Publication Information

{'id': 'https://openalex.org/W4281667127', 'doi': 'https://doi.org/10.31635/ccschem.022.202201931', 'title': 'Efficient Photocatalytic Reduction of CO <sub>2</sub> Catalyzed by the Metal–Organic Framework MFM-300(Ga)', 'display_name': 'Efficient Photocatalytic Reduction of CO <sub>2</sub> Catalyzed by the Metal–Organic Framework MFM-300(Ga)', 'publication_year': 2022, 'publication_date': '2022-05-27', 'ids': {'openalex': 'https://openalex.org/W4281667127', 'doi': 'https://doi.org/10.31635/ccschem.022.202201931'}, 'language': 'en', 'primary_location': {'is_oa': False, 'landing_page_url': 'https://doi.org/10.31635/ccschem.022.202201931', 'pdf_url': None, 'source': {'id': 'https://openalex.org/S4210239486', 'display_name': 'CCS Chemistry', 'issn_l': '2096-5745', 'issn': ['2096-5745'], 'is_oa': True, 'is_in_doaj': True, 'is_core': True, 'host_organization': 'https://openalex.org/P4310311897', 'host_organization_name': 'Chinese Chemical Society', 'host_organization_lineage': 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201, 211, 220, 226, 236, 239, 258, 261, 280, 283, 300, 320, 346, 356, 361, 382, 396, 413, 428, 474, 492, 509, 516, 526, 532, 551, 556, 574, 620, 628, 646, 664, 672, 697, 702, 710, 713, 733, 738, 746, 781, 794, 851, 870, 882, 888, 902, 904, 935, 941, 943, 959, 996, 1005, 1016, 1021, 1082, 1131, 1137, 1168, 1188, 1201, 1207, 1232, 1261, 1267, 1276, 1286, 1297, 1320, 1325, 1336, 1377, 1382, 1428, 1433, 1470, 1480, 1508, 1515, 1522, 1529, 1563, 1609, 1612, 1615, 1674, 1678, 1683, 2019, 2036, 2056, 2075, 2084, 2100, 2108, 2114, 2132, 2139, 2175, 2193, 2199, 2206, 2213, 2216, 2337, 2370, 2375, 2397, 2448, 2468, 2481, 2498, 2510, 2525, 2568, 2583, 2593, 2621, 2642, 2704, 2734, 2740, 2747, 2762, 2835, 2854, 2869, 2913, 2917, 2981, 2999, 3015, 3023, 3028, 3044, 3073, 3076, 3094, 3133, 3142, 3145, 3151, 3158, 3169, 3179, 3187, 3190, 3194, 3214, 3267, 3289, 3298, 3306, 3312, 3339, 3344, 3347, 3358, 3378, 3394, 3419, 3441, 3447, 3466, 3474, 3483, 3533, 3698, 3731, 3793, 3869, 3874, 3883, 3903], 'CO2': [8, 301, 321, 347, 397, 419, 433, 569, 698, 768, 795, 839, 871, 883, 942, 1344, 1383, 1536, 1616, 1634, 1696, 2040, 2060, 2109, 2140, 2200, 2229, 2235, 2247, 2253, 2259, 2267, 2273, 2279, 2285, 2291, 2297, 2465, 2511, 2808, 2855, 2918, 2988, 3016, 3052, 3059, 3077, 3105, 3134, 3207, 3299, 3383, 3411, 3586, 3631, 3667, 3699, 3737, 3812, 3844, 3884, 3904], 'Catalyzed': [9, 3704], 'by': [10, 391, 727, 908, 917, 966, 1349, 1409, 1416, 2070, 2141, 2403, 2425, 2514, 2967, 3033, 3166, 3183, 3368, 3456, 3523, 3550, 3633, 3872, 3885], 'the': [11, 317, 335, 380, 400, 405, 410, 472, 479, 489, 506, 523, 544, 548, 552, 565, 572, 595, 662, 670, 677, 693, 700, 708, 724, 729, 774, 778, 792, 821, 838, 849, 868, 886, 892, 897, 960, 1019, 1038, 1092, 1096, 1108, 1114, 1129, 1132, 1138, 1142, 1155, 1178, 1185, 1189, 1236, 1247, 1380, 1393, 1413, 1426, 1449, 1454, 1502, 1506, 1527, 1556, 1578, 1598, 1605, 1675, 1690, 2034, 2053, 2063, 2071, 2097, 2106, 2124, 2129, 2136, 2180, 2190, 2202, 2357, 2368, 2378, 2434, 2446, 2464, 2493, 2506, 2522, 2532, 2550, 2565, 2581, 2584, 2589, 2610, 2638, 2643, 2670, 2676, 2702, 2713, 2718, 2732, 2744, 2760, 2807, 2813, 2825, 2833, 2840, 2852, 2914, 2942, 2945, 2952, 2957, 2961, 2968, 2974, 2994, 3012, 3019, 3026, 3042, 3050, 3057, 3063, 3071, 3103, 3130, 3140, 3148, 3156, 3159, 3167, 3176, 3184, 3199, 3202, 3212, 3286, 3296, 3345, 3356, 3359, 3364, 3369, 3374, 3381, 3392, 3407, 3417, 3460, 3464, 3475, 3481, 3492, 3497, 3531, 3555, 3569, 3880], 'Metal–Organic': [12], 'Framework': [13], 'MFM-300(Ga)': [14, 349, 378, 790, 899, 928, 997, 1017, 1083, 1169, 1233, 1268, 1277, 1298, 1347, 1378, 1474, 1509, 1523, 1647, 1679, 1731, 2194, 2226, 2238, 2244, 2250, 2256, 2301, 2482, 2503, 2526, 2631, 2873, 2938, 3024, 3048, 3108, 3331, 3379], 'Tian': [15, 49, 3657], 'Luo,': [16], 'Zi': [17, 61], 'Wang,': [18], 'Xue': [19, 83], 'Han,': [20], 'Yinlin': [21, 95], 'Chen,': [22], 'Dinu': [23, 107], 'Iuga,': [24], 'Daniel': [25, 119], 'Lee,': [26], 'Bing': [27, 135], 'An,': [28], 'Shaojun': [29, 147], 'Xu,': [30], 'Xinchen': [31, 159], 'Kang,': [32], 'Floriana': [33, 171], 'Tuna,': [34], 'Eric': [35, 193], 'J.': [36, 194, 3655, 3762, 3774], 'L.': [37, 195, 3768], 'McInnes,': [38], 'Lewis': [39, 217], 'Hughes,': [40], 'Ben': [41, 232], 'F.': [42, 233], 'Spencer,': [43], 'Martin': [44, 245], 'Schröder': [45, 246], 'and': [46, 125, 222, 266, 341, 366, 394, 453, 500, 502, 512, 546, 568, 604, 611, 649, 680, 695, 731, 748, 770, 786, 803, 819, 857, 879, 911, 938, 949, 976, 988, 1026, 1032, 1050, 1095, 1103, 1173, 1214, 1220, 1223, 1242, 1258, 1289, 1299, 1306, 1333, 1359, 1367, 1412, 1457, 1505, 1545, 1547, 1559, 1565, 1680, 1725, 2061, 2104, 2121, 2135, 2177, 2201, 2204, 2263, 2343, 2372, 2382, 2414, 2421, 2458, 2470, 2496, 2508, 2518, 2535, 2544, 2558, 2573, 2588, 2637, 2690, 2776, 2784, 2791, 2799, 2881, 2897, 2941, 2956, 3087, 3135, 3196, 3205, 3264, 3274, 3308, 3320, 3380, 3398, 3432, 3437, 3463, 3470, 3503, 3525, 3547, 3554, 3590, 3635, 3905], 'Sihai': [47, 267], 'Yang': [48, 268, 3759], 'Luo': [50], 'Department': [51, 63, 85, 97, 109, 121, 137, 149, 173, 197, 219, 235, 257, 279], 'Chemistry,': [53, 65, 87, 99, 139, 151, 163, 175, 199, 259, 281], 'University': [54, 66, 76, 88, 100, 112, 128, 140, 152, 176, 186, 200, 210, 225, 238, 260, 282, 3465, 3482, 3532], 'Manchester,': [56, 68, 78, 90, 102, 130, 142, 154, 178, 188, 202, 212, 227, 240, 262, 284], 'Manchester': [57, 69, 79, 91, 103, 131, 143, 155, 179, 189, 203, 213, 228, 241, 263, 285, 3467], 'M13': [58, 70, 80, 92, 104, 132, 144, 156, 180, 190, 204, 214, 229, 242, 264, 286], '9PL': [59, 71, 81, 93, 105, 133, 