Complex Featuring Two Double Dative Bonds Between Carbon(0) and Uranium

Name: Work Video:
Duration: 3 min 30 s
Wei Fang; Sudip Pan; Wei Su; Shuao Wang; Lili Zhao; Gernot Frenking; Congqing Zhu
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3061, 3099, 3129, 4543], 'uranyl': [283, 408, 437, 544, 578, 771, 1181], 'with': [284, 304, 329, 374, 388, 499, 536, 546, 626, 658, 728, 762, 772, 802, 815, 826, 879, 1053, 1182, 1238, 1402, 1458, 1488, 1583, 1626, 1639, 1673, 1682, 1805, 2200, 2216, 2640, 2665, 2891, 3068, 3690, 3763, 3898, 4199, 4209, 4504, 4584, 4924, 4928], 'two': [285, 305, 431, 489, 580, 659, 674, 729, 735, 763, 785, 1030, 1234, 1529, 1561, 1621, 1634, 2517, 2958, 2980], 'U=O': [286, 433], 'double': [287, 307, 366, 389, 483, 508, 582, 612, 764, 818, 1062, 1235, 1289, 1689, 2793, 2960, 2981, 3011, 3050, 3838, 5032], 'bonds': [288, 308, 341, 391, 397, 435, 509, 613, 661, 1237, 1625, 1638, 1665, 2388, 2831, 2851, 2860, 2962, 2983, 3013, 3063, 3072], 'is': [289, 413, 647, 655, 726, 779, 897, 1047, 1051, 1071, 1091, 1123, 1152, 1156, 1194, 1204, 1226, 1270, 1274, 1330, 1337, 1364, 1466, 1581, 1598, 1766, 1772, 1849, 1861, 2072, 2264, 2268, 2398, 2418, 2502, 2575, 2713, 2717, 2812, 2824, 2847, 2867, 2975, 3023, 3053, 3110], 'a': [290, 410, 473, 511, 518, 532, 542, 547, 560, 627, 648, 656, 686, 724, 773, 789, 816, 848, 1037, 1231, 1239, 1250, 1319, 1455, 1720, 2484, 2792, 2825, 2840, 2990, 2997, 3054, 3078, 3399, 3406, 3518, 3661, 3808, 3817, 3982, 4047, 4079, 4168, 4205, 4263, 4332, 4452, 4737, 4841, 5001], 'well-known': [291], 'predominant': [293], 'form': [294], 'uranium': [296, 321, 359, 421, 460, 467, 533, 561, 595, 759, 791, 803, 1039, 1133, 1296, 1698, 2193, 2299, 3018, 3043], 'in': [297, 331, 363, 420, 436, 471, 521, 556, 597, 614, 631, 706, 722, 733, 840, 844, 862, 889, 902, 993, 1045, 1057, 1066, 1080, 1089, 1098, 1112, 1121, 1135, 1147, 1161, 1174, 1190, 1212, 1218, 1298, 1351, 1406, 1472, 1501, 1542, 1600, 1618, 1656, 1750, 1803, 1832, 1855, 2002, 2022, 2034, 2038, 2056, 2228, 2274, 2307, 2406, 2446, 2474, 2492, 2622, 2626, 2677, 2723, 2742, 2861, 2886, 2898, 2972, 2989, 3001, 3164, 3594, 3640, 3706, 3739, 3770, 3941, 3974, 4161, 4685, 4710, 4953, 4977, 5061], 'the': [298, 301, 316, 325, 332, 339, 352, 364, 371, 381, 416, 441, 451, 457, 465, 529, 588, 594, 598, 604, 610, 615, 624, 632, 637, 640, 664, 697, 731, 743, 755, 770, 782, 808, 845, 872, 910, 945, 998, 1054, 1061, 1075, 1085, 1094, 1109, 1127, 1132, 1141, 1172, 1180, 1187, 1207, 1227, 1261, 1277, 1295, 1341, 1347, 1352, 1375, 1383, 1403, 1434, 1443, 1446, 1459, 1475, 1489, 1508, 1516, 1519, 1543, 1547, 1560, 1572, 1584, 1594, 1606, 1614, 1650, 1670, 1683, 1694, 1697, 1727, 1745, 1755, 1761, 1782, 1814, 1847, 1858, 1866, 1875, 1987, 2003, 2007, 2023, 2027, 2041, 2045, 2059, 2063, 2082, 2092, 2095, 2100, 2112, 2131, 2142, 2158, 2172, 2177, 2180, 2185, 2201, 2209, 2219, 2226, 2229, 2233, 2237, 2245, 2252, 2255, 2261, 2289, 2292, 2298, 2328, 2331, 2338, 2342, 2353, 2357, 2369, 2403, 2407, 2415, 2422, 2439, 2451, 2462, 2475, 2479, 2488, 2493, 2496, 2510, 2516, 2521, 2524, 2533, 2539, 2578, 2583, 2592, 2610, 2619, 2623, 2648, 2658, 2668, 2675, 2678, 2682, 2686, 2694, 2701, 2704, 2710, 2732, 2749, 2758, 2783, 2802, 2815, 2829, 2858, 2863, 2871, 2879, 2887, 2892, 2899, 2914, 2920, 2938, 2947, 2976, 2986, 3008, 3017, 3021, 3031, 3040, 3049, 3083, 3141, 3155, 3177, 3181, 3192, 3218, 3237, 3443, 3475, 3613, 3616, 3665, 3695, 3730, 3760, 3821, 3831, 4129, 4153, 4157, 4915, 4995, 5004, 5038, 5052, 5074, 5078, 5089], 'environment,': [299], 'but': [300, 495, 2523], 'carbon-based': [302], 'analog': [303, 545, 576, 768], 'U=C': [306, 365, 500, 581, 611, 629, 817, 1042, 1064, 1086, 1096, 1118, 3343, 3901], 'has': [309, 424, 1454, 2963], 'rarely': [310], 'been': [311, 493, 553, 679, 953, 2964], 'synthesized.': [312], 'Here,': [313, 752], 'we': [314, 753, 1513, 2730], 'describe': [315], 'formation': [317, 809, 846], 'an': [319, 375, 478, 767, 1287, 1640, 2376, 2399, 2614, 3637, 4231, 4422], 'unprecedented': [320], 'complex': [322, 761, 778, 852, 895, 921, 933, 1407, 1417, 1751, 2235, 2494, 2625, 2684, 2955], '[(PyPh2P)2C]2UCl2]2+·2(BPh4−)': [323, 853], 'from': [324, 935, 1197, 2081, 2091, 2111, 2327, 2547, 2797, 3014, 3098, 3201, 4012, 5098], 'reaction': [326, 797, 823, 873], 'UCl4': [328, 883], 'carbodiphosphorane': [330, 701], 'presence': [333, 429], 'NaBPh4.': [335], 'nature': [337, 1447, 1780, 2873], 'U–C': [340, 1076, 2362, 2378, 2651, 2784, 2876, 2888], 'was': [342, 469, 526, 571, 585, 703, 711, 856, 1010, 1305, 2457, 3138, 5035], 'revealed': [343, 2576], 'by': [344, 486, 528, 587, 603, 621, 714, 781, 871, 1012, 1307, 1797, 2384, 2577, 2736, 2771, 2809, 3140, 3591, 3733, 4358, 5037], 'density': [345, 1587, 1597, 2755, 2838], 'functional': [346, 1424], 'theory': [347, 1425, 2739], 'calculations,': [348], 'which': [349, 550, 684, 723, 734, 1033, 1050, 1155, 1214, 1273, 1336, 1465, 1680, 2086, 2167, 2198, 2213, 2351, 2364, 2564, 2645, 2662], 'show': [350, 2946], 'that': [351, 380, 1160, 1528, 1701, 1846, 2184, 2414, 2461, 2538, 2787, 3048, 3282], '5f': [353, 1704, 2188, 4154], '6d': [355, 