neutrality.1–4': [528], 'Natural': [529], 'photosynthesis': [530, 562], 'systems': [531, 563], 'give': [532, 2020], 'an': [533, 1235, 2248, 3069, 3502, 3703], 'excellent': [534], 'example': [535], 'realizing': [537], 'delicate': [539], 'assembly': [540], 'organelles': [542], 'varying': [544, 1558], 'nano-/microstructures': [545], 'chemical': [547, 993, 1753, 2027, 2418, 2447, 2554, 3293, 3999], 'composition,': [548, 2419, 3639], 'enables': [550], 'efficient': [552, 582, 829, 895, 932, 1139, 2249], 'capturing': [553, 760], 'continuous': [555, 2992], 'CO2.5–8': [558], 'Research': [559], 'mimicking': [561], 'has': [564, 813, 3484], 'sparked': [565, 602], 'significant': [566, 1418, 2105, 2478, 2515, 3262], 'interest': [567], 'developing': [569], 'mesostructured': [571], 'complex': [572], 'diverse': [575], 'compositions': [576, 600, 1754, 2555], 'purpose': [579], 'highly': [581], 'reduction.9–13': [585], 'Among': [586], 'them,': [587], 'multishelled': [589], 'structures': [590, 1457, 1713, 1806, 3182], 'adjustable': [594], 'shell': [595, 599, 1065, 1456, 1559, 1978, 2569, 3395], 'architecture': [596], 'adaptable': [598], 'have': [601, 676, 792, 2057, 2244, 3090], 'pioneering': [603], 'explorations': [604], 'valorization.14–16': [607], 'Notably,': [608], 'distinctive': [610, 2469], 'temporal-spatial': [611], 'ordering': [612], 'characteristic': [613, 1416, 2122, 2158], 'ensures': [615], 'proper': [617], 'sequence': [618], 'through': [622, 800, 833, 886, 2391, 2456, 3339, 3699], 'shells,': [623, 1026, 1706], 'either': [624], 'interior': [627], 'exterior': [630], 'or': [631, 741, 1205, 1226], 'opposite': [632], 'direction': [633], 'would': [634], 'leverage': [636], 'multiscale': [638], 'benefits': [639], 'energy': [645, 1682, 2063, 2590, 2966, 3018], 'processes': [647, 859], 'reduction,': [650], 'leading': [651], 'enhanced': [653, 998, 1180, 1411], 'incident': [654, 3470], 'light': [655, 3461, 3471], 'absorption,': [656], 'accelerated': [657, 801, 1081, 1144], 'transfer,': [659, 701], 'improved': [661, 782, 3123, 3514], 'reactant': [662], 'enrichment,': [663], 'thereby': [664, 958, 3331], 'molecules.17': [670], 'Boosted': [671], 'activities': [675, 724], 'been': [677, 1230, 3485], 'achieved': [678, 799, 3418, 3456, 3698], 'Co3O4,18': [680], 'SnO2/SnS2,19': [681], 'ZnS/CdS,20': [682], 'TiO2/CeO2': [684], 'photocatalysts,21': [686], 'demonstrating': [687], 'effectiveness': [689, 964], 'structural': [691, 898, 2975], 'regulation': [692], 'promoting': [694], 'ability,': [697], 'improving': [698], 'interfacial': [699, 2586, 3305], 'active': [704, 892, 1358], 'sites.22': [705], 'Despite': [706, 2010], 'advancements,': [708], 'sluggish': [710], 'reaction': [719, 1531], 'still': [720], 'hinders': [721], 'their': [722, 2258], 'lowly': [727], 'concentrated': [728], 'environment.': [730, 1118, 1137], 'To': [731, 808, 1329, 1434, 3898], 'realize': [732], 'low': [739, 1131, 1164, 1432, 3679, 3732], 'concentrations': [740, 1132], 'even': [742], 'CO2,': [744, 773, 798, 3493], 'scenarios': [746], 'more': [751, 1050, 2098, 3274, 3391, 3817], 'stringent': [752], 'requirements': [753], 'are': [754, 1016, 1043, 1290, 1718, 1817, 1882, 1900, 2045, 2195, 2205, 2716, 2811, 2827, 2912, 3109, 3172, 3183, 3216, 3316, 3646], 'proposed': [755], 'HoMS-based': [757, 823, 966, 3558], 'photoreactors.23': [758], 'Effectively': [759], 'atmosphere': [765, 3605], 'necessitates': [766], 'heightened': [768], 