145, 157, 181, 191, 205, 215, 230, 243, 265, 287], ',': [60, 82, 94, 106, 118, 134, 146, 158, 170, 192, 216, 231, 244], 'Wang': [62, 3821, 3825, 3861, 3896], 'Photon': [72, 182, 206], 'Science': [73, 183, 207, 3541], 'Institute': [74, 161, 184, 208], '(PSI),': [75, 185, 209], 'Han': [84], 'Chen': [96], 'Iuga': [108], 'Physics,': [111], 'Warwick,': [114], 'Coventry': [115], 'CV4': [116], '7AL': [117], 'Lee': [120], 'Chemical': [123, 1694], 'Engineering': [124], 'Analytical': [126], 'Science,': [127, 167], 'An': [136, 2768], 'Xu': [148], 'Kang': [160], 'Chinese': [164], 'Academy': [165], 'Beijing': [168], '100190': [169], 'Tuna': [172], 'McInnes': [196], 'Hughes': [218], 'Earth': [221], 'Environmental': [223], 'Sciences,': [224], 'Spencer': [234], 'Materials,': [237], '*Corresponding': [247, 269], 'authors:': [248, 270], 'E-mail': [249, 253, 271, 275], 'Address:': [250, 254, 272, 276], '[email': [251, 255, 273, 277], 'protected]': [252, 256, 274, 278], 'https://doi.org/10.31635/ccschem.022.202201931': [288], 'SectionsSupplemental': [289], 'MaterialAboutAbstractPDF': [290], 'ToolsAdd': [291], 'to': [292, 302, 312, 431, 443, 461, 478, 505, 521, 584, 668, 691, 756, 764, 808, 848, 873, 891, 920, 1141, 1184, 1438, 1573, 2128, 2328, 2418, 2492, 2563, 2579, 2600, 2680, 2758, 2794, 2816, 2832, 2951, 2989, 3018, 3049, 3065, 3111, 3120, 3300, 3449, 3563, 3700, 3784], 'favoritesDownload': [293], 'CitationsTrack': [294], 'Citations': [295], 'ShareFacebookTwitterLinked': [296], 'InEmail': [297], 'reduction': [299, 663, 1381, 1635, 2447, 2916, 3064, 3075, 3144], 'carbon': [303, 2054], 'fuels': [304], 'is': [305, 843, 900, 1145, 1182, 1524, 1548, 1555, 1582, 1623, 2043, 2059, 2091, 2195, 2474, 2489, 2598, 2632, 2640, 2650, 2663, 2678, 2692, 2697, 2737, 2812, 2839, 2931, 2939, 3081, 3109, 3127, 3181, 3430, 3444], 'an': [306, 804, 846, 939, 1002, 1171, 1198, 3327, 3402, 3677], 'important': [307, 659, 2098, 3403], 'target': [308], 'but': [309, 3054], 'highly': [310, 1056], 'challenging': [311], 'achieve.': [313], 'Here,': [314], 'we': [315, 771], 'report': [316, 772, 1585, 3285], 'efficient': [318, 429, 719, 779, 3282, 3399], 'photoconversion': [319], 'into': [322, 434, 796, 1537, 1577, 1617, 2014, 3078, 3139, 3845, 3907], 'formic': [323, 351, 797, 852, 1486, 1538, 1618, 2057, 2088, 2818, 3079, 3301, 3348], 'acid': [324, 352, 798, 853, 1447, 1487, 1619, 1992, 2058, 3080, 3302], 'over': [325, 348, 598, 854, 1473, 1512, 1620, 1636, 2856, 2872, 2907, 2919, 3172, 3336, 3910], 'a': [326, 354, 358, 387, 414, 575, 581, 617, 623, 800, 922, 930, 1055, 1061, 1104, 1317, 1440, 1468, 1477, 1583, 1587, 1681, 2017, 2081, 2172, 2334, 2459, 2633, 2755, 2844, 2857, 2891, 2898, 2978, 3066, 3091, 3113, 3122, 3290, 3304, 3309, 3670, 3703], 'Ga(III)-based': [327, 415], 'metal–organic': [328], 'framework': [329, 632, 2191, 2373, 2495, 2533], '(MOF)': [330, 633], 'material': [331, 962], 'using': [332, 2156, 2874, 3324], 'triethanolamine': [333, 1390], 'as': [334, 386, 449, 459, 609, 658, 845, 1392, 1425, 1467, 1541, 2179, 2438, 2512, 2652, 2754, 2764, 2876, 3031, 3084, 3281, 3326, 3363, 3528, 3530, 3676], 'sacrificial': [336, 1394, 2970, 3329], 'agent.': [337, 3330], 'Under': [338, 783, 2433], 'light': [339, 476, 784, 1248, 1661, 2315, 2884, 2936, 3318, 3415], 'irradiation': [340, 785, 1241, 1397, 1662, 2316, 3319], 'at': [342, 399, 787, 946, 1028, 1313, 1398, 1490, 2626, 2960, 3090, 3321, 3480], 'room': [343, 788, 3322], 'temperature,': [344, 789], 'photoreduction': [345, 745, 780, 869, 2853, 3132, 3297], 'yields': [350, 1197], 'with': [353, 799, 1001, 1037, 1060, 1088, 1107, 1121, 1154, 1269, 1278, 1316, 1443, 1592, 1655, 2077, 2093, 2309, 2540, 2701, 2772, 2886, 2977, 3270, 3303, 3341, 3386, 3423, 3468, 3571, 3669, 3739, 3787, 3876], 'selectivity': [355, 802, 3305], '100%,': [357], 'high': [359, 875, 877, 1478, 3310], 'productivity': [360, 625, 806, 1479, 2083, 3311, 3346], '502': [362, 809, 1481, 1741, 2230, 3313], '±': [363, 810, 1482, 3314], '18': [364, 811, 1483, 3315], 'μmol·gcat−1·h−1,': [365, 812], 'excellent': [367, 805, 2699, 3333], 'catalytic': [368, 647, 2719, 2926, 3334], 'stability.': [369], 'In': [370, 441, 754, 1350, 2864, 3350], 'situ': [371, 830, 1351, 2516, 2722, 2865, 3035, 3351], 'electron': [372, 592, 831, 985, 990, 2969, 3115, 3328], 'paramagnetic': [373, 832], 'resonance': [374, 833], 'spectroscopy': [375, 835, 1013, 1053, 1166], 'reveals': [376], 'that': [377, 837, 994, 1206, 1235, 1476, 2052, 2062, 2189, 2478, 2504, 2630, 2806, 2843, 3011, 3293], 'promotes': [379, 3041], 'generation': [381, 3357], 'CO2•−': [383, 2990, 3123, 3360], 'radical': [384, 840, 2714, 2809, 2821, 2847, 2991, 3124, 3361], 'anions': [385], 'reaction': [388, 1471, 1516, 1640, 2064, 2436, 2826, 2930, 3365], 'intermediate': [389, 847, 2815, 2846, 3366], 'driven': [390, 2069], 'strong': [392, 703, 880, 1089, 3013, 3152, 3370, 3395], 'binding': [393, 881, 1337, 2103, 2138, 2509, 3014, 3396], 'activation': [395, 696, 3157], 'molecules': [398, 884, 1345, 3017, 3053, 3171], 'bridging': [401, 893, 3020, 3375], '–OH': [402, 894, 1340], 'sites': [403, 637, 683, 1338, 1576, 2501, 3022, 3397], 'within': [404, 1346], 'pore.': [406], 'This': [407, 494, 1742, 2187, 2488, 2804, 3009, 3061, 3452, 3485], 'study': [408], 'represents': [409], 'first': [411, 775, 2841, 3287], 'example': [412, 776, 3288], 'MOF': [416, 739, 760, 2072, 2441], 'catalyst': [417, 499, 1434, 3203], 'for': [418, 626, 661, 744, 767, 777, 825, 867, 1217, 1342, 1401, 1485, 1534, 1663, 1686, 2087, 2197, 2317, 2391, 2412, 2672, 2824, 2928, 3006, 3472, 3568, 3608, 3736, 3841, 3879], 'reduction.': [420], 'Download': [421, 423, 1370, 1372, 1666, 1668, 2921, 2923], 'figure': [422, 1371, 