1702, 2186], 'orbital': [356, 1535, 1553, 1609, 1807, 1839, 2065, 2084, 2108, 2149, 2323, 2499, 2527, 2535, 2894], 'electrons': [357, 672, 1531], 'are': [360, 462, 719, 740, 746, 1034, 1400, 1499, 1539, 1557, 1654, 1666, 1830, 2032, 2040, 2058, 2154, 2214, 2273, 2281, 2305, 2365, 2389, 2519, 2529, 2603, 2663, 2722, 2764], 'remarkably': [361], 'involved': [362], 'bonds.': [367, 401, 2762, 2877, 3076], 'inspection': [369], 'bonding': [372, 446, 641, 710, 1222, 2404, 2490, 2557, 2620, 2633, 2734, 3041, 3056], 'characteristics': [373], 'energy': [376, 989, 1473, 1799, 2837], 'decomposition': [377, 1800], 'analysis': [378, 1015, 1611, 1801, 1829, 2335, 2995], 'suggests': [379], 'uranium-ligand': [382, 444], 'bond': [383, 484, 630, 819, 960, 1043, 1065, 1078, 1087, 1119, 1143, 1291, 1608, 1926, 1940, 2785, 2804, 2889, 3000, 3052], 'may': [384, 3064], 'be': [385, 619, 869, 925, 1216, 1372, 1795, 2079, 2089, 2382, 2789, 3066, 3093], 'alternatively': [386], 'described': [387, 2790, 3067], 'dative': [390, 660, 765, 1063, 1221, 1236, 1290, 2385, 2643, 2961, 2982, 3012, 3051], '[C⇉U⇇C]': [392, 774, 1240, 2970], 'or': [393, 488, 937, 1170], 'strong': [394, 2629, 3069], 'electron-sharing': [395, 1924, 1938, 2377, 2394, 2555, 3070], 'π': [396, 1565, 1616, 1624, 1664, 1709, 1784, 1925, 1939, 1946, 1959, 2165, 2556, 2632, 3071], 'weak': [399, 2641, 3074], 'σ': [400, 1574, 1637, 1662, 1707, 1788, 1918, 1932, 1952, 1965, 1971, 1976, 2123, 2285, 2315, 2600, 2642, 3075], 'Download': [402, 404, 1001, 1003, 1419, 1421, 1775, 1777, 2276, 2278, 2725, 2727, 2949, 2951], 'figure': [403, 1002, 1420, 1776, 2277, 2726, 2950], 'PowerPoint': [405, 1004, 1422, 1778, 2279, 2728, 2952], 'Introduction': [406, 3156, 5053], '(with': [409, 510], '[O=U=O]': [411, 1185], 'core)': [412, 513], 'one': [414, 487, 1997, 2017, 2469], 'most': [417, 698, 2075, 2221, 2670], 'common': [418, 903, 1365, 2826], 'species': [419, 476, 540, 721, 811, 1232, 1369, 2344, 2442], 'chemistry': [422, 458], 'attracted': [425], 'remarkable': [426], 'attention.1,2': [427], 'translinear': [432], 'multiple': [434, 445, 569, 1142], 'continues': [438], 'stimulate': [440], 'development': [442], 'chemistry.': [447], 'In': [448], 'contrast': [449], 'well-developed': [452], 'transition-metal': [453], 'carbenes,': [454], 'reports': [455], 'concerning': [456], 'carbenes': [461, 596], 'few.3,4': [463], 'Since': [464], 'first': [466, 704, 756, 1228, 1514, 2977], 'carbene': [468, 534, 562], 'reported': [470, 705, 1367], '1981,5': [472], 'handful': [474], 'containing': [477, 1233], 'An=C': [479], '(An': [480], '=': [481, 504, 524, 3703, 3826, 3891], 'actinide)': [482], 'stabilized': [485, 586], 'phosphorus': [490], 'substituents': [491], 'have': [492, 678, 685, 952], 'reported,6–13': [494], 'only': [496, 555], 'few': [497], 'examples': [498, 732], 'U=E': [502], '(E': [503], 'O,': [505], 'N,': [506], 'C)': [507], '[C=U=E]': [512, 599, 616, 633], 'were': [514, 601, 1428], 'realized.14–19': [515], 'For': [516, 2857], 'example,': [517], 'trans-C=U=O': [519], 'linkage': [520, 617], '[(BIPM)UOCl2]': [522], '(BIPM': [523], 'C(PPh2NSiMe3)2)': [525], 'synthesized': [527], 'oxidation': [530], '[(BIPM)UCl3Li(THF)2]': [535], '4-methylmorpholine': [537], 'N-oxide.20': [538], 'This': [539, 776, 2574, 2823, 3033, 3136], 'represents': [541], 'rare': [543], '[C=U=O]': [548], 'unit,': [549], 'previously': [551], 'had': [552], 'observed': [554, 1279], 'matrix': [557], 'experiments.': [558], 'Remarkably,': [559, 1605], 'imido': [563], 'oxo': [564], 'complex,': [565], 'featuring': [566, 579, 2957], 'three': [567], 'different': [568, 628, 688], 'bonds,': [570, 583, 766, 2363], 'also': [572, 868, 1612, 1773, 2482, 2646, 3024, 3065], 'synthesized.11': [573], 'carbon': [575, 666, 1293, 1671, 1686, 2132, 2339], '[C=U=C],': [584], 'pincer-type': [589], 'methanediide': [590, 607], 'ligands.21–23': [591], 'Without': [592], 'exception,': [593], 'core': [600, 634, 2971], 'constructed': [602, 620], 'chelating': [605], 'tridentate': [606], 'ligands.': [608, 2358, 2424], 'If': [609], 'could': [618, 923], 'other': [622, 2008, 2028, 2480], 'precursors,': [623], 'combination': [625, 1804, 2113], 'should': [635], 'enhance': [636], 'understanding': [638, 3038], 'uranium.24–29': [643], 'A': [644, 1300, 1356, 1691, 1879, 3893, 4238, 4454, 4667, 4688], 'possible': [645], 'candidate': [646], 'carbone': [649, 653, 725, 739, 760, 786, 2354], 'CL2': [650, 654], 'ligand.': [651], 'carbon(0)': [657, 3045], 'L→C←L': [662], 'where': [663, 1685, 1813, 2128, 2288, 2450, 3020], 'central': [665], 'atom': [667, 2988], 'retains': [668], 'its': [669, 709, 1177, 1449], 'four': [670, 2070, 2283], 'valence': [671, 1810], 'as': [673, 681, 858, 1559, 1688, 1706, 1821, 1996, 2006, 2016, 2026, 2195, 2345, 2443, 2468, 2478, 2567, 2569, 2791, 3280, 4927], 'electron': [675, 736, 2630, 2754, 2910], 'pairs.30': [676], 'Carbones': [677], 'recognized': [680], 'four-electron': [682, 2346], 'donors,': [683, 2350], 'distinctively': [687], 'electronic': [689, 1435, 1462, 1509, 2448], 'structure': [690, 941, 1007, 1436, 1510], 'reactivity': [692], 'than': [693, 1074, 1093, 1159, 1340, 1474, 