'affinity': [769, 1332], 'between': [770, 1845, 2359, 3064, 3307], 'accompanied': [774, 2331, 2838], 'enlarged': [778], 'area': [780, 2744, 2807], 'kinetic': [783, 999, 1363, 2641], 'selectivity': [784, 1000, 3870, 3936, 3973, 3991], 'CO2/N2.24,25': [786], 'Additionally,': [787, 2210, 2571, 2889, 3077], 'it': [788, 812, 1342], 'crucial': [790, 3317], 'fast': [794, 2858], 'boosted': [805], 'reaction.26': [807], 'meet': [809], 'requirements,': [811], 'become': [814], 'imperative': [815], 'meticulously': [817], 'customize': [818], 'local': [820, 2347], 'environment': [821, 1856, 1919, 2348], 'photoreactors,': [824], 'ensuring': [825], 'optimal': [826], 'conversion.': [831], 'Accordingly,': [832, 3279], 'construction': [835], 'multishells,': [839], 'resulting': [841, 1027, 1409, 1707, 2429, 2923, 3052, 3210], 'composite': [842, 1030, 2286], 'can': [844, 879, 1312, 2556, 2576, 2754, 3193, 3696], 'be': [845, 1313, 1606, 2247, 2500, 2557, 2605, 2774, 3194, 3697], 'optimized': [847], 'enhance': [849, 881, 1330, 1387], 'its': [850], 'performance': [851, 3325, 3521, 3615], 'targeted': [853], 'electron': [857, 1145, 1646, 1931, 2965, 2980], 'reactions.': [864], 'Building': [865], 'upon': [866], 'metal': [867, 875], 'oxide': [868], '(MO)': [869], 'photocatalysts,': [871], 'integration': [873], 'organic': [876], 'frameworks': [877], '(MOFs)': [878], 'pores': [888, 906, 1062], 'provide': [890], 'additional': [891, 1203, 2021, 2904], 'sites': [893, 3083], 'adsorption.27–30': [896], 'characteristics': [899, 2781], 'elevate': [902], 'utilization': [904, 3672], 'MOFs': [908, 922], 'self-supported': [911], 'well-aligned': [913], 'MO/MOFs': [914], 'heterostructure.': [916], 'tunable': [918], 'micropores': [919], 'present': [920], 'within': [921, 936, 2990, 3919], 'opportunity': [926], 'molecular': [928, 1423, 4031], 'sieving,': [929], 'enabling': [930], 'mesopores': [938], 'shells': [941, 1289, 1670, 1881, 3926], 'HoMS.31': [945], 'complementary': [947], 'roles': [948], 'two': [950, 1716, 2453, 3066], 'counterparts': [951, 1448, 1717], 'may': [952, 1382, 2275], 'improve': [953], 'kinetics,': [957, 2356], 'contributing': [960], 'overall': [963, 3122], 'photoreactors.': [967], 'Herein,': [968], 'select': [970], 'prototypical': [972], '(ZIF-8),': [976], 'also': [977, 1120, 1158, 2913, 3984], 'known': [978], 'metal-azolate': [980], 'framework-4': [981], 'initially': [983], 'reported': [984, 1209, 1403, 3580, 3583], 'Chen': [987], 'group,32': [988], 'possesses': [990], 'high': [991, 3971], 'intrinsic': [992], 'stability,': [994], 'activity,': [996, 1087, 2636], 'CO2/N2,': [1002], 'modify': [1004], 'HoMS.': [1009, 1947, 1962, 2178], 'Through': [1010], 'controlled': [1011, 1291, 1502, 2303], 'in-situ': [1012], 'growth,': [1013], 'layers': [1015, 1286, 1602, 3929], 'uniformly': [1017], 'formed': [1018], 'both': [1020, 1701, 3161, 3951], 'inner': [1022, 1451], 'outer': [1024, 1453], 'heterointerfaces.': [1035, 1926, 2379, 2852, 3142], 'Enriched': [1036], 'observed': [1044, 2230, 3370, 3567], 'abundant': [1051, 2847], 'supply': [1052, 1151], 'Zn2+': [1054, 1279, 2306, 2564, 2794, 3206, 3212], 'ions': [1055, 1280, 1813, 1859, 2086, 2795, 3207], 'multiple': [1057], 'shells.': [1058], 'Significantly,': [1059], 'increased': [1061, 3079, 3340, 3821, 3826], 'boost': [1071], 'kinetics.': [1078, 2367], 'Synergistically,': [1079], 'strengthens': [1084], 'affording': [1088], '3S': [1089, 1656, 1839, 1912, 1945, 