1667, 2922], 'PowerPoint': [424, 1373, 1669, 2924], 'Introduction': [425], 'The': [426, 957, 1072, 1194, 1229, 1264, 1374, 1404, 1420, 1464, 1519, 1580, 2394, 2410, 2596, 2618, 2645, 2686, 2910, 2925, 3262, 3511, 3560], 'development': [427], 'photocatalysts': [430, 460, 660, 824, 3422], 'convert': [432], 'value-added': [435], 'chemicals': [436], 'has': [437, 761, 963, 1384, 2400, 2848, 3162, 3487], 'attracted': [438], 'much': [439, 2475], 'interest.1,2': [440], 'addition': [442], 'TiO2,': [444], 'various': [445], 'Ga-based': [446, 527, 600, 759, 817], 'semiconductors,': [447], 'such': [448, 608, 1540], 'GaN,': [450], 'GaP,': [451], 'Ga2O3,': [452], 'ZnGa2O4,': [454], 'have': [455, 518, 741, 2118], 'been': [456, 519, 742, 762, 964, 1385, 2119, 2401, 2849, 3164], 'widely': [457, 3082], 'investigated': [458], 'drive': [462], 'this': [463, 826, 1085, 1687, 2015, 2392, 2838, 2929, 3007, 3519], 'reaction.3–7': [464], 'However,': [465, 594], 'their': [466, 485, 2554, 3271], 'wide': [467], 'optical': [468, 1199], 'bandgap': [469, 545, 1200, 2703], '(Eg)': [470], 'restricts': [471], 'use': [473], 'solar': [475], 'mainly': [477], 'ultraviolet': [480, 1179], 'region,': [481, 1180], 'and,': [482], 'more': [483, 1086, 1109, 2667, 3067], 'importantly,': [484, 707, 1501, 3198], 'nonporous': [486], 'nature': [487], 'limits': [488], 'mass': [490, 2133], 'transport': [491, 2107, 2507], 'CO2.': [493, 782, 2449, 3146], 'impedes': [495], 'charge': [496, 652, 3191], 'transfer': [497, 2134, 2205, 3043], 'between': [498, 1091, 1113, 2688, 3201, 3373], 'substrate': [501, 3161], 'also': [503, 3055, 3163, 3488], 'leads': [504], 'undesirable': [507], 'recombination': [508], 'photogenerated': [510], 'electrons': [511, 2943, 2976, 3046, 3086], 'holes.8': [513], 'A': [514, 736, 1607, 2112, 3838], 'number': [515, 737], 'strategies': [517], 'exploited': [520], 'improve': [522, 547], 'photocatalytic': [524, 596, 624, 1375, 1421, 1465, 1503, 1520, 2067, 2379, 2443, 2555, 2727, 2870, 2905, 2915, 3074, 3143, 3177, 3408], 'performance': [525, 1466], 'semiconductors.': [528], 'For': [529, 615, 675, 2320, 2331, 2354], 'example,': [530, 616, 676], 'doping': [531], 'metals': [533], '(e.g.,': [534, 539], 'Ge,': [535], 'Zn)': [536], 'or': [537, 560, 580, 587, 2046, 2171], 'nonmetals': [538], 'N,': [540], 'Si)': [541], 'can': [542, 563, 590, 687, 717, 2986, 3294], 'narrow': [543], 'light-harvesting': [549], 'efficiency': [550, 597, 1422, 1521, 2131], 'resultant': [553], 'material.9–12': [554], 'Fabrication': [555], 'ultrathin': [557], 'nanosheets,': [558], 'nanowires,': [559], 'porous': [561, 3173], 'structures': [562, 2374], 'increase': [564], 'surface': [566, 933, 2454], 'area': [567, 934], 'uptake.13–15': [570], 'Meanwhile': [571], 'introduction': [573], 'cocatalyst,': [576], 'noble': [577], 'metal': [578, 1558, 1594], 'nanoparticles,': [579], 'second': [582], 'semiconductor': [583, 3273, 3292], 'construct': [585], 'Z-scheme': [586], 'heterojunction-type': [588], 'systems': [589, 740, 1562], 'promote': [591, 692, 2505, 3295], 'transfer.10,16–18': [593], 'state-of-the-art': [599, 1610], 'semiconductors': [601, 818], 'remains': [602], 'limited,': [603], 'only': [605, 1450, 1549, 3040], 'gaseous': [606, 1405, 1460], 'products': [607, 1406, 1461], 'CH4': [610], 'CO': [612, 627, 3217, 3223, 3238, 3870], 'are': [613, 655, 751, 914, 1363, 1568, 2416, 2949, 2963], 'produced.': [614], 'top-performing': [618], 'heterostructure': [619], 'Au/Al2O3/p-GaN': [621], 'shows': [622, 929, 1018, 1170, 2442, 3332], '230': [629], 'μmol·g−1·h−1.4': [630], 'Metal–organic': [631], 'materials': [634], 'incorporate': [635], 'active': [636, 682, 2499], 'fixed': [638], 'uniformly': [639], 'in': [640, 685, 829, 896, 1159, 1177, 1365, 1387, 1453, 1604, 1625, 1689, 2033, 2102, 2110, 2143, 2363, 2502, 2515, 2531, 2542, 2549, 2553, 2698, 2717, 2721, 2851, 2944, 3034, 3107, 3129, 3390, 3405, 3518, 3583, 3791], '3D': [641], 'space,': [642], 'thus': [643, 722, 2693], 'preventing': [644], 'aggregation': [645], 'centers': [648], 'potentially': [650], 'enhancing': [651], 'separation.': [653], 'MOFs': [654, 686, 711, 750, 1531, 1684, 2399, 3180], 'therefore': [656], 'emerging': [657], 'CO2,': [665, 3195], 'showing': [666, 2451, 2890], 'potential': [667, 2648, 2980, 2998, 3093], 'overcome': [669], 'barriers': [671], 'conventional': [673, 816], 'semiconductors.19,20': [674], 'intrinsic': [678, 3272], 'microporosity': [679], 'catalytically': [681], 'confined': [684], 'form': [688, 921, 2817], 'unique': [689], '"microreactors"': [690], 'adsorption': [694, 2198, 2466], 'via': [699, 885, 1570, 2066, 3116, 3536], 'formation': [701, 887, 3027], 'host–guest': [704, 3117, 3371], 'interactions.21': [705], 'More': [706, 1500], 'backbone': [709, 2534], 'consisting': [712], 'infinite': [714], 'metal-ligand': [715], 'linkages': [716], 'facilitate': [718], 'ligand-to-metal-charge-transfer': [720], '(LMCT),': [721], 'prolonging': [723], 'excitation': [725, 1303], 'lifetime': [726, 2733], 'boosting': [728, 3406], 'isolation': [730], 'utilisation': [732], 'photoinduced': [734, 2207, 2958, 2975, 3045], 'electrons.22': [735], 'tested': [743], 'CO2,19,20': [747], 'Ti-based': [749], 'particularly': [752], 'attractive.23,24': [753], 'contrast,': [755, 3102], 'date,': [757], 'no': [758, 1122, 1458, 2151, 3445], 'shown': [763, 1158], 'exhibit': [765, 998], 'activity': [766, 1376, 1504, 2126, 2444, 3178, 3409], 'conversion,': [769], 'here': [773], 'catalyzes': [791], 'conversion': [793, 3168], '100%': [801, 3307], 'up': [807, 2966], 'significantly': [813], 'higher': [814, 1525], 'than': [815, 1205, 1526, 1551, 2477, 2669, 2743], 'among': [820], 'best-behaving': [822], 'MOF-based': [823, 1621, 