1853, 2368, 2393, 3030], 'carbenes.30–41': [694], 'One': [695], 'classical': [699], 'carbones,': [700], '(CDP)': [702], '1961,42': [707], 'fully': [712], 'investigated': [713], 'theoretical': [715, 3124], 'studies.43–46': [716], 'Although': [717], 'there': [718, 2397], 'various': [720, 2447], 'coordinated': [727, 1035], 'acceptors,47–50': [730], 'pairs': [737], 'donated': [741], 'same': [744, 2987], 'acceptor': [745, 1710, 2196], 'rare,51': [747], 'especially': [748], 'f-block': [750], 'elements.52': [751], 'report': [754], 'example': [757, 1229, 2978], 'core.': [775, 1241], 'uranium–carbon': [777, 2959, 2999, 3062], 'formed': [780, 1753], 'coordination': [783, 1129], 'ligands': [787, 2437], 'single': [790, 1038, 1077, 2379], 'center.': [792, 1040, 2300], 'Results': [793, 1873, 3973], 'Discussion': [795], '[(PyPh2P)2C]': [799], '(': [800, 813, 854, 1256, 1452, 1991, 2011, 3080], '1)': [801], 'tetrachloride': [804], '(UCl4)': [805], 'led': [806, 1176], '[(PyPh2P)2C=UCl4]': [812], '2)': [814], '(Figure': [820, 1016, 1311, 1492, 1645, 2104, 2587], '1a).52': [821], 'Further': [822, 3004], '2': [825, 827, 875, 885, 1067, 1162, 1281, 1312, 1410], 'equiv': [828, 833, 876, 881, 886], 'NaBPh4': [830, 888], '1': [832, 835, 878, 880, 928, 936, 1870], 'at': [836, 891, 944, 997, 1192, 1253, 1333, 1361, 1391, 1589, 1677, 1760, 1986, 2244, 2421, 2693, 2757, 2775, 2913, 2919, 3612, 4670, 4862], 'room': [837], 'temperature': [838], '(RT)': [839], 'tetrahydrofuran': [841], '(THF)': [842], 'resulted': [843], 'yellow-green': [849], 'suspension.': [850], '3)': [855, 1453, 3081], 'isolated': [857], 'yellowish': [859], 'green': [860], 'crystals': [861], '40%': [863], 'yield.': [864], 'Complex': [865, 1027, 1224, 3897], '3': [866, 896, 922, 934, 943, 992, 1009, 1028, 1046, 1090, 1122, 1175, 1225, 1248, 1304, 1329, 1438, 1740, 1752, 2918, 2956], 'can': [867, 1215, 1371, 1794, 2078, 2087, 2381, 2788, 3092], 'prepared': [870, 2966], 'THF': [890], 'RT': [892], 'directly.': [893], 'Crystalline': [894], 'moisture-sensitive,': [898], 'shows': [899, 1249, 1527, 1700, 2183, 2537, 2748, 2996, 3047], 'low': [900], 'solubility': [901], 'organic': [904], 'solvents,': [905], 'easily': [907, 2088], 'decomposes': [908], 'CDP': [911, 1031, 1732, 2343, 3015], 'ligand': [912, 1733], '1.': [913, 1834, 3211], 'Therefore,': [914, 2878], 'NMR,': [915], 'UV–vis,': [916], 'near-infrared': [918], 'spectra': [919], 'not': [924], 'obtained.': [926], 'Figure': [927, 1021, 1259, 1316, 1409, 1525, 1603, 1739, 2204, 2310, 2653, 2746, 2902], '|': [929, 1411, 1741, 1871, 2206, 2655, 2904], '(a)': [930], 'Synthesis': [931, 3346], '2.': [938, 3225], '(b)': [939], 'Solid-state': [940], '50%': [946], 'level.': [947, 1000, 1763, 2247, 2696, 2922], 'Hydrogen': [948], 'atoms': [949, 1759, 2340, 2741], 'BPh4−': [951], 'omitted': [954], 'clarity.': [956], 'Selected': [957], 'experimental': [958, 1490, 3114], '[calculated]': [959], 'distances': [961, 1097], '(Å)': [962], 'angles': [964], '(deg):': [965], 'U–C1': [966], '2.491(4)': [967, 1048], '[2.425],': [968], 'U–Cl1': [969], '2.6237(12)': [970, 1153], '[2.622],': [971], 'U–N1': [972], '2.646(3)': [973], '[2.633],': [974], 'U–N2': [975], '2.702(3)': [976], '[2.691],': [977], 'C1–P1': [978], '1.682(4)': [979], '[1.712],': [980], 'C1–P2': [981], '1.713(4)': [982], '[1.724];': [983], 'C1–U1-C1a': [984], '143.73(17)': [985], '[148.28].': [986], 'minimum': [988], 'geometry': [990], 'triplet': [994, 1460, 1818, 1993, 2024, 2230, 2453, 2476, 2679], 'ground': [995, 1354, 1463], 'state': [996, 2005, 2025, 2231, 2454, 2477, 2680], 'BP86-D3(BJ)/def2-SVP/Stuttgart': [999], 'solid-state': [1006], 'confirmed': [1011], 'X-ray': [1013, 2993, 3116], 'crystallographic': [1014, 2994, 3085, 3117], '1b': [1017], 'Supporting': [1019, 1257, 1314, 1502, 1523, 1601, 1657, 2308, 3106, 3108], 'Information': [1020, 1258, 1315, 1503, 1524, 1602, 1658, 2309, 3107, 3109, 5023], 'S3,': [1022], 'Tables': [1023], 'S1': [1024], 'S2).a': [1026], 'contains': [1029, 3082], 'ligands,': [1032], 'distance': [1044, 1056, 1079, 1111, 1120], 'Å,': [1049, 1154], 'comparable': [1052], 'U=CBIPM': [1055], '[U{C(SiMe3)(PPh2)}(BIPMTMS)(Cl)][Li(2,2,2-cryptand)]': [1058], '(2.459(2))12': [1059], '(2.471(7)': [1068], 'Å)52': [1069], 'obviously': [1072], 'shorter': [1073, 1158], '[UO2Cl2(IMes)2]': [1081], '(2.626(7)': [1082], 'Å).53': [1083], 'However,': [1084, 2396, 2801], 'length': [1088, 1151], 'longer': [1092, 1117, 2367, 2392], 'typical': [1095], '[U(CHPMe2Ph)(η5-C5H5)3]': [1099], '(2.293(2)': [1100], 'Å),5': [1101], '[U(CHPPh3){N(SiMe3)2}3]': [1102], '(2.278(8)': [1103], 'Å),8': [1104], '[U(BIPMTMS)(Cl)(μ-Cl)2Li(THF)2]': [1105], '(2.310(4)': [1106], 'Å),9': [1107], 'U=Ccarbene': [1110], '[U{C(SiMe3)(PPh2)}(BIPMTMS)(DMAP)2]': [1113], '(2.296(5)': [1114], 'Å).12': [1115], 'probably': [1124], 'due': [1125, 2156], 'greater': [1128], 'number': [1130, 1628], 'center': [1134, 1297, 1699, 2133], 'this': [1136, 1828, 2973, 3002, 3088], 'system.': [1137], 'These': [1138, 1284, 1398, 3090], 'data': [1139, 1285, 1415, 3086, 3091], 'suggest': [1140, 1286, 2413, 2613], 'character': [1144, 2355], 'U1–C1': [1146], '3.': [1148, 