1960, 1967, 1971, 2388, 2465, 2520, 3421, 3444, 3595, 3758, 3843, 3855, 3966], 'highest': [1093, 1113, 3414, 3451], 'atmospheres': [1101, 3729], 'airflow': [1106], '100%': [1109, 3409], 'selectivity,': [1110, 3411], 'reaching': [1111, 3424], 'production': [1115, 1162], 'We': [1119, 2414], 'demonstrate': [1121, 2171], 'applications': [1129], 'ability': [1147, 3829], 'ensure': [1148], 'tandem': [1154, 3700], 'system,': [1156, 2315], 'demonstrates': [1159, 1830], 'CO2-to-C2': [1161], 'feeding': [1166, 3728], '(Scheme': [1167], '1).': [1168], 'Scheme': [1169], '1': [1170, 1928, 2620, 3890], '|': [1171, 1929, 2672, 3837], 'Illustration': [1172, 2674], 'composited': [1175, 3619, 3675], 'toward': [1184, 1339, 3336], 'reduction.': [1187], 'Experimental': [1192], 'Commercially': [1193], 'available': [1194], 'reagents': [1195], 'starting': [1197, 1438], 'materials': [1198, 2408, 2455], 'were': [1199, 1206, 1218, 1255], 'utilized': [1200, 2971], 'without': [1201], 'any': [1202], 'purification': [1204], 'prepared': [1207], 'using': [1208, 1221, 2401, 3702, 3944], 'methods': [1210], 'specified.': [1212], 'All': [1213, 3405], 'reactions,': [1214], 'unless': [1215], 'stated': [1216], 'otherwise,': [1217], 'carried': [1219], 'out': [1220, 1347], 'dry': [1222], 'solvents': [1223], 'autoclaves': [1225], 'vials': [1227], 'had': [1229], 'dried': [1231], 'sealed': [1233], 'air': [1236, 3610], 'atmosphere.': [1237], 'Briefly,': [1238], 'synthesis': [1240, 2284], 'follows': [1244], 'sequential': [1246, 1259], 'templating': [1247], 'approach,': [1248], 'Zn': [1251, 1475, 1774, 1811, 1836, 1858, 1921, 1993, 2042, 2085, 2679, 3006], 'precursor-enriched': [1252], 'carbonaceous': [1253], 'spheres': [1254, 1570], 'adopted': [1256, 1494], 'templates.': [1260], 'fabrication': [1262], 'then': [1267, 1818, 2370, 2812, 3448], 'applied': [1268], 'DMF-based': [1271], 'liquid': [1272], 'phase,': [1273], 'dissolution': [1277, 1503, 2297, 2326, 2336, 2344, 2355, 2598, 2628, 2634, 3310], 'growth': [1283, 1445, 1694, 2069, 2317], 'concentration': [1294], 'ligands.': [1296], 'experimental': [1299, 2412], 'details': [1300, 2800], 'regarding': [1301, 3998], 'syntheses': [1303], 'characterization': [1305, 1324], 'compounds': [1307], 'mentioned': [1308], 'study': [1311], 'accessed': [1314], 'Supporting': [1317, 1525, 1546, 1592, 1636, 1739, 1800, 1893, 2033, 2153, 2239, 2488, 2541, 2546, 3043, 3146, 3401, 3474, 3506, 3540, 3627, 3663, 3711, 3956], 'Information.': [1318], 'Results': [1319], 'Discussion': [1321], 'Fabrication': [1322], 'MO-based': [1335], 'essential': [1344], 'carry': [1346], 'appropriate': [1348], 'modifications': [1349], 'enrich': [1351], 'pore': [1353], 'distribution': [1354, 1680], 'increase': [1356, 2106, 3550, 3808], 'area.33': [1360], 'Considering': [1361], 'diameters': [1364], '(3.30': [1367], 'Å)': [1368, 1372], 'N2': [1370, 3790, 3954], '(3.64': [1371], 'micropore': [1377], 'size': [1378], '3.4': [1380], 'Å': [1381], 'induce': [1383], 'molecule': [1384], 'molecules.34': [1393], 'Further': [1394], 'compositing': [1395], 'MO': [1400], 'substrates': [1401], 'fix': [1405], 'ligand': [1407], 'rotation,': [1408], 'lattice': [1412], 'rigidity.35': [1413], 'This': [1414, 1550, 2074, 3560], 'specific': [1415], 'advantages': [1419], 'achieving': [1421], 'precise': [1422, 3915], 'particularly': [1428], 'when': [1429, 3158], 'dealing': [1430], 'concentrations.': [1433], 'goal,': [1437], 