2858, 3421], 'reaction.': [827, 2365], 'Importantly,': [828], '(EPR)': [834], 'confirms': [836, 1234, 3355], 'anion': [841, 2810, 3362], '(CO2•−)': [842, 2811], 'generated': [844], 'production': [850], 'MFM-300(Ga).': [855, 1262, 1637, 2569, 2908, 2920], 'Results': [856], 'Discussion': [858], 'MFM-300(Ga),': [859, 2038, 2594], '[Ga2(OH)2(L)]': [860], '(H4L': [861], '=': [862, 1100, 1118, 1211, 1226, 2161, 2165, 2169, 2774, 2781, 2786, 3230, 3253], 'biphenyl-3,3ʹ,5,5ʹ-tetracarboxylic': [863, 1957], 'acid)': [864], 'was': [865, 1423, 1448, 1488, 2029, 2153, 2326, 2752, 2789, 2822, 3454, 3521], 'chosen': [866], 'due': [872, 2127, 2491], 'its': [874], 'stability,': [876], 'adsorption,': [878], 'hydrogen': [889, 1357, 2606, 3029, 3118], 'bonds': [890, 1358, 3030], 'groups': [895, 3377], 'pore.25': [898], 'comprised': [901], 'chains': [903, 913], '[GaO4(OH)2]∞': [905], 'octahedra': [906], 'linked': [907], 'cis-μ2-OH': [909], 'groups,': [910], 'these': [912, 2398], 'further': [915, 2012], 'bridged': [916], 'tetracarboxylate': [918], 'ligands': [919, 2371], "'wine": [923], "rack'": [924], 'open': [925], 'framework.': [926, 1579], 'Desolvated': [927], 'Brunauer–Emmett–Teller': [931], '(BET)': [932], '1064': [936], 'm2·g−1': [937], 'uptake': [940, 3193], '5.00': [944, 1736], 'mmol·g−1': [945], '298': [947], 'K': [948], '1': [950, 1255, 1671, 2225, 3546], 'bar': [951], '(see': [952, 971, 979, 1067, 1147, 1249, 2145, 2182, 2405, 2428, 2483, 2613, 2657, 2796], 'Supporting': [953, 972, 980, 1044, 1068, 1148, 1250, 1496, 1626, 2146, 2183, 2406, 2429, 2484, 2614, 2658, 2800, 3426, 3428], 'Information': [954, 973, 981, 1045, 1069, 1149, 1251, 1497, 1627, 2147, 2184, 2407, 2430, 2485, 2615, 2659, 2801, 3427, 3429], 'Figure': [955, 974, 982, 1046, 1070, 1150, 1252, 1254, 1498, 1630, 2148, 2185, 2408, 2431, 2616, 2660, 2797, 2860], 'S1).': [956], 'purity': [958, 2396], 'bulk': [961], 'confirmed': [965, 2402, 2513], 'powder': [967], 'X-ray': [968, 1011, 1353, 3037], 'diffraction': [969], '(PXRD)': [970], 'S2)': [975], 'thermogravimetric': [977], 'analysis': [978, 1015, 2427, 2572, 3354], 'S3a).': [983], 'Scanning': [984], 'microscopy': [986, 991], '(SEM)': [987], 'transmission': [989], '(TEM)': [992], 'show': [993], 'crystals': [995], 'cuboid-shaped': [999], 'morphology': [1000], 'average': [1003], 'size': [1004], '15': [1006], 'μm': [1007], '(Figure': [1008, 1041, 1126, 1192, 1517, 2933], '1b).': [1009], 'High-resolution': [1010], 'photoelectron': [1012], '(XPS)': [1014], 'peaks': [1020], 'Ga': [1022, 1093, 1287], '2p1/2,': [1023], '2p3/2,': [1024], '3d3/2,': [1025], '3d5/2': [1027], '1145.5,': [1029], '1118.6,': [1030], '21.2,': [1031], '20.7': [1033], 'eV,': [1034, 1203, 2423, 2695], 'respectively,': [1035, 2424], 'consistent': [1036, 1059, 1153, 2092], 'trivalent': [1039], 'Ga(III)': [1040], '1c,': [1042], 'see': [1043, 1495], 'S4).': [1047], 'Solid-state': [1048, 1162], '13C': [1049], '71Ga': [1051, 1304], 'NMR': [1052, 1080, 1134, 1295, 1310, 1418, 3515], 'reveal': [1054], 'ordered': [1057], 'structure': [1058, 1260, 1324, 2192, 2460], 'single': [1062, 3114], 'repeating': [1063], 'octahedral': [1064, 1328], '[GaO4(OH)2]': [1065, 2462], 'environment': [1066, 1094], 'S5).26': [1071], 'high-field': [1073], '71Ga{1H}': [1074, 1291], '2D': [1075, 1293], 'through-space': [1076], '(dipolar)': [1077], 'heteronuclear': [1078], 'correlation': [1079], 'spectrum': [1081, 1266, 1285, 1296, 2889], 'demonstrates': [1084, 1597, 2123, 2527], 'extensively': [1087], 'correlations': [1090, 1124], 'hydroxyls': [1097], '(at': [1098, 1116], 'δ{1H}': [1099, 1117], '2.8': [1101], 'ppm)': [1102], 'weaker': [1105], 'interaction': [1106, 3200], 'distant': [1110], 'aromatic': [1111, 1139], 'proton': [1112], 'carboxylates': [1115], '9.0': [1119], 'ppm),': [1120], 'other': [1123, 1581, 3387], 'observed': [1125, 2154], '1d).': [1127], 'Moreover,': [1128], 'ratio': [1130], '1H': [1133, 1307, 1417], 'signal': [1135, 2771], 'intensities': [1136], 'protons': [1140, 1144, 3088], 'hydroxy': [1143], '∼3:1': [1146], 'S5c),': [1151], 'entirely': [1152], 'structural': [1156], 'model': [1157], 'Figures': [1160], '1e–1h.': [1161], 'UV–vis': [1163], 'diffuse': [1164], 'reflectance': [1165], '(UV-DRS)': [1167], 'intensive': [1172], 'broad': [1174], 'absorption': [1175], 'band': [1176, 2586, 2591, 2647], 'which': [1181, 1567, 1596, 2090, 2662, 2696, 3126, 3209, 3413], 'assigned': [1183, 2793], 'π→π*': [1186], 'transition': [1187], 'biphenyl': [1190, 2523], 'ligand': [1191, 1561, 2524], '1a).27': [1193], 'Tauc': [1195, 1270], 'plot': [1196, 1271], '3.30': [1202, 2705], 'lower': [1204, 1550, 2476], 'commercial': [1208], 'Ga2O3': [1209, 2157, 2270, 3732, 3875], '(Eg': [1210, 1225, 2164, 2168], '4.56,': [1212], '4.70,': [1213], '4.67': [1215], 'eV': [1216, 2706], 'α-,': [1218], 'β-,': [1219], 'γ-Ga2O3,': [1221], 'respectively)28': [1222], 'ZnGa2O4': [1224, 3786], '4.18': [1227], 'eV).9': [1228], 'photocurrent': [1230], 'response': [1231], 'current': [1237], 'density': [1238], 'increases': [1239], 'upon': [1240, 1244], 'decreases': [1243], 'turning': [1245], 'off': [1246], 'S6).': [1253], '|': [1256, 1632, 1672, 2211, 2862], 'Characterisation': [1257], 'crystal': [1259, 1323], '(a)': [1263, 1638, 2863], 'UV-DRS': [1265, 2426, 2709], '(insert);': [1272, 1281], '(b)': [1273, 1642, 2909], 'SEM': [1274], 'image': [1275, 1280], 'TEM': [1279], '(c)': [1282], 'high-resolution': [1283], 'XPS': [1284, 2575, 3572], '2p,': [1288], '(d)': [1290], 'D-HMQC': [1292], 'MAS': [1294, 1309, 1318], 'corresponding': [1300], '1D': [1301], 'direct': [1302, 1441, 2814, 2845], '(top)': [1305], '(left)': [1308], 'spectra,': [1311, 2749], 'recorded': [1312, 2625], '20.0': [1314], 