1299, 1408, 1418, 3250], 'U1–Cl1': [1150], 'slightly': [1157, 1338, 1357], '(av.': [1163], '2.648': [1164], 'Å).': [1165], 'Efforts': [1166], 'either': [1168], 'reduce': [1169], 'abstract': [1171], 'chloride': [1173], 'decomposition.': [1178], 'Unlike': [1179], 'nearly': [1183, 2520], 'linear': [1184], 'core,': [1186], 'C=U=C': [1188, 1201], 'angle': [1189, 1209], '3,': [1191, 1512, 2862], '143.73(17)°,': [1193], 'significantly': [1195, 3028], 'distorted': [1196], 'linearity.': [1198], 'bent': [1200], 'structural': [1202], 'feature': [1203], 'analogous': [1205], 'bending': [1208], '156°': [1211], 'C(CO)2,': [1213], 'rationalized': [1217], 'terms': [1219, 1619, 2324, 2536, 2627], 'OC→C←CO.49,50': [1223], 'Fourier-transform': [1243], 'infrared': [1244], '(FT-IR)': [1245], 'spectrum': [1246], 'vibration': [1251], 'band': [1252], '765.2': [1254], 'cm−1': [1255], 'S2,': [1260], 'computed': [1262], 'value': [1263, 1278, 1343, 1588, 2371, 2866, 2883], 'IR': [1265], 'active': [1266], 'C–U–C': [1267], 'asymmetric': [1268], 'stretching': [1269], '760.8': [1271], 'cm−1),': [1272], 'close': [1275], '(690': [1282], 'cm−1).': [1283], 'intrinsic': [1288], 'between': [1292, 1754, 2558, 2634, 3042], 'crystalline': [1301], 'sample': [1302], 'studied': [1306], 'variable-temperature': [1308], 'magnetic': [1309, 1326, 1359, 1384], 'measurements': [1310], 'S1)': [1317], 'on': [1318, 1442, 1726, 4156, 4167, 4428, 4458], 'superconducting': [1320], 'quantum': [1321, 2738], 'interference': [1322], 'device': [1323], '(SQUID).': [1324], 'moment': [1327, 1360, 1385], '3.27': [1331], 'μB': [1332, 1390], '300': [1334, 1362], 'K,': [1335], 'lower': [1339, 1358, 1471, 2503], 'expected': [1342], '(3.58': [1344], 'μB)': [1345], '5f2': [1348], 'U(IV)': [1349, 1368, 1404], 'ion': [1350], '3H4': [1353], 'state.54': [1355], 'K': [1363, 1393], 'attributed': [1373], 'quenching': [1376], 'spin–orbit': [1378], 'coupling.55,56': [1379], 'With': [1380], 'decreasing': [1381], 'temperature,': [1382], 'declines': [1386], 'smoothly': [1387], '0.50': [1389], '1.8': [1392], 'tends': [1395], 'zero.': [1397], 'results': [1399, 1826, 2608, 2735], 'consistent': [1401], 'formulation': [1405], 'Variable-temperature': [1412], 'SQUID': [1413], 'magnetization': [1414], 'Density': [1423], '(DFT)': [1426], 'calculations': [1427, 2430, 3006], 'performed': [1429], 'gain': [1431], 'insight': [1432], 'into': [1433], 'shed': [1440], 'light': [1441], 'stability': [1444], 'bonding.': [1450, 2386], 'Molecule': [1451, 3732, 3762, 4860], 'C2': [1456], 'symmetry': [1457], '3A': [1461], 'state,': [1464], '17.8': [1467], '37.4': [1469], 'kcal/mol': [1470], 'corresponding': [1476, 1595, 1770, 2096, 2220, 2669, 2864], 'quintet': [1477, 2013, 2465], 'singlet': [1479, 1815, 2004], 'states,': [1480], 'respectively.': [1481], 'calculated': [1483, 1495, 2497], 'geometrical': [1484], 'parameters': [1485], 'match': [1486], 'well': [1487, 2568], 'values': [1491, 2031, 2037, 2055, 2272, 2721], '1).': [1493], 'energies': [1496, 1844], 'coordinates': [1498], 'given': [1500, 2033], 'Table': [1504, 1659, 1833, 1869], 'S4.': [1505], 'To': [1506], 'understand': [1507], 'inspected': [1515], 'shape': [1517, 1577, 1743], 'molecular': [1520, 1534, 1552], 'orbitals': [1521, 1545, 1580, 1653, 1705, 1711, 1749, 2103, 2182, 2190, 2224, 2586, 2673], '(MOs).': [1522], 'S4': [1526], 'odd': [1530], '[singly': [1532], 'occupied': [1533, 1551], '(SOMO)': [1536], 'SOMO-1]': [1538], 'located': [1540, 2813], 'exclusively': [1541], 'f': [1544], 'U': [1548, 1590, 1756, 2781], 'atom.': [1549], 'Highest': [1550], '(HOMO)': [1554], 'HOMO-1': [1556], 'identified': [1558, 2090], 'sets': [1562], 'CDP→U': [1564, 1573, 1615, 1783, 1787], 'donations,': [1566], 'while': [1567], 'HOMO-2': [1568], 'HOMO-13': [1570], 'represent': [1571, 2937], 'donations.': [1575], 'SOMO': [1579], 'correlated': [1582], 'natural': [1585, 1607, 1651, 1716, 1806], 'spin': [1586, 1596], '(2.03': [1591], 'au),': [1592], 'plotted': [1599], 'S5.': [1604], '(NBO)': [1610], 'localizes': [1613], 'donations': [1617, 1785, 1789, 2286], '2c–2e': [1622, 1635], 'C–U': [1623, 1636, 1652, 2803, 2859], 'occupation': [1627], '(ON)': [1629], '1.66': [1631], 'e−': [1632, 1644, 1725, 1736], 'ON': [1641, 1771], '1.84': [1643], '3).': [1646], 'compositions': [1648], 'tabulated': [1655], 'S3.': [1660], 'Both': [1661], 'strongly': [1667], 'polarized': [1668], 'towards': [1669, 2780], 'end': [1672], '83%': [1674], '89%': [1676], 'carbon,': [1678], 'respectively,': [1679], 'agrees': [1681, 2199], 'model': [1684], 'acts': [1687], 'donor.': [1690], 'review': [1692], 'hybridization': [1695], 'contribute': [1712], 'almost': [1713], 'equally.': [1714], 'charge': [1717, 1722, 2256, 2262, 2296, 2417, 2705, 2711, 2768, 2816, 3097], 'distribution': [1718], 'gives': [1719, 2483], 'net': [1721], '0.38': [1724], 'UCl2': [1728, 1889, 2014, 2441, 2466, 2559, 2635, 2688], 'fragment,': [1729], 'indicating': [1730, 2870], 'each': [1731], 'donates': [1734, 2295], '0.81': [1735], 'UCl2.': [1738], 'σ-': [1746], 'π-natural': [1748], 'C': [1758, 2798], 'BP86-D3(BJ)/def2-TZVPP/Stuttgart//BP86-D3(BJ)/def2-SVP/Stuttgart': [1762], 