'photoactive': [1441], 'HoMS,': [1443, 2184, 2783], 'surfaces': [1454], 'conducted': [1459], 'following': [1460], 'reaction:': [1462], '+': [1464, 1485], '2': [1465, 1472, 1482, 1484, 1487, 2671], '(': [1466, 1476, 1524, 1545, 1591, 1635, 2032, 2238, 2487, 2545, 2616, 3042, 3473, 3505, 3662, 3710, 3955], 'C': [1467, 1477], '4': [1468, 1478], 'H': [1469, 1479, 1486], '6': [1470], 'N': [1471, 1481, 1866, 4011], ')': [1473, 1483, 2618], '→': [1474], '5': [1480], 'O(1)': [1488], 'A': [1489], 'diluted': [1490], '2-MIM': [1491, 2132, 2181, 2360], 'fabricating': [1496, 2253], 'HoMS@ZIF-8,': [1498, 1577, 1841, 1914, 2467, 3423], 'nucleation': [1507, 1520, 2292], 'substrate,': [1515], 'avoiding': [1517], 'homogeneous': [1519], 'crystals': [1523], 'Information': [1526, 1547, 1593, 1637, 1740, 1801, 1894, 2034, 2154, 2240, 2489, 2542, 2547, 3044, 3147, 3402, 3475, 3507, 3541, 3628, 3664, 3712, 3957], 'Figure': [1527, 1548, 1564, 1594, 1638, 1651, 1689, 1741, 1828, 1895, 1927, 2035, 2155, 2241, 2490, 2543, 2670, 2809, 2833, 2982, 3009, 3045, 3118, 3148, 3403, 3476, 3508, 3542, 3665, 3713, 3769, 3835, 3958], 'S1).36': [1528], 'By': [1529], 'optimizing': [1530], 'time,': [1532], 'full': [1534], 'coverage': [1535], 'layer': [1539, 1698, 2321, 2475, 3741], 'good': [1541], 'crystallinity': [1542], 'realized': [1544], 'S2).': [1549, 2549], 'development': [1551], 'applicable': [1553], 'numbers.': [1560], 'As': [1561, 1760, 2150, 2380, 3143, 3537], 'shown': [1562, 1891, 2151], '1a–c,': [1565], 'single-shelled': [1567], '@ZIF-8': [1571], '(ZnO': [1572], 'HS@ZIF-8),': [1573], 'double-shelled': [1574], '(2S)': [1575], 'triple-shelled': [1579], '(3S)': [1580], 'maintain': [1583], 'integrity': [1585, 3633], 'nano-microstructure': [1588], 'after': [1589, 2067, 2431, 3651, 3782], 'transformation': [1590, 2860], 'S3).': [1595, 3630], 'thickness': [1597], 'covered': [1600], 'was': [1603, 3748, 3910], 'measured': [1604], 'approximately': [1607, 3425], '53': [1608], 'nm': [1609, 3459], 'all': [1611], 'structures,': [1612], 'providing': [1613, 2903, 3653, 3716], 'consistent': [1615], 'platform': [1616], 'studying': [1618], 'merits': [1620], 'brought': [1621], 'about': [1622, 2023], 'scaffold': [1626, 2251], 'MO/MOF': [1629], 'uniform': [1632], 'heterostructures': [1634], 'S4).': [1639], 'high-angle': [1641], 'annular': [1642], 'darkfield': [1643], 'scanning': [1644], 'transmission': [1645], 'microscopy': [1647, 1932], '(HAADF-STEM)': [1648], 'image': [1649, 1950, 1976, 2686], '1d': [1652], 'single': [1655, 1959], 'clearly': [1659, 2863], 'illustrates': [1660, 2984], 'different': [1662, 1752, 2579, 3137, 3252, 3762, 3847, 3862], 'contrasts': [1663], 'result': [1665, 2785], 'rigid': [1668], 'flexible': [1672], 'layer.': [1674, 2073], 'Moreover,': [1675, 2964, 3631], 'carbon/nitrogen': [1677], '(C/N)': [1678], 'element': [1679], 'dispersive': [1683], 'spectral': [1684], '(EDS)': [1685], 'mapping': [1686, 1955], 'images': [1687, 1934, 1956, 2697, 2727], '1e': [1690], 'indicates': [1691], 'happens': [1699], 'sides': [1702], 'sandwich-like': [1709], 'heteroshells.': [1710], 'crystal': [1712, 2343, 2450, 2841, 2871, 2905, 2940, 3230], 'investigated': [1719, 2416, 3749], 'powder': [1721], 'X-ray': [1722, 1743, 1821, 1887, 1953, 2015], 'diffraction': [1723], '(XRD)': [1724], 'analysis,': [1725, 3881], 'shows': [1727], 'well-crystalized': [1728], 'hexagonal': [1729], 'wurtzite': [1730, 2867], 'cubic': [1733], 