'T': [1315], 'frequency': [1319], '60': [1321, 1865], 'kHz;': [1322], 'MFM-300(Ga):': [1326], '(e)': [1327], '[GaO4(OH)2];': [1329], '(f)': [1330], 'ligand;': [1331], '(g': [1332], 'h)': [1334], 'views': [1335], '(bridging': [1339], 'groups)': [1341], 'adsorbed': [1343, 3058, 3104, 3160, 3206, 3382], 'studied': [1348, 1386, 2390], 'synchrotron': [1352, 3036], 'single-crystal': [1354], 'diffraction.25': [1355], 'Host–guest': [1356], 'intermolecular': [1360], 'dipole': [1361], 'interactions': [1362, 3154, 3372], 'highlighted': [1364], 'cyan': [1366], 'yellow,': [1368], 'respectively.': [1369], 'toward': [1379, 2445, 3410], 'CO2-saturated': [1388], 'CH3CN-containing': [1389], '(TEOA)': [1391], 'agent': [1395, 2971], 'under': [1396, 2726, 2828, 2904, 3317, 3496], '350–780': [1399, 1659, 2227, 2233, 2239, 2245, 2257, 2265, 2271, 2277, 2283, 2289, 2295, 2313], 'nm': [1400], '1–12': [1402], 'h.': [1403, 1665, 2319], 'were': [1407, 1462, 1510, 2022, 2349, 2360, 2389, 2561, 2577, 2729], 'analysed': [1408], 'gas': [1410], 'chromatography': [1411], 'liquid': [1414, 1455], 'product': [1415, 1429, 1451, 2028, 2152], 'spectroscopy.': [1419], 'measured': [1424], 'moles': [1427], 'obtained': [1430, 2707], 'per': [1431, 1435], 'gram': [1432], 'hour': [1436], '(mol·gcat−1·h−1)': [1437], 'afford': [1439], 'comparison': [1442, 1608], 'reported': [1444, 1530, 1603, 3388], 'catalysts.': [1445], 'Formic': [1446], 'detected': [1452, 2030, 2790, 2850], 'phase,': [1456], 'carbon-containing': [1459, 2027], 'detected.': [1463], 'function': [1469], 'time': [1472, 2746, 2842], 'indicates': [1475, 2188, 2629, 2805, 3010], 'μmol·gcat−1·h−1': [1484, 2086, 3316], 'achieved': [1489], '4': [1491, 1664, 1921, 2243, 2318], 'h': [1492], '(Figures': [1493], '2a,': [1494], 'S7).': [1499], 'crystallinity': [1507], 'retained': [1511], 'three': [1513, 3337], 'cycles': [1514, 3338], '2b).': [1518], 'majority': [1528], '(Table': [1532, 2024], '1)': [1533], 'converting': [1535], 'acid,': [1539, 2089, 2388], 'amino-functionalised': [1542], 'MIL-125(Ti),': [1543], 'UiO-66(Zr),': [1544], 'MIL-101(Fe),23,31,44': [1546], 'two': [1552], 'cases.': [1553], 'One': [1554], 'mixed': [1557, 1560], 'NH2-UiO-66(Zr/Ti)': [1564], '(NH2)2-UiO-66(Zr/Ti),24': [1566], 'prepared': [1569], 'post-synthetic': [1571], 'modifications': [1572], 'introduce': [1574], 'Ti(IV)': [1575], 'recent': [1584, 2094], 'describing': [1586], 'π-conjugated': [1588], 'naphthoporphyrin': [1589], 'system': [1590], 'constructed': [1591, 2385], 'Zr': [1593], 'clusters,': [1595], 'highest': [1599, 2125], 'value': [1600], '(6630': [1601], 'μmol·gcat−1·h−1)': [1602], 'literature.29': [1606], 'studies': [1611, 2576], 'thermal': [1613], 'hydrogenation': [1614], 'catalysts': [1622, 2358], 'given': [1624, 2993], 'Table': [1628, 1670, 2209, 2486, 2802], 'S1.': [1629], '2': [1631, 2210, 2231, 3218, 3224, 3239, 3241, 3245, 3548], 'Different': [1639], 'time;': [1641], 'recycling': [1643], 'tests.': [1644], 'Reaction': [1645, 1688, 2214, 2299], 'conditions:': [1646, 2300], '(10': [1648, 2302], 'mg),': [1649, 2303], 'TEOA/CH3CN': [1650, 2304], '(3': [1651, 2305], 'mL/15': [1652, 2306], 'mL,': [1653, 2307], 'saturated': [1654, 2308], 'CO2),': [1656, 2310], '25': [1657, 2311], '°C,': [1658, 2312], 'nm,': [1660, 2314], 'Comparison': [1673, 2217], 'Efficiency': [1677, 1704], 'Selection': [1682], 'Reported': [1685], 'Literature': [1691], 'MOF-Based': [1692], 'Materials': [1693, 3544], 'Formula': [1695], 'Uptake/mmol·g−1': [1697], '(1': [1698], 'atm)': [1699], 'Sacrificial': [1700], 'Agent': [1701], 'Solvents': [1702], '(μmol·gcat−1·h−1)': [1705], 'References': [1706, 3574], 'TNP-MOF': [1707], 'Zr6(OH)4O4(TNP)3': [1708], '1.69': [1709], '(273': [1710, 1734, 1762, 1765, 1768, 1771, 1774, 1777, 1822, 1858, 1870, 1882, 1891, 1913, 1916, 1927, 1930, 1941, 1944], 'K)': [1711, 1714, 1735, 1738, 1763, 1766, 1769, 1772, 1775, 1778, 1796, 1799, 1809, 1812, 1823, 1826, 1859, 1862, 1871, 1874, 1883, 1892, 1895, 1904, 1914, 1917, 1928, 1931, 1942, 1945], '1.03': [1712], '(298': [1713, 1737, 1795, 1798, 1808, 1811, 1825, 1861, 1873, 1894, 1903], 'TEOA': [1715, 1724, 1739, 1779, 1834, 1841, 1850, 1863, 1875, 1896, 1918, 1932, 1946, 2076, 2101, 2142, 2228, 2234, 2240, 2252, 2266, 2272, 2278, 2284, 2290, 2296, 3325], 'CH3CN': [1716, 1727, 1740, 1780, 1801, 1835, 1842, 1851, 1864, 1876, 1897, 1919, 1933, 1947, 2122], '6630': [1717], '29': [1718], 'NH2-UiO-66-Zr(Ti)': [1719], '(NH2)2-UiO-66-Zr(Ti)': [1720], '–': [1721, 1723, 1747, 1833, 1840, 1849, 1905], 'Zr4.3Ti1.7O4(OH)4(C8H7O4N)5.17(C8H8O4N2)0.83': [1722], 'BNAH': [1726, 1748], '782': [1728], '1052': [1729], '24': [1730], 'Ga2(OH)2(L)': [1732], '6.77': [1733], 'work': [1743], 'Co-MOF,': [1744], 'LIFM-45': [1745], 'Co3(HL0)2·4DMF·4H2O': [1746], 'DMAc': [1749], '456': [1750], '30': [1751], 'NH2-MIL-101(Fe)': [1752], 'MIL-101(Fe)': [1753], 'NH2-MIL-53(Fe)': [1754], 'MIL-53(Fe)': [1755], 'NH2-MIL-88(Fe)': [1756], 'MIL-88(Fe)': [1757], 'Fe3OCl(H2O)3(BDC-NH2)3Fe3OCl(H2O)3(BDC)3FeIII(OH)(BDC-NH2)': [1758], 'FeIII(OH)(BDC)': [1759], 'FeIII3O(CH3OH)3(BDC-NH2)3FeIII3O(CH3OH)3(BDC)3': [1760], '1.52': [1761], '1.18': [1764], '0.89': [1767], '0.60': [1770], '0.64': [1773], '0.46': [1776], '445': [1781], '148': [1782], '116': [1783], '74': [1784], '75': [1785], '23': [1786, 1922], '31': [1787], 'AD-MOF-2': [1788], 'AD-MOF-1': [1789], '[Co2(HAD)2(AD)2': [1790], '(IA)2]·DMF': [1791], '[Co2(HAD)2': [1792], '(AD)2-(BA)]·DMF·2H2O': [1793], '1.86': [1794], '2.33': [1797], 'TIPA': [1800, 1813, 1827, 1884], '443': [1802], '179': [1803], '32': [1804], 'Fe3-Fe2-NH2Fe3-Fe2': [1805], '[{Fe2-Tri}{Fe3(μ3-O)(BDC-NH2)3}]·4NO3[{Fe2-Tri}{Fe3(μ3-O)(BDC)3}]·4NO3': [1806], '1.38': [1807], '1.23': [1810], 