'isovalue': [1765, 2267, 2716], '0.035': [1767], 'e/Å3.': [1768], 'provided.': [1774], 'their': [1791], 'individual': [1792], 'strengths': [1793], 'evaluated': [1796], 'using': [1798, 1990, 2236, 2431, 2515, 2609, 2685], '(EDA)': [1802], 'chemical': [1809], '(NOCV)': [1811], 'theory,': [1812], '(CDP)2': [1816, 1886, 2000, 2242, 2423], 'UCl22+': [1819, 1883, 1994, 2239], 'act': [1820], 'interacting': [1822, 2181, 2223, 2444, 2672], 'fragments.': [1823, 2332], 'numerical': [1825], 'shown': [1831, 2306], 'relative': [1836, 2507], 'size': [1837, 2253, 2702], '(ΔEorb)': [1840], 'electrostatic': [1842, 1854, 2511], '(ΔEelstat)': [1843], 'reveals': [1845, 2352], 'interaction': [1848, 2109, 2500, 2895], 'somewhat': [1850], 'more': [1851, 2841], 'covalent': [1852, 2173, 2513, 2850, 2872], 'nature,': [1856], 'whereas': [1857], 'dispersion': [1859], 'contribution': [1860], 'substantial,': [1862], 'contributing': [1863], '7%': [1864], 'total': [1867, 2046, 2064, 2143, 2313, 2498], 'attraction.': [1868], 'EDA-NOCV': [1872], 'Triplet': [1876], '(CDP)2UCl22+': [1877, 2234, 2408, 2456, 2624, 2683], 'Complexa': [1878], 'B': [1880], 'Energies': [1881], 'Interaction': [1882, 1888], '(T)': [1884, 1893, 1995, 2021, 2240, 2473, 2639, 2692], '+': [1885, 1891, 2050, 2052, 2241, 2690], '(S)': [1887, 2001, 2243], '(Q)': [1890, 2015, 2467, 2560, 2636, 2689], '(CDP)22+': [1892, 2020, 2472, 2562, 2638, 2691], 'ΔEint': [1894], '−480.2': [1895], '−322.1': [1896], 'ΔEPauli': [1897], '313.9': [1898], '375.8': [1899], 'ΔEdispb': [1900], '−55.0': [1901], '(6.9%)': [1902], '−54.1': [1903], '(7.8%)': [1904], 'ΔEelstatb': [1905], '−338.1': [1906], '(42.6%)': [1907], '−278.2': [1908], '(39.9%)': [1909], 'ΔEorbb': [1910], '−401.0': [1911], '(50.5%)': [1912, 2896], '−365.6': [1913], '(52.3%)': [1914], 'ΔEorb1c': [1915], 'CDP(C)→[UCl2]2+←(C)CDP(+,': [1916, 1930, 1944, 1957], '+)': [1917, 1937, 1951, 1958, 2117, 2163, 2554, 2599], 'donation': [1919, 1933, 1947, 1953, 1960, 1966, 1972, 1977, 2124, 2316, 2601, 2796], '−73.5': [1920], '(18.3%)': [1921], 'CDP(C)+−[UCl2]−(C)CDP+(+,': [1922, 1936], '−)': [1923, 1931, 1945, 1964, 2121, 2160, 2550, 2595], '−148.4': [1927], '(40.6%)': [1928], 'ΔEorb2c': [1929], '−53.3': [1934], '(13.3%)': [1935], '−108.7': [1941], '(29.7%)': [1942], 'ΔEorb3c': [1943], '−27.4': [1948], '(6.8%)': [1949], 'CDP(C)+→[UCl2]←(C)CDP+(+,': [1950, 1963], '−23.1': [1954], '(6.3%)': [1955], 'ΔEorb4c': [1956], '−24.6': [1961], '(6.1%)': [1962], '−11.9': [1967], '(3.3%)': [1968], 'ΔEorb5c,d': [1969], 'CDP(N)→[UCl2]2+←(N)CDP': [1970, 2284], '−74.6': [1973], '(18.6%)': [1974], 'CDP(N)+→[UCl2]←(N)CDP+': [1975], '−29.5': [1978], '(8.1%)': [1979], 'ΔEorb(rest)': [1980], '−147.6': [1981], '(36.9%)': [1982], '−44.0': [1983], '(12.0%)': [1984], 'aEDA–NOCV': [1985], 'BP86-D3(BJ)/TZ2P-ZORA//BP86-D3(BJ)/def2-SVP/Stuttgart': [1988, 2246, 2695], 'level': [1989], 'A)': [1992], 'fragment': [1998, 2009, 2018, 2470, 2481, 2585], 'B)': [2012], 'fragment.': [2029], 'Energy': [2030, 2271, 2720], 'kcal/mol.': [2035, 2275, 2724], 'bThe': [2036], 'parentheses': [2039, 2057], 'percentage': [2042, 2060], 'contributions': [2043, 2061, 2508, 2590], 'attractive': [2047], 'interactions': [2048, 2066, 2514, 2528, 2541], 'ΔEelstat': [2049], 'ΔEorb': [2051, 2144, 2501], 'ΔEdisp.': [2053], 'cThe': [2054], 'ΔEorb.': [2067, 2320], 'dSum': [2068], 'components': [2071], 'given.': [2073], 'useful': [2076], 'information': [2077], 'extracted': [2080], 'pairwise': [2083, 2148, 2534], 'interactions,': [2085, 2150], 'plot': [2093, 2750, 2906], 'deformation': [2097, 2210, 2303, 2580, 2659], 'densities': [2098, 2211, 2304, 2581, 2660], 'associated': [2101, 2215, 2302, 2440, 2579, 2664], 'fragments': [2102, 2227, 2238, 2445, 2518, 2612, 2676, 2687], '4).': [2105], 'strongest': [2107], 'originates': [2110], 'in-phase': [2115, 2552, 2597], '(+,': [2116, 2120, 2159, 2162, 2549, 2553, 2594, 2598], 'out-of-phase': [2119, 2548, 2593], 'CDP(C)→[UCl2]2+←(C)CDP': [2122, 2164], '(ΔEorb1': [2125], 'ΔEorb2),': [2127], '(C)': [2129], 'denotes': [2130], 'CDP.': [2135], 'C→U': [2137], 'σ-donation': [2138], 'provides': [2139], '31.6%': [2140], 'value.': [2145], 'next': [2147], 'ΔEorb3': [2151], 'ΔEorb4,': [2153], 'likewise': [2155], 'donation,': [2166], 'accounts': [2168], '13%': [2170], 'interaction.': [2174], 'Inspection': [2175, 2531], 'composition': [2178], 'atomic': [2189], '(AOs)': [2191], 'serve': [2194], 'functions,': [2197], 'NBO': [2202, 2411], 'results.': [2203], '4': [2205], 'Shape': [2207, 2656], 'Δρ1–4,': [2212], 'ΔEorb1–4': [2217], 'important': [2222, 2671], 'eigenvalues': [2249, 2698], 'ν': [2250, 2699], 'indicate': [2251, 2700, 2927], 'migration.': [2257, 2706], 'direction': [2259, 2708], 'flow': [2263, 2712], 'red→blue.': [2265, 2714], '0.0005': [2269, 2718], 'au.': [2270, 2719], 'There': [2280, 2763], 'additionally': [2282], '(ΔEorb5)': [2287], 'nitrogen': [2290], 'pyridine': [2293], 'ring': [2294], 'S6.': [2311], 'N→U': [2314], 'contributes': [2317], '18.6%': [2318], 'remaining': [2322], 'mainly': [2325, 2419], 'come': [2326, 2546], 'polarization': [2329], 'within': [2330], 'EDA–NOCV': [2334, 2429, 2607, 2900], 