'phases': [1735], '(Figure': [1736, 1758, 1797, 2338, 2887, 2907, 2962, 3624, 3933], '1f': [1737], 'S5).': [1742], 'EDS': [1744, 1954, 1983], 'results': [1745, 1984, 2019, 2234, 2855, 3187, 3239, 3772], 'selected': [1747, 1987, 2720, 2743, 2806, 3242], 'areas': [1748], 'further': [1749, 2139, 2534, 3095, 3526, 4003], 'confirmed': [1750, 2140, 3647], '1g).': [1759], 'compared': [1761, 3616, 3976], 'area-1': [1763], 'red': [1765, 2708, 2830], 'dotted': [1766], 'lines,': [1767], 'percent': [1770], 'O': [1772, 2227], 'dramatically': [1775], 'decreased': [1776], '9.0%': [1778], '2.3%': [1780], '7.7%': [1782], '1.5%,': [1784], 'suggesting': [1785, 2767, 2843, 2942, 2952], 'main': [1790], 'counterpart': [1791], '1h': [1798], 'Table': [1802, 2548, 3629], 'S1).': [1803], 'electronic': [1805], 'coordination': [1808, 1855, 1918, 3093, 3642], 'environments': [1809, 2028], 'central': [1812], 'studied': [1819], 'absorption': [1822, 1888], 'edge': [1824, 3080], '(XANES)': [1826], 'spectra.': [1827], '1i': [1829], 'negative': [1832], 'shift': [1833, 2075, 3014], 'K-edge': [1837, 1994], 'positioned': [1844], 'edges': [1848], 'ZIF-8.': [1852], 'altered': [1854], 'attributed': [1861, 2196, 2471, 2558, 3195], 'incorporation': [1864], 'atoms,': [1867], 'increases': [1869, 3472], 'number': [1871, 3056, 3094, 3396], 'electrons.': [1873], 'changes': [1875], 'Zn-O': [1878, 2091], 'Zn-N': [1880, 2094], 'revealed': [1883], 'extended': [1886], 'fine': [1889], 'S6.': [1896], 'peak': [1898, 2108, 2213, 3003], 'positions': [1899], 'quite': [1901, 3233], 'similar,': [1902], 'except': [1903], 'slight': [1906, 3013], 'decrease': [1907, 2080, 2516, 3268], 'bond': [1909], 'length': [1910], 'indicating': [1915, 2710, 3020, 3120], 'distorted': [1917], 'atoms': [1922, 3089], 'around': [1923, 2215], 'Transmission': [1930], '(TEM)': [1933], '(a)': [1936, 2673, 3838], 'HS@ZIF-8;': [1938], '(b)': [1939, 2684, 3850], '2S': [1940], 'HoMS@ZIF-8;': [1942], '(c)': [1944, 3866], '(d)': [1948, 3875], 'HAADF-STEM': [1949, 1975], '(e)': [1952, 3879], '(f)': [1963, 3883], 'XRD': [1964, 2462], 'patterns': [1965, 2463, 2718, 2862], 'HoMS@ZIF-8.': [1973, 2209, 3129], '(g)': [1974], '(h)': [1981], 'corresponding': [1982, 1996, 2030, 2116, 2160, 3873], 'area.': [1988], '(i)': [1989], 'XANES': [1990], 'spectra': [1991, 2170, 3885], 'samples,': [1997], 'inset': [2000], 'showing': [2001], 'magnified': [2003], 'edges.': [2005], 'compositional': [2012, 3221], 'variation,': [2013], 'surface-sensitive': [2014], 'photoelectron': [2016], 'spectroscopy': [2017, 2146, 2968], '(XPS)': [2018], 'information': [2022], 'change': [2025, 3263], 'elements': [2031], 'S7).': [2036], 'high-resolution': [2038, 2815], 'XPS': [2039, 2233], 'peaks': [2040, 2159, 2186, 2470, 3256], '2p,': [2043], 'located': [2046], 'at': [2047, 2111, 2214, 2645, 3084, 3139, 3244, 3568], '1021.8': [2048], 'eV': [2049, 2054, 2066, 2115], '(Zn': [2050, 2055], '2p3/2)': [2051], '1044.9': [2053], '2p1/2),': [2056], 'shifted': [2058], 'higher': [2061], 'binding': [2062], 'due': [2077, 3026, 3271, 3830], 'valence': [2082, 3024], 'electrons': [2083, 2099, 3041], 'alteration': [2089], 'bonds': [2092], 'bonds,': [2095], 'involves': [2097], 'hybridized': [2102], 'orbitals.29': [2103], 'intensity': [2109, 2481, 3270], 'centered': [2110], '284.8': [2112], '286.0': [2114], 'sp2': [2118], 'C–C': [2119, 2165], 'bonding': [2120, 2127], 'sp2-hybridized': [2123], 'N–C=N': [2126], 'verifies': [2128], 