'CH3CN/H2O': [1814, 1885], '(1:1)': [1815], '396': [1816], '309': [1817], '33': [1818], 'PCN-138': [1819], '[Zr6(μ3-O)4(μ3-OH)4][TCPP][TBTB]8/3': [1820], '2.82': [1821], '1.82': [1824], 'H2O': [1828, 1906, 3675, 3906], '168': [1829], '34': [1830], 'Ir-CP': [1831], '[Y(Ir(ppy)2(dcbpy)2][OH]': [1832], '158': [1836], '35': [1837], 'Eu-Ru(Phen)3': [1838], '[Eu2(μ2-H2O)(H2O)3(L1)2]·(NO3)2·(2-FBA)2·(H2O)22': [1839], '94': [1843], '36': [1844], 'Cd/Ru-MOF-1': [1845], 'Cd/Ru-MOF-2': [1846], '{Cd3[Ru-L2]2·2(Me2NH2)·solvent}n': [1847], '{Cd[Ru-L3]·3(H2O)}n': [1848], '67': [1852], '72': [1853], '37': [1854], 'PCN-222(Zr)': [1855], 'Zr6(μ3-OH)8(OH)8(TCPP)2': [1856], '2.59': [1857], '1.56': [1860], '38': [1866], 'NNU-28(Zr)': [1867], '[Zr6O4(OH)4(L4)6]·6DMF': [1868], '2.83': [1869], '1.49': [1872], '53': [1877], '39': [1878], 'PCN-136': [1879], 'Zr6(μ3-O)4(μ3-OH)4(OH)6(H2O)6(HCHC)': [1880], '2.72': [1881], '44': [1886, 1950], '40': [1887], 'Zr-SDCA-NH2': [1888], '[Zr6O4(OH)4(L5)6]·8DMF': [1889], '3.74': [1890], '1.57': [1893], '41': [1898, 1899], 'NNU-31-Zn': [1900], 'Fe2Zn(μ3-O)(TCA)2(H2O)3': [1901], '1.65': [1902], '26': [1907, 1948], '42': [1908], 'NH2-MIL-125(Ti)': [1909], 'MIL-125(Ti)': [1910], 'Ti8O8(OH)4(BDC-NH2)6Ti8O8(OH)4(BDC)6': [1911], '5.90': [1912], '4.40': [1915], '16': [1920], 'NH2-UiO-66-(Zr/Ti)': [1923], 'NH2-UiO-66(Zr)': [1924, 1937], '(Zr/Ti)6O4(OH)4(BDC-NH2)6Zr6O4(OH)4(BDC-NH2)6': [1925], '3.79': [1926], '3.04': [1929, 1940], '12': [1934, 2293], '7': [1935, 2261], '43': [1936], 'UiO-66(Zr)': [1938], 'Zr6O4(OH)4(BDC-NH2)6Zr6O4(OH)4(BDC)6': [1939], '2.37': [1943], '0': [1949, 3228, 3251], 'Notes:': [1951], 'TEOA,': [1952], 'triethanolamine;': [1953], 'BNAH,': [1954], '1-benzyl-1,4-dihydronicotinamide;': [1955], 'H4L,': [1956], 'acid;': [1958, 1961, 1966, 1969, 1988, 2001, 2007], 'H2BDC,': [1959], 'benzene-1,4-dicarboxylic': [1960], 'HAD,': [1962], 'adenine;': [1963], 'BA,': [1964], 'butanedioic': [1965], 'IA,': [1967], 'isobutyric': [1968], 'DMF,': [1970], 'N,N-dimethylformamide;': [1971], 'Tri,': [1972], '1,2,4-triazole;': [1973], 'DMAc,': [1974], 'N,N-dimethylacetamide;': [1975], 'TIPA,': [1976], 'triisopropanolamine;': [1977], 'H2TCPP,': [1978], 'tetrakis(4-carboxyphenyl)porphyrin;': [1979], 'TBTB,': [1980], '4,4ʹ,4″-(2,4,6-trimethylbenzene-1,3,5-triyl)tribenzoate;': [1981], 'ppy,': [1982], '2-phenylpyridine;': [1983], 'dcbpy,': [1984], '2,2ʹ-bipyridine-4,4ʹ-dicarboxylate;': [1985], 'H4L0,': [1986], '2ʹ-amino-[1,1ʹ:4ʹ,1″-terphenyl]-3,3″,5,5″-tetracarboxylic': [1987], 'H3L1,': [1989], 'Ru(phen)3-derived': [1990], 'tricarboxylate': [1991], 'metalloligand;': [1993], '2-FBA,': [1994], '2-fluorobenzoate;': [1995], 'L2=5,5ʹ-dcbpy=2,2ʹ-bipyridine-5,5ʹ-dicarboxylate;': [1996], 'L3=(4,4ʹ-dcbpy)2(bpy),': [1997], 'bpy=2,2ʹ-bipyridine;': [1998], 'H2L4,': [1999], '4,4ʹ-(anthracene-9,10-diylbis(e-thyne-2,1-diyl))dibenzoic': [2000], 'HCHC,': [2002], 'hexakis(4-carboxyphenyl)hexabenzocoronene;': [2003], 'H2L5,': [2004], '2,2ʹ-diamino-4,4ʹ-stilbene': [2005], 'dicarboxylic': [2006], 'TCA,': [2008], '4,4ʹ,4″-tricarboxytriphenylamine.': [2009], 'To': [2010, 2366, 2711], 'gain': [2011], 'insights': [2013, 3138], 'reaction,': [2016], 'series': [2018], 'control': [2020], 'experiments': [2021, 2560, 2725], 'conducted': [2023, 2562, 2578, 2827], '2).': [2025], 'No': [2026, 2820, 3508], 'from': [2031, 2386, 2609, 2708, 3047, 3491], 'reactions': [2032, 2871, 3340], 'absence': [2035], '(1)': [2037, 3237], '(2)': [2039, 3260], '(where': [2041], 'N2': [2042, 2241], 'used': [2044, 2350, 2359, 2753, 3517], 'instead),': [2045], '(3)': [2047], 'light.': [2048], 'These': [2049, 2546], 'results': [2050], 'confirm': [2051], 'source': [2055], 'proceeds': [2065], 'routes': [2068], 'catalyst.': [2073, 2859], 'Replacement': [2074], 'triethylamine': [2078], '(TEA)45': [2079], 'gives': [2080], 'low': [2082], '64': [2085, 2260], 'reports': [2095], 'on': [2096, 2377, 3155, 3416], 'role': [2099, 3404], 'assisting': [2105], 'CH3CN.46,47': [2111], 'range': [2113], 'different': [2115, 2627], 'organic': [2116], 'solvents': [2117], 'tested,': [2120], 'optimal': [2130], 'enhanced': [2137, 2537], 'CH3CN47': [2144], 'S8).': [2149], 'Interestingly,': [2150, 3070], 'when': [2155], '(∼50': [2158], 'mesh,': [2159], 'Eg': [2160], '4.57),': [2162], 'GaN': [2163, 2276], '3.04),': [2166], 'GaP': [2167, 2282], '1.92),': [2170], 'powdered': [2173, 2335], 'mixture': [2174, 2336], 'Ga(NO3)3': [2176], 'H4L': [2178, 2264, 2344], 'photocatalyst': [2181], 'S9).': [2186], 'crucial': [2196], 'separation': [2203], 'electrons.': [2208], 'Summary': [2212], 'Conditions': [2215], 'Experiments': [2218], 'Entry': [2219], 'Catalyst': [2220], 'Light': [2221], '(nm)': [2222], 'Gas': [2223], 'HCOOH': [2224, 3249], 'n.a.': [2232, 2236, 2242, 2246, 2248, 2251, 2254, 2268, 2274, 2280, 2286, 2292, 2298], '3': [2237, 2323, 2861], '5': [2249], '6': [2255], 'TEA': [2258, 2325], 'Ga(NO3)3·9H2O': [2262, 2338], '8': [2269], '9': [2275], '10': [2281, 2361], '11': [2287], 'MIL-53(Ga)': [2288, 2381, 2413, 2469, 2543], 'MIL-68(Ga)': [2294, 2415, 2471], 'entry': [2321, 2332, 2355], '6,': [2322, 3682], 'mL': [2324], 'added': [2327], 'replace': [2329], 'TEOA;': [2330], '7,': [2333], '(0.04': [2339], 'mmol,': [2340, 2346], '16.7': [2341], 'mg)': [2342, 2348], '(0.02': [2345], '6.6': [2347], '(H4L,': [2351], 'biphenyl-3,3,5ʹ,5ʹ-tetracarboxylic': [2352], 'acid);': [2353], '8–12,': [2356], 'mg': [2362], 'each': [2364], 'investigate': [2367], 'effects': [2369], 'Ga-MOFs': [2376, 3389], 'property,': [2380], 'MIL-68(Ga),': [2383], 'both': [2384], 'terephthalic': [2387], 'reaction.48–50': [2393], 'phase': [2395], 'PXRD': [2404], 'S10).': [2409], 'bandgaps': [2411], 