'clearly': [2336], 'identifies': [2337], '(σ': [2347], 'π)': [2349], 'rather': [2360, 2649], 'long': [2361, 2650], 'even': [2366], 'standard': [2370], '2.45': [2373], 'Å': [2374], 'bond,57': [2380], 'explained': [2383], 'always': [2390], 'much': [2391, 2604], 'bonds.50': [2395], 'alternative': [2400, 2615], 'description': [2401, 2486, 2617], 'situation': [2405, 2491, 2621], 'complex.': [2409, 3003], 'charges': [2412], 'positive': [2416, 2820, 2853], 'localized': [2420], 'We': [2425, 2459], 'carried': [2426], 'out': [2427], 'further': [2428, 3035], 'singly': [2432], 'doubly': [2434], 'charged': [2435], '(CDP)2q': [2436], 'configurations': [2449], 'overall': [2452], 'retained.': [2458], 'found': [2460], 'use': [2463], 'reasonable': [2485], 'final': [2489], 'because': [2495], '(Table': [2504], '1).58–60': [2505], 'same,': [2522], 'types': [2525], 'different.': [2530], 'dominant': [2540], 'ΔEorb1': [2542], 'ΔEorb2': [2544], 'now': [2545], '(T),': [2563], 'involves': [2565], 'f(π)': [2566], 'd(π)': [2570], 'AOs': [2571], 'uranium.': [2573], 'connected': [2584], '5).': [2588], 'CDP(C)+→[UCl2]←(C)CDP+': [2602], 'smaller.': [2605], 'latter': [2611], 'unusual': [2616], 'sharing': [2631], 'bonding,': [2644], 'rationalizes': [2647], 'distances.': [2652], '5': [2654], 'Δρ1–2,': [2661], 'ΔEorb1–2': [2666], 'Finally,': [2729], 'elaborated': [2731], 'above': [2733], 'performing': [2737], 'molecules': [2743], '(QTAIM)': [2744], 'analysis.': [2745], '6': [2747, 2903], 'Laplacian': [2752, 2908], '(∇2ρ(r))': [2756], 'plane': [2759, 2916], 'C1–U–C1a': [2761, 2915], 'large': [2765, 2881, 2893], 'areas': [2766], 'concentration': [2769], '(indicated': [2770], 'red': [2772, 2934], 'dotted': [2773, 2935], 'region)': [2774], 'C1a': [2776], 'C1': [2778], 'directed': [2779], 'along': [2782], 'path': [2786], 'lone': [2794], 'pair': [2795], 'U.': [2800, 4098], 'critical': [2805], 'point': [2806], '(BCP),': [2807], 'indicated': [2808], 'blue': [2810, 2924], 'spheres,': [2811], 'outside': [2814], 'concentrated': [2817], 'region,': [2818], 'giving': [2819], '∇2ρ(rc)': [2821], 'values.': [2822], 'characteristic': [2827], 'polar': [2830], 'involving': [2832], 'heavy': [2833], 'elements.': [2834, 3060], 'local': [2836], 'H(rc),': [2839], 'reliable': [2842], 'descriptor': [2843], 'these': [2845, 2875], 'cases,': [2846], 'negative': [2848, 2882], 'noncovalent': [2855], 'bonds.61': [2856], 'H(rc)': [2865, 2885], '−0.128': [2868], 'Hartree/Å3,': [2869], 'quite': [2880, 3025], 'corroborates': [2890], 'obtained': [2897, 3094], 'method.': [2901], 'density,': [2911], '∇2ρ(r)': [2912, 2930, 2941], 'BP86-D3(BJ)/def2-TZVPP/SARC-ZORA//BP86-D3(BJ)/def2-SVP/Stuttgart': [2921], 'solid': [2925], 'lines': [2926, 2936], 'area': [2928, 2939], '>': [2931], '0': [2932], '<': [2942], '0.': [2943], 'Blue': [2944], 'spheres': [2945], 'BCP.': [2948], 'Conclusion': [2953], 'successfully': [2965], 'characterized.': [2968], 'adduct': [2974], 'linked': [2984], 'molecule.': [2991], 'Single-crystal': [2992], 'short': [2998], 'DFT': [3005], 'support': [3007, 3200, 5097], 'assignment': [3009], 'center,': [3019], 'π-bond': [3022], 'strong,': [3026], 'although': [3027], 'weaker': [3029], 'σ-bond.': [3032], 'study': [3034], 'enhances': [3036], 'our': [3037], 'general': [3055], 'motif': [3057], 'actinide': [3059], 'Footnote': [3077], 'CCDC-2064061': [3079], 'supplementary': [3084], 'paper.': [3089], 'free': [3095], 'Cambridge': [3100], 'Crystallographic': [3101], 'Data': [3102], 'Centre': [3103], 'via': [3104, 3402, 4869], 'www.ccdc.cam.ac.uk/data_request/cif': [3105], 'available': [3111], 'includes': [3113], 'procedures,': [3115], 'analysis,': [3118], 'supporting': [3119, 3191, 5088], 'figures,': [3120], 'details': [3122], 'calculations.': [3125], 'Conflict': [3126], 'Interest': [3128], 'authors': [3130], 'declare': [3131], 'no': [3132], 'competing': [3133], 'interests.': [3134], 'Acknowledgments': [3135], 'research': [3137, 5034], 'supported': [3139, 5036], 'Natural': [3143, 5040], 'Science': [3144, 5041], 'Foundation': [3145, 5042], 'China': [3147, 5044], '(grant': [3148, 3205, 5045, 5102], 'nos.': [3149, 3206, 5046, 5103], '21772088,': [3150, 5047], '91961116,': [3151, 5048], '21973044),': [3153, 5050], 'Program': [3157, 5054], 'High-level': [3159, 5056], 'Entrepreneurial': [3160, 5057], 'Innovative': [3162, 5059], 'Talents': [3163, 5060], 'Province': [3166, 5063], '(individual': [3167, 5064], 'group': [3169, 5066], 'programs).': [3170, 5067], 'S.P.': [3171, 5068], 'thanks': [3172, 5069], 'University': [3175, 3189, 3204, 5072, 5086, 5101], 'postdoctoral': [3178, 5075], 'fellowship': [3179, 5076], 'High': [3182, 5079], 'Performance': [3183, 5080], 'Computing': [3184, 5081], 'computational': [3193, 5090], 'resources.': [3194, 5091], 'L.Z.': [3195, 5092], 'G.F.': [3197, 5094], 'acknowledge': [3198, 5095], 'financial': [3199, 5096], '39837123': [3207, 5104], '39837132).': [3209, 5106], 'References': [3210], 'Comyns': [3212], 'A.': [3213, 3254, 3433, 3509, 3540, 3557, 3573, 3803, 3881, 3926, 3933, 4039, 4071, 4107, 4899], 'E.The': [3214], 'Actinides.Chem.': [3219], 'Rev.1960,': [3220], '60,': [3221], '115–146.': [3222], 