'existence': [2130], 'ligands': [2133], 'surface,': [2136], 'Fourier': [2142, 2859], 'transform': [2143], 'infrared': [2144], '(FTIR)': [2145], 'Raman': [2148, 2169, 3884], 'results.': [2149], 'S8,': [2156], 'Zn–N,': [2162], '–C–N,': [2163], 'vibrations': [2166, 2201], 'introduction': [2173, 3375], 'Compared': [2179, 2459], '800': [2189], '1500': [2191], 'cm−1': [2192], 'range,': [2193], 'typical': [2199, 2866], 'skeletal': [2200], 'aromatic': [2203], 'heterocycles,': [2204], 'well-preserved': [2206], 'broad': [2212], '3400': [2216], 'cm−1,': [2217], 'assigned': [2219], 'hydroxyl': [2223], 'groups,': [2224], 'explains': [2225], '1s': [2228], 'signal': [2229], 'S9).': [2242], 'proven': [2245], 'composites,': [2255, 3285], 'owing': [2256], 'exceptional': [2259, 2787], 'properties.37': [2262], 'It': [2263, 3223], 'noteworthy': [2265, 3225], 'confinement': [2268], 'potentially': [2276, 2773], 'influence': [2277, 2423], 'properties': [2279, 2375, 3126, 3322], 'during': [2282, 3280], 'structures.': [2287, 2570, 2981], 'initiation': [2289], 'triggered': [2294], 'substrates,': [2300, 2362], 'flux': [2307, 2562, 4032], 'liquid–solid': [2310], 'interface.': [2311], 'occurs': [2322, 3918], 'concomitantly': [2323], 'ZnO,': [2328], 'progression': [2334], 'pits': [2337, 2948, 2958, 3116], '2a).': [2339], 'According': [2340], 'theory,': [2345], 'nanostructures': [2351], 'influences': [2352], 'interplay': [2358], 'crystallization': [2366], 'These': [2368, 3214, 3314], 'factors': [2369, 3315], 'shape': [2371], 'distinct': [2373, 2454, 2584, 2778], 'physicochemical': [2374, 2420, 3321], 'comparison,': [2382], 'disrupted': [2384], 'grinding': [2392], 'obtained': [2394, 3938], 'batch': [2396], 'NPs@ZIF-8': [2399, 2485, 2527, 3134, 3249, 3982], 'samples': [2400, 2486, 3135, 3250, 3406, 3860, 3888], 'afforded': [2403], 'debris': [2405], 'raw': [2407], 'same': [2411], 'conditions.': [2413], 'thoroughly': [2415], 'properties,': [2421], 'heterojunction': [2425], 'interfaces': [2426, 3246], 'transformation,': [2432], 'focus': [2435], 'impact': [2438, 2976, 3512], 'structure.': [2442, 3278], 'Initially,': [2443], 'analyzed': [2445], 'composition': [2448, 2575, 3294], 'macroscopic': [2457, 3292], 'characterizations.': [2458, 3222], 'exhibited': [2476, 3969], 'S10).': [2491], 'content': [2493], 'components': [2498], 'could': [2499, 2604, 2772, 3598], 'estimated': [2501], 'ratios': [2504], 'intensities': [2506], '(010)': [2509], '(101)': [2512], 'peaks.': [2513], '1.65': [2518], '0.57': [2524], 'confirms': [2528], 'suppressed': [2530], 'conversion,': [2531], 'evidenced': [2535, 3495], 'thermogravimetric': [2538], 'analysis': [2539, 3871], 'S11': [2544], 'Therefore,': [2550], 'variations': [2552, 2573], 'limited': [2561, 3174, 3189], 'caused': [2565], 'broken': [2568], 'lead': [2577], 'heterointerfaces,': [2581, 3051], 'possess': [2583], 'chemical,': [2585], 'energy,': [2587], 'strain': [2589], 'properties.': [2591], 'Focusing': [2592], 'advancement': [2595], 'pits,': [2599], 'step': [2601, 3190], 'rate': [2602, 3383, 3593], 'v': [2603, 2608, 2762], 'described': [2606, 2661], 'as:': [2607, 2662], '=': [2609, 2664, 4013], 'ω': [2610, 2622], 'β': [2611, 2638], 'e': [2613, 2668], '{': [2614], 'exp': [2615], 'σ': [2617, 2652, 2663], '−': [2619, 4014], '}(2)where': [2621], 'volume': [2625, 3764, 3864], 'unit,': [2629], 'ae': [2630], 'equilibrium': [2633], 'unit': [2635], 'coefficient': [2642], '(remains': [2643], 