'determined': [2417, 2599, 2651, 3032, 3182], 'be': [2419, 2601, 2681], '3.21': [2420], '3.93': [2422], 'S11).': [2432], 'same': [2435], 'conditions': [2437, 2728, 2906], 'above,': [2439], 'neither': [2440], 'Although': [2450], 'similar': [2452], 'BET': [2453], 'areas': [2455], '(1117–1140': [2456], 'm2·g−1)': [2457], 'comprising': [2461], 'moieties,': [2463], 'capacity': [2467], '(1.46–1.65': [2472], 'mmol·g−1)': [2473, 2480], '(5.00': [2479], 'S2).': [2487], 'likely': [2490], 'rigid': [2494], 'presence': [2497, 3393], 'μ2-OH': [2500, 3021, 3376], 'crystallographic': [2517], 'spectroscopic': [2519, 3353], 'analyses.25': [2520], 'Furthermore,': [2521], 'increased': [2528], 'π-electron': [2529], 'delocalisation': [2530], 'hence': [2536], 'LMCT': [2538, 3400], 'compared': [2539], 'terephthalate': [2541], 'MIL-68(Ga).': [2545], 'collectively': [2547], 'result': [2548, 2612], 'drastic': [2551], 'difference': [2552], 'activity.': [2556, 3425], 'Photophysical': [2557], 'electrochemical': [2559], 'understand': [2564], 'redox': [2566, 2997, 3092, 3229, 3252], 'properties': [2567], 'Mott-Schottky': [2570], '(MS)': [2571], 'valence-band': [2574], 'determine': [2580], 'positions': [2582], 'conduction': [2585], '(ECB)': [2587], 'valence': [2590], '(EVB)': [2592], 'respectively.32,51': [2595], 'EVB': [2597], '2.2': [2602], 'V': [2603, 2654, 2666, 2683, 2983, 3001, 3096, 3233, 3256], 'versus': [2604, 2655, 2684, 2984, 3002, 3097], 'normalised': [2605], 'electrode': [2607], '(NHE)': [2608], 'VB-XPS': [2611], 'S12a).': [2617], 'positive': [2619, 2668, 3149], 'slope': [2620], 'all': [2622], 'MS': [2623], 'plots': [2624], 'frequencies': [2628], 'typical': [2634], 'n-type': [2635, 2673], 'semiconductor,': [2636], 'intercept': [2639], 'independent': [2641], 'frequency.': [2644], 'flat': [2646], '(EFB)': [2649], '−0.99': [2653], 'NHE': [2656, 2985, 3003, 3098, 3236, 3259], 'S12b),': [2661], 'usually': [2664], '∼0.1': [2665], 'ECB': [2671, 2677], 'materials.52': [2674], 'Thus,': [2675, 3175], 'estimated': [2679], '−1.09': [2682, 2982], 'NHE.': [2685], 'gap': [2687], 'VB': [2689, 2946, 2962], 'CB': [2691, 2953], '3.29': [2694], 'agreement': [2700, 3507], 'analysis.': [2710], 'identify': [2712], 'species': [2715], 'involved': [2716], 'process,': [2720], 'spin-trapping': [2723], 'EPR': [2724, 2748, 2867, 3352, 3478], 'conducted.': [2730], 'Since': [2731], 'free': [2735], 'radicals': [2736, 2763], 'several': [2738], 'orders': [2739], 'magnitude': [2741], 'shorter': [2742], 'acquisition': [2745], '5,5-dimethyl-1-pyrroline-n-oxide': [2750], '(DMPO)': [2751], 'spin': [2756, 2877], 'trap': [2757], 'enable': [2759], 'identification': [2761], 'long-lived': [2765], 'DMPO-radical': [2766], 'adducts.53': [2767], 'intense': [2769], 'six-line': [2770], 'g': [2773], '2.005': [2775], 'hyperfine': [2777], 'coupling': [2778], 'constants': [2779], 'AN': [2780], '15.2': [2782], 'G': [2783, 2788], 'AH': [2785], '18.9': [2787], 'unambiguously': [2792], 'DMPO-CO2•−54,55': [2795], '3a': [2798], 'S3).': [2803], 'acid.': [2819, 3349], 'captured': [2823], 'dark': [2829], 'conditions.': [2830], 'Significantly,': [2831], 'best': [2834], 'our': [2836], 'knowledge,': [2837], 'X-band': [2866], 'spectra': [2868], 'DMPO': [2875], 'trap,': [2878], '(black)': [2879], 'before': [2880], '(red)': [2882], 'after': [2883], 'irradiation,': [2885, 2937], 'simulated': [2887], '(blue)': [2888], 'major': [2892], 'component,': [2893, 2900], 'DMPO-CO2•−': [2894], '(green,': [2895], 'simulation),': [2896], 'minor': [2899], 'DMPO-Ox': [2901], '(cyan,': [2902], 'simulation)': [2903], 'proposed': [2911, 2932], 'mechanism': [2912, 3141], 'cycle': [2927], '3b).': [2934], 'Upon': [2935], 'activated,': [2940], '(2.2': [2947], 'V)': [2948], 'promoted': [2950, 3367], '(−1.09': [2954], 'V),': [2955], 'holes': [2959], 'readily': [2964], 'filled': [2965], 'TEOA.': [2972], 'Surprisingly,': [2973], 'reductive': [2979], 'reduce': [2987], 'anions,': [2992], 'strongly': [2995], 'negative': [2996], '−1.90': [3000], '[Eq.': [3004, 3099], '(1)]': [3005], 'process.56': [3008], 'through': [3025, 3539], 'diffraction25': [3038], 'not': [3039], 'bound': [3051], 'activates': [3056], 'molecules.': [3060, 3384], 'shifts': [3062], 'anodic': [3068], 'potential.': [3069], 'path': [3072], 'regarded': [3083], 'accepting': [3085], 'simultaneously': [3089], '−0.61': [3095], '(2)].56': [3100], 'By': [3101], 'molecule': [3106], 'able': [3110], 'accept': [3112], 'bonding': [3119], 'generate': [3121], 'anion,': [3125], 'unprecedented': [3128], 'MOF-driven': [3131], 'affords': [3136], 'new': [3137, 3215], 'Recently,': [3147], 'impact': [3150], 'host-guest': [3153], 'demonstrated': [3165], 'small': [3170], 'catalysts.57,58': [3174], 'synergistic': [3185], 'effect': [3186], 'bandgap,': [3188], 'rate': [3189], 'transfer,': [3192], 'most': [3197], 'scaffold': [3204], 'molecules,': [3208], 'will': [3210], 'inform': [3211], 'design': [3213, 3265, 3418], 'photocatalysts.': [3216, 3283], '+': [3219, 3240, 3243, 3244, 3248], 'e': [3220, 3246], '−': [3221, 3226, 3231, 3247, 3254], '→': [3222], '•': [3225], 'E': [3227, 3250], '1.90': [3232], 'vs': [3234, 3257], '.': [3235, 3258], 'H': [3242], '0.61': [3255], 'Conclusion': [3261], 'porosity': [3263], 'flexibility': [3266], 'MOFs,': [3268], 'coupled': [3269], 'photoelectrical': [3275], 'properties,': [3276], 'make': [3277], 'them': [3278], 'promising': [3279], 'candidates': [3280], 'We': [3284, 3613], 'Ga-MOF-based': [3291], 'temperature': [3323], 'stability': [3335], 'full': [3342], 'retention': [3343], 'Compared': [3385], 'literature,': [3391], 'plays': [3401], 'reduction,': [3412], 'sheds': [3414], 'future': [3420], 'improved': [3424], 'available': [3431], 