'Google': [3223, 3248, 3269, 3296, 3325, 3359, 3385, 3414, 3460, 3490, 3529, 3553, 3602, 3621, 3650, 3674, 3714, 3745, 3778, 3845, 3870, 3907, 3951, 3989, 4022, 4054, 4086, 4138, 4176, 4189, 4218, 4247, 4271, 4287, 4315, 4342, 4366, 4396, 4439, 4465, 4512, 4530, 4553, 4570, 4596, 4630, 4653, 4679, 4698, 4718, 4746, 4773, 4805, 4821, 4853, 4874, 4891, 4937, 4960, 4983, 5012], 'Scholar': [3224, 3249, 3270, 3297, 3326, 3360, 3386, 3415, 3461, 3491, 3530, 3554, 3603, 3622, 3651, 3675, 3715, 3746, 3779, 3846, 3871, 3908, 3952, 3990, 4023, 4055, 4087, 4139, 4177, 4190, 4219, 4248, 4272, 4288, 4316, 4343, 4367, 4397, 4440, 4466, 4513, 4531, 4554, 4571, 4597, 4631, 4654, 4680, 4699, 4719, 4747, 4774, 4806, 4822, 4854, 4875, 4892, 4938, 4961, 4984, 5013], 'Katz': [3226], 'J.': [3227, 3306, 3309, 3391, 3504, 3535, 3566, 3628, 3791, 3921, 3969, 4006, 4032, 4064, 4104, 4119, 4833, 4967], 'J.;': [3228, 3255, 3258, 3419, 3424, 3434, 3497, 3499, 3510, 3541, 3558, 3574, 3682, 3718, 3753, 3786, 3797, 3875, 3877, 3882, 3929, 3934, 4035, 4040, 4067, 4072, 4099, 4105, 4108, 4117, 4347, 4377, 4726, 4778], 'Seaborg': [3229], 'G.': [3230, 3569, 3996, 4412, 4490], 'T.;': [3231, 3329, 3331, 3468, 3536, 3958, 4473, 4608, 4942], 'Morss': [3232], 'L.': [3233, 4122, 4941], 'R.The': [3234], 'Actinide': [3238, 3285, 3945], 'Elements,': [3239], '2nd': [3240], 'ed.;': [3241], 'Chapman': [3242], 'Hall:': [3244], 'New': [3245, 4668, 4673], 'York,': [3246], '1986.': [3247], 'Gregson': [3251, 3537, 3910], 'M.;': [3252, 3337, 3538, 3578, 3629, 3678, 3911, 3997, 4027, 4059, 4253, 4319, 4374, 4478, 4634, 4704, 4724, 4781, 4834, 4907, 4945, 4965], 'Wooles': [3253, 3539, 3556], 'Cooper': [3256, 3417, 3495, 3784, 3873], 'O.': [3257, 3418, 3496, 3785, 3874, 4825], 'Liddle': [3259, 3435, 3511, 3542, 3585, 3883, 3937, 4041, 4073], 'S.': [3260, 3436, 3512, 3543, 3586, 3805, 3884, 3938, 3999, 4042, 4074, 4093, 4352, 4379, 4780], 'T.Covalent': [3261], 'Carbene': [3263, 3352, 3446, 3520, 3865, 4201, 4798, 4916], 'Chemistry.Comment.': [3264], 'Inorg.': [3265], 'Chem.2015,': [3266], '35,': [3267], '262–294.': [3268], '4.': [3271], 'Cai': [3272], 'W.;': [3273, 3363, 3431, 3507, 3571, 3580, 3626, 3801, 3879, 3931, 4037, 4069, 4148, 4540, 4730, 4750, 4831], 'Chen': [3274, 3276, 4405, 4468], 'C.-H.;': [3275], 'N.;': [3277, 3472, 3855, 4004, 4606, 4706, 4900], 'Echegoyen': [3278], 'L.Fullerenes': [3279], 'Nanocontainers': [3281], 'Stabilize': [3283], 'Unique': [3284], 'Species': [3286], 'Inside:': [3287], 'Structures,': [3288], 'Formation,': [3289], 'Reactivity.Acc.': [3291], 'Chem.': [3292, 3321, 3355, 3410, 3455, 3486, 3524, 3548, 3646, 3670, 3710, 3774, 3841, 4172, 4213, 4242, 4266, 4282, 4310, 4337, 4362, 4392, 4434, 4460, 4508, 4526, 4548, 4675, 4693, 4714, 4741, 4849, 4933, 5007], 'Res.2019,': [3293], '52,': [3294], '1824–1833.': [3295], '5.': [3298], 'Cramer': [3299], 'R.': [3300, 3303, 3955], 'E.;': [3301, 3494, 3533, 3721, 3913, 3964, 4030, 4114], 'Maynard': [3302], 'B.;': [3304, 3584, 3723, 3751, 4227, 4296, 4323, 4519, 4521, 4538, 4722], 'Paw': [3305], 'C.;': [3307, 3924, 3927, 4350, 4371, 4443, 4828, 4895], 'Gilje': [3308], 'W.A': [3310], 'Uranium-Carbon': [3311], 'Multiple': [3312, 3438, 3588, 3764], 'Bond.': [3313], 'Crystal': [3314], 'Structure': [3317, 3887, 4045, 4795, 4913], '(η5-C5H5)3UCHP(CH3)2(C6H5).J.': [3319], 'Am.': [3320, 3354, 3409, 3485, 3645, 3669, 3709, 3773, 3840, 4171, 4361, 4391, 4507, 4525, 4848, 4932], 'Soc.1981,': [3322], '103,': [3323], '3589–3590.': [3324], '6.': [3327], 'Cantat': [3328, 3467, 3957], 'Arliguie': [3330], 'Noël': [3332], 'A.;': [3333, 3936, 4102, 4223, 4251, 4294, 4414, 4492, 4610], 'Thuéry': [3334, 3469, 3852], 'P.;': [3335, 3422, 3470, 3561, 3783, 3853, 3916, 4321, 4826, 4878], 'Ephritikhine': [3336, 3473, 3605, 3859], 'Floch': [3338, 3856], 'P.': [3339, 3857, 3993, 4113, 4413, 4491], 'L.;': [3340, 3505, 3567, 3582, 3632, 3680, 3749, 3792, 3858, 3922, 3961, 3994, 4033, 4065, 4142, 4445, 4475, 4702, 4758, 4784, 4968], 'Mézailles': [3341, 3471, 3854], 'N.The': [3342], 'Bond:': [3345, 3372], 'Study': [3348, 3377], 'Nucleophilic': [3351, 3864], 'Complexes.J.': [3353, 4360], 'Soc.2009,': [3356], '131,': [3357], '963–972.': [3358], '7.': [3361], 'Ren': [3362], 'Deng': [3364], 'X.;': [3365, 4754], 'Zi': [3366, 4145], 'G.;': [3367, 3394, 3656, 4002, 4144, 4146, 4180, 4325, 4447, 4496, 4600, 4638, 4760, 4909, 4947], 'D.