'constant': [2644], 'given': [2647], 'temperature': [2648], 'additive': [2650], 'concentration).38': [2651], 'defined': [2654], 'undersaturation': [2657], 'degree,': [2658], 'ln': [2665], '(3)': [2669, 2760], 'formation': [2677], 'flux-driven': [2680], 'steps.': [2683, 2714], 'TEM': [2685], 'heterointerface.': [2690, 2928], '(c,': [2691, 2735, 2746], 'd)': [2692], 'High-resolution': [2693], 'spherical': [2694, 2816], 'aberration-corrected': [2695, 2817], 'STEM': [2696, 2726, 2818], 'heterointerface': [2700, 2771, 3171, 3379], 'viewed': [2701, 2897, 3159], '[001]': [2703, 3162], '[100]': [2705, 2901, 3164], 'faces': [2706], 'arrows': [2709, 2831], 'atom': [2713, 3059], 'Insets': [2715], 'FFT': [2717], 'areas.': [2721], '(e,': [2722], 'f)': [2723], 'Simulated': [2724], 'illustrations': [2729], 'd).': [2736, 2747], '(g,': [2737], 'h)': [2738], 'EELS': [2739, 2988, 3112, 3238], 'acquired': [2740], 'Hence,': [2752], 'deduce': [2755], 'eqs': [2757], '(2)': [2758], 'proportional': [2764], 'a,': [2766], 'influenced': [2775], 'nanostructures,': [2788], 'arising': [2789], 'surface.39': [2798], '2b': [2810], 'inspected': [2813], 'images.': [2819], 'Two': [2820], 'states': [2822], 'observed.': [2828, 3185], '2c': [2834], 'indicate': [2835, 3188, 3773], 'indented': [2836], 'configurations': [2837, 3231], 'pitted': [2840], 'surfaces,': [2842], 'presence': [2845, 2944, 2954], 'simulation': [2854], '(FFT)': [2861], 'illustrate': [2864], 'orientation': [2872], '[001].': [2874], 'interface': [2876, 2933, 3181, 3235, 3277, 3297], 'verified,': [2883], 'designated': [2884], '(100)/(010)': [2886], '2e).': [2888], 'another': [2890], 'representative': [2891], 'exposed': [2892], 'facet': [2893], 'orientation,': [2902], '2d).': [2908], 'witnessed': [2914], 'coarse': [2917], 'grind,': [2922], 'blurry': [2926], 'verified': [2935, 3486], 'simulated': [2938, 3229], 'configuration,': [2941], '(010)/(001)': [2947, 2957, 3115], '2f).': [2963], 'loss': [2967], '(EELS)': [2969], 'monitor': [2973], '2a': [2983], 'collection': [2986], 'data': [2989], 'three': [2991], 'regions:': [2993], 'crystal,': [2996], 'interface,': [2998], 'counterparts.': [3001], 'position': [3004], 'L2,3': [3007], '2g': [3010], 'exhibits': [3011, 3547, 3778], 'towards': [3015], 'lower': [3017, 3092], 'direction,': [3019], 'state': [3025], 'transition': [3029], '[ZnO4]': [3032], 'tetrahedron': [3033], '[ZnN4]': [3036], 'tetrahedron,': [3037], 'provides': [3039], 'extra': [3040], 'S12).40': [3046], 'large': [3055], 'steps,': [3060], 'creates': [3061], 'close': [3062], 'interactions': [3063], 'counterparts,': [3067], 'generating': [3068], 'unbalanced': [3070], 'electric': [3071, 3101], 'field': [3072], 'enhances': [3074, 3381], 'transfer.': [3076], 'corner': [3082], 'where': [3087], 'activate': [3096], 'stabilize': [3099], 'dipole': [3102], 'intermediates': [3104], '(e.g.,': [3105], '*CO2).25': [3106], 'Similar': [3107], 'observations': [3108], 'made': [3110], '2h,': [3119], 'contrast,': [3131], 'exhibit': [3136, 3251, 3407], 'depicted': [3144, 3399, 3538], 'S13,': [3149], 'grinds': [3154], 'appears': [3155], 'much': [3156], 'smoother': [3157], 'perspectives.': [3165], 'Surface': [3166], 'typically': [3173], '2–3': [3176], 'layers,': [3178], 'rarely': [3184], 'propagation,': [3191], 'inability': [3198], 'NPs': [3201], 'localize': [3203], 'dissolved': [3205], 'insufficient': [3211], 'flux.': [3213], 'findings': [3215, 