'includes': [3433], 'detailed': [3434], 'experimental': [3435], 'procedures': [3436], 'characterization': [3438], 'data.': [3439], 'Conflict': [3440], 'Interest': [3442], 'There': [3443], 'conflict': [3446], 'interest': [3448], 'report.': [3450], 'Acknowledgments': [3451], 'research': [3453, 3502, 3520], 'supported': [3455, 3549], 'EPSRC': [3457, 3471, 3476, 3524], '(EP/I011870,': [3458], 'EP/V056409),': [3459], 'Royal': [3461], 'Society': [3462], 'funding,': [3469], 'funding': [3473, 3490, 3538], 'National': [3477], 'Facility': [3479, 3516], 'Manchester.': [3484], 'project': [3486], 'received': [3489], 'European': [3493, 3498, 3556], 'Research': [3494], 'Council': [3495], "Union's": [3499], 'Horizon': [3500], '2020': [3501], 'innovation': [3504], 'programme': [3505], '(grant': [3506], '742401,': [3509], 'NANOCHEM).': [3510], 'UK': [3512], 'High-Field': [3513], 'Solid-State': [3514], 'funded': [3522], 'BBSRC': [3526], '(EP/T015063/1)': [3527], 'well': [3529], 'Warwick': [3534], 'including': [3535], 'partial': [3537], 'Birmingham': [3540], 'City': [3542], 'Advanced': [3543], 'Projects': [3545], 'Advantage': [3551], 'West': [3552], 'Midlands': [3553], 'Regional': [3557], 'Development': [3558], 'Fund.': [3559], 'authors': [3561], 'wish': [3562], 'acknowledge': [3564], 'Dr.': [3565], 'Marek': [3566], 'Nikiel': [3567], 'help': [3570], 'measurement.': [3573], '1.': [3575], 'Ran': [3576], 'J.;': [3577, 3758, 3769, 3808, 3822], 'Jaroniec': [3578, 3809], 'M.;': [3579, 3692, 3718, 3726, 3760, 3804], 'Qiao': [3580], 'S.': [3581, 3752, 3755], 'Z.Cocatalysts': [3582], 'Semiconductor-Based': [3584], 'Reduction:': [3587], 'Achievements,': [3588], 'Challenges,': [3589], 'Opportunities.Adv.': [3591], 'Mater.2018,': [3592], '30,': [3593], '1704649.': [3594], 'Google': [3595, 3620, 3644, 3684, 3714, 3748, 3800, 3816, 3852, 3889], 'Scholar': [3596, 3621, 3645, 3685, 3715, 3749, 3801, 3817, 3853, 3890], '2.': [3597], 'Zhang': [3598], 'W.;': [3599, 3658], 'Mohamed': [3600], 'A.': [3601, 3694], 'R.;': [3602, 3648, 3722], 'Ong': [3603], 'W.': [3604], 'J.Z-Scheme': [3605], 'Systems': [3607], 'Carbon': [3609], 'Dioxide': [3610], 'Reduction:Where': [3611], 'Are': [3612], 'Now?Angew.': [3614], 'Chem.': [3615, 3710, 3795], 'Int.': [3616, 3796], 'Ed.2020,': [3617], '59,': [3618], '22894–22915.': [3619], '3.': [3622], 'Dhakshinamoorthy': [3623], 'A.;': [3624, 3628, 3724], 'Navalon': [3625], 'S.;': [3626, 3656, 3772, 3806, 3820, 3866, 3893], 'Corma': [3627], 'Garcia': [3629], 'H.Photocatalytic': [3630], 'TiO2': [3634], 'Related': [3636], 'Titanium': [3637], 'Containing': [3638], 'Solids.Energy': [3639], 'Environ.': [3640], 'Sci.2012,': [3641], '5,': [3642], '9217–9233.': [3643], '4.': [3646], 'Li': [3647, 3659, 3770, 3829, 3898], 'Cheng': [3649], 'W.-H.;': [3650], 'Richter': [3651], 'M.': [3652], 'H.;': [3653, 3775, 3824, 3828, 3856, 3864, 3895], 'DuChene': [3654], 'C.;': [3660, 3753], 'Atwater': [3661], 'H.': [3662], 'A.Unassisted': [3663], 'Highly': [3664, 3734], 'Selective': [3665], 'Gas-Phase': [3666], 'Plasmonic': [3671], 'Au/p-GaN': [3672], 'Photocatalyst': [3673, 3733, 3840], 'Using': [3674, 3702], 'Electron': [3678], 'Donor.ACS': [3679], 'Energy': [3680], 'Lett.2021,': [3681], '1849–1856.': [3683], '5.': [3686], 'Barton': [3687], 'E.': [3688], 'E.;': [3689], 'Rampulla': [3690], 'D.': [3691], 'Bocarsly': [3693], 'B.Selective': [3695], 'Solar-Driven': [3696], 'Methanol': [3701], 'p-GaP': [3705], 'Based': [3706], 'Photoelectrochemical': [3707], 'Cell.J.': [3708], 'Am.': [3709], 'Soc.2008,': [3711], '130,': [3712], '6342–6344.': [3713], '6.': [3716], 'Akatsuka': [3717], 'Kawaguchi': [3719], 'Y.;': [3720, 3763, 3777, 3832], 'Itoh': [3721], 'Ozawa': [3723], 'Yamamoto': [3725], 'Tanabe': [3727], 'T.;': [3728], 'Yoshida': [3729], 'T.Preparation': [3730], 'Active': [3735], 'Water': [3740], 'Without': [3741], 'Cocatalyst.Appl.': [3742], 'Catal.': [3743], 'B': [3744], 'Environ.2020,': [3745], '262,': [3746], '118247.': [3747], '7.': [3750], 'Yan': [3751, 3819, 3892], 'Ouyang': [3754], 'X.;': [3756, 3766], 'Gao': [3757, 3823], 'Feng': [3761], 'Fan': [3764], 'X.': [3765], 'Wan': [3767], 'Z.': [3771, 3779], 'Ye': [3773], 'Zhou': [3776, 3831], 'Zou': [3778, 3833, 3900], 'G.A': [3780], 'Room-Temperature': [3781], 'Reactive-Template': [3782], 'Route': [3783], 'Mesoporous': [3785], 'Improved': [3788], 'Activity': [3790], 'CO2.Angew.': [3794], 'Ed.2010,': [3797], '122,': [3798], '6544–6548.': [3799], '8.': [3802], 'Marszewski': [3803], 'Cao': [3805], 'Yu': [3807, 3827, 3894], 'M.Semiconductor-Based': [3810], 'Conversion.Mater.Horizons2015,': [3813], '2,': [3814], '261–278.': [3815], '9.': [3818], 'N.;': [3826, 3897], 'Z.;': [3830, 3860, 3862, 3899], 'Z.Zinc': [3834], 'Gallogermanate': [3835], 'Solid': [3836], 'Solution:': [3837], 'Novel': [3839], 'Efficiently': [3842], 'Converting': [3843], 'Solar': [3846], 'Fuels.Adv.': [3847], 'Funct.': [3848], 'Mater.2013,': [3849], '23,': [3850], '1839–1845.': [3851], '10.': [3854], 'Tatsumi': [3855], 'Teramura': [3857], 'K.;': [3858], 'Huang': [3859], 'Asakura': [3863], 'Hosokawa': [3865], 'Tanaka': [3867], 'T.Enhancement': [3868], 'Evolution': [3871], 'Modification': [3873], 'Rare-Earth': [3877], 'Elements': [3878], 'Conversion': [3882, 3902], 'H2O.Langmuir2017,': [3886], '33,': [3887], '13929–13935.': [3888], '11.': [3891], 'Z.Efficient': [3901], 'Hydrocarbon': [3908], 'Fuel': [3909], 'ZnAl2O4-Mod': [3911]}, 'cited_by_api_url': 'https://api.openalex.org/works?filter=cites:W4281667127', 'counts_by_year': [{'year': 2024, 'cited_by_count': 8}, {'year': 2023, 'cited_by_count': 5}, {'year': 2022, 'cited_by_count': 3}], 'updated_date': '2024-12-12T23:53:56.691262', 'created_date': '2022-06-13'}