3668], 'line': [3218], 'although': [3227], 'confirm': [3232], 'similar': [3234, 3618, 3622], 'geometries,': [3236], 'regions': [3243], 'trends.': [3253], 'L2,3-edge': [3259], 'show': [3260], 'no': [3261], 'but': [3264], 'there': [3265], 'regular': [3275], 'preparation': [3282], 'impacts': [3290], 'microscopic': [3296], 'product': [3301], 'influencing': [3303], 'reactions': [3306, 3701], 'substrate': [3309], 'growth.': [3313], 'defining': [3319], 'as-synthesized': [3328], 'hybrid': [3329], 'materials,': [3330], 'efficiency': [3335], 'affinity.41': [3341], 'Next,': [3349], 'proceed': [3351], 'assess': [3353], 'activity': [3358, 3755, 3781, 3841, 3853], 'investigate': [3364], 'underlying': [3366], 'mechanism': [3367, 3902], 'enhancement': [3371], 'activity.': [3373], 'evolution,': [3386], 'promotion': [3389, 3901], 'becoming': [3390], 'prominent': [3392], 'increases,': [3397], 'S14.': [3404], 'nearly': [3408], '161': [3426], 'μmol/h/g': [3427, 3433], 'H2O': [3429], 'vapor': [3430], '393': [3432], 'sacrificial': [3436], 'reagent.': [3437], 'apparent': [3439], 'quantum': [3440], '(AQY)': [3442], 'studied.': [3449], 'AQY': [3452], '0.091%': [3454], '300': [3458], 'monochromatic': [3460], 'irradiation,': [3462], 'drops': [3464], 'sharply': [3465], 'wavelength': [3468], 'S15).': [3477], 'origin': [3479], 'produced': [3482], 'stem': [3488], 'use': [3498], '13CO2': [3500], 'isotopic': [3503], 'tracer': [3504], 'S16).': [3509], 'beneficial': [3511], 'validated': [3527], 'catalyst': [3531, 3578], 'loading': [3532, 3554, 3570], 'reactor.': [3536], 'S17,': [3543], 'linear': [3549, 3941], 'augmented': [3553], 'amount': [3555, 3571], 'nanoreactors.': [3559], 'trend': [3561], 'continues': [3562], 'until': [3563], 'plateau': [3565], '120': [3573], 'mg,': [3574], 'surpasses': [3576], 'usage': [3579], 'most': [3582], 'studies.': [3584], 'fixed-bed': [3587], 'reactor,': [3589], 'reach': [3599], '0.76': [3607], 'flow,': [3611], 'exhibiting': [3612], 'best': [3614], '3a': [3625], 'scaffold,': [3637], 'crystallinity,': [3640], 'remain': [3649], 'intact': [3650], 'photocatalysis,': [3652], 'strong': [3654], 'evidence': [3655], 'robustness': [3658], 'S18).': [3666], 'highlight': [3669], 'abundance': [3681], 'addition,': [3684], 'subsequently': [3692], 'C2': [3694, 3725], 'H-cell': [3704], 'fitted': [3705], 'copper': [3708], 'electrode': [3709], 'S19),': [3714], 'viable': [3718], 'alternative': [3719], 'route': [3720], 'converting': [3722], 'relatively': [3731], 'concentrations.42': [3734], 'contribution': [3736], 'evaluating': [3751], 'evolution': [3754, 3840, 3852], 'grated': [3757, 3776, 3813, 3859], 'fractions,': [3765], 'illustrated': [3767], '3b.': [3770], 'mixing': [3783], '60': [3784], 'vol': [3785], '%': [3786], 'atmosphere,': [3791], 'confirming': [3792], 'multistructures': [3798], 'contributes': [3799], 'process.': [3805], 'Importantly,': [3806], 'sensitive': [3818], 'concentration,': [3823], 'revealing': [3824], 'layer.25': [3834], '3': [3836], 'gas': [3848, 4054], 'flows.': [3849], 'fractions.': [3865], 'CO2/N2': [3868, 3908, 3972], 'samples.': [3874], 'isotherms,': [3878], 'TPD': [3880], 'CO2-saturated': [3887], 'wt%': [3891], 'Au': [3892], 'loading.': [3893], 'understand': [3899], 'photoreduction,': [3906], 'system': [3909], 'employed': [3911], 'validate': [3913], 'nanoreactors,': [3923], 'feature': [3925], '3c).': [3934], 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