-C.The': [3369], 'Th=C': [3370], 'An': [3373], 'Experimental': [3374, 4163], 'Computational': [3376, 4165], 'Thorium': [3379], 'Poly-Carbene': [3380], 'Complexes.Dalton': [3381, 3866], 'Trans.2011,': [3382], '40,': [3383], '9662–9664.': [3384], '8.': [3387], 'Fortier': [3388, 3653], 'S.;': [3389, 3429, 3654, 3795, 4123, 4604, 4752, 4756, 4897], 'Walensky': [3390, 4118], 'R.;': [3392, 3967, 4120, 4193, 4255, 4534, 4557, 4574, 4602, 4640, 4728, 4810, 4902], 'Wu': [3393, 3655], 'Hayton': [3395, 3624, 3657], 'T.': [3396, 3570, 3625, 3658], 'W.Synthesis': [3397, 3659, 4450], 'Phosphorano-Stabilized': [3400], 'U(IV)-Carbene': [3401], 'One-Electron': [3403], 'Oxidation': [3404], 'U(III)-Ylide': [3407], 'Adduct.J.': [3408], 'Soc.2011,': [3411, 3487], '133,': [3412, 3488], '6894–6897.': [3413], '9.': [3416], 'Mills': [3420, 3559, 3781, 3914], 'D.': [3421, 3560, 3782, 3915, 3963, 4026, 4058, 4373, 4449, 4477, 4792, 4809, 4906, 4944, 4964], 'McMaster': [3423, 3498, 3796, 3876, 3928, 4034, 4066], 'Moro': [3425, 3798], 'F.;': [3426, 3501, 3563, 3576, 3788, 3799, 3918, 4061, 4516, 4536], 'Davies': [3427, 3793], 'E.': [3428, 3503, 3565, 3634, 3790, 3794, 3920, 3966, 4063, 4116], 'Lewis': [3430, 3506, 3579, 3800, 3878, 3930, 4036, 4068, 4106, 4590, 4665], 'Blake': [3432, 3508, 3802, 3880, 3932, 4038, 4070], 'T.Uranium-Carbon': [3437], 'Bonding:': [3439], 'Facile': [3440], 'Access': [3441, 3861], 'Pentavalent': [3444], '[U{C(PPh2NSiMe3)2}(Cl)2(I)]': [3447], 'Comparison': [3449, 3829], 'UV=C': [3451], 'UIV=C': [3453], 'Bonds.Angew.': [3454], 'Int.': [3456, 3525, 3549, 4214, 4243, 4267, 4283, 4311, 4338, 4435, 4461, 4549, 4694, 4742, 5008], 'Ed.2011,': [3457, 4743], '50,': [3458, 4744], '2383–2386.': [3459], '10.': [3462], 'Tourneux': [3463, 3848], 'J.-C.;': [3464, 3466, 3849], 'Berthet': [3465, 3850], 'M.Exploring': [3474], 'Uranyl': [3476, 3666, 3823, 4013, 4801], 'Organometallic': [3477], 'Chemistry:': [3478], 'From': [3479], 'Single': [3480], 'Uranium−Carbon': [3483], 'Bonds.J.': [3484, 4931], '6162–6165.': [3489], '11.': [3492], 'Lu': [3493, 3532, 3912], 'Tuna': [3500, 3562, 3787, 3917, 4028, 4060], 'McInnes': [3502, 3564, 3789, 3919, 4031, 4062], 'T.Synthesis,': [3513], 'Characterization,': [3514], 'Reactivity': [3516, 4160, 4503, 4735, 4868], 'Uranium(VI)': [3519], 'Imido': [3521, 3638], 'Oxo': [3522, 4014], 'Complex.Angew.': [3523], 'Ed.2014,': [3526, 4695], '53,': [3527, 4696], '6696–6700.': [3528], '12.': [3531], 'Boronski': [3534], 'T.Silyl-Phosphino-Carbene': [3544], 'Complexes': [3545, 3642, 3758, 4011, 4583, 4644, 4799], 'Uranium(IV).Angew.': [3547], 'Ed.2018,': [3550], '57,': [3551], '5506–5511.': [3552], '13.': [3555], 'Law': [3568], 'Fuller': [3572], 'Kremer': [3575], 'Ridgway': [3577], 'Gagliardi': [3581, 4121], 'Vlaisavljevich': [3583], 'T.Uranium(III)-Carbon': [3587], 'Bonding': [3589, 4158, 4616, 4709, 4951, 4976, 4992], 'Supported': [3590], 'Arene': [3592], 'δ-Bonding': [3593], 'Mixed-Valence': [3595], 'Hexauranium': [3596], 'Nanometre-Scale': [3597], 'Rings.Nat.': [3598], 'Commun.2018,': [3599], '9,': [3600, 4771], '2097.': [3601], '14.': [3604], 'M.The': [3606], 'Vitality': [3607], 'Dawn': [3614], 'XXIst': [3617], 'Century.Dalton': [3618], 'Trans.2006,': [3619], '2501–2516.': [3620], '15.': [3623], 'Boncella': [3627], 'Scott': [3630, 3959, 4782], 'B.': [3631, 3684, 3720, 3755, 3960, 4101, 4783], 'Batista': [3633, 3965], 'R.Exchange': [3635], 'Ligand': [3639, 4300, 4329], 'Bis(imido)': [3641], 'Uranium.J.': [3644], 'Soc.2006,': [3647], '128,': [3648], '12622–12623.': [3649], '16.': [3652], 'Nitrido-Substituted': [3662], 'Analogue': [3663, 3819], 'Ion,': [3667], '[N=U=O]+.J.': [3668], 'Soc.2010,': [3671], '132,': [3672], '6888–6889.': [3673], '17.': [3676], 'Zhou': [3677], 'Andrews': [3679, 3724, 3748], 'Li': [3681, 3717, 3752], 'Bursten': [3683, 3719, 3754], 'E.Reaction': [3685], 'Laser-Ablated': [3687], 'Atoms': [3689, 3738, 3769, 4624], 'CO:': [3691], 'Infrared': [3692], 'Spectra': [3693], 'CUO,': [3696], 'CUO−,': [3697], 'OUCCO,': [3698], '(η2-C2)UO2,': [3699], 'U(CO)x': [3701], '(x': [3702], '1−6)': [3704], 'Molecules': [3705, 4208], 'Solid': [3707], 'Neon.J.': [3708], 'Soc.1999,': [3711], '121,': [3712], '9712–9721.': [3713], '18.': [3716], 'Liang': [3722, 3750], 'L.Noble': [3725], 'Gas-Actinide': [3726, 3757], 'Compounds:': [3727, 4687], 'Complexation': [3728], 'CUO': [3731, 3761], 'Ar,': [3734, 3765], 'Kr,': [3735, 3766], 'Xe': [3737, 3768], 'Noble': [3740], 'Gas': [3741], 'Matrices.Science2002,': [3742], '295,': [3743], '2242–2245.': [3744], '19.': [3747], 'E.Noble': [3756], 'Noble-Gas': [3771], 'Matrices.J.': [3772], 'Soc.2003,': [3775], '125,': [3776], '3126–3139.': [3777], '20.': [3780], 'J.Liddle': [3804], 'T.Synthesis': [3806, 3885, 4043], 'Uranium(VI)-Carbene:': [3809], 'Reductive': [3810, 4017], 'Formation': [3811, 4130], 'Uranyl(V)-Methanides,': [3813], 'Oxidative': [3814], 'Preparation': [3815], '[R2C=U=O]2+': [3818], '[O=U=O]2+': [3822], 'Ion': [3824], '(R': [3825], 'Ph2PNSiMe3),': [3827], 'Nature': [3832], 'UIV=C,': [3834], 'UV=C,': [3835], 'UVI=C': [3837], 'bonds.J.': [3839], 'Soc.2012,': [3842], '134,': [3843], '10047–10054.': [3844], '21.': [3847], 'J-C.;': [3851], 'M.Easy': [3860], 'Trans.2010,': [3867, 3904], '39,': [3868, 3905], '2494–2496.': [3869], '22.': [3872], '[U{C(PPh2NMes)2}2]': [3889], '(Mes': [3890], '2,4,6-Me3C6H2):': [3892], 'Homoleptic': [3894], 'Bis(carbene)': [3896, 3946], 'Formal': [3900], 'Bonds.Dalton': [3903], '5074–5076.': [3906], '23.': [3909], 'Hennig': [3923], 'Scheinost': [3925], 'Kerridge': [3935], 'T.The': [3939], 'Inverse-Trans-Influence': [3940], 'Tetravalent': [3942], 'Lanthanide': [3943], 'Complexes.Nat.': [3947], 'Commun.2017,': [3948], '8,': [3949], '14137.': [3950], '24.': [3953], 'Thomson': [3954], 'K.;': [3956, 4613, 4636], 'Morris': [3962], 'Kiplinger': [3968], 'L.Uranium': [3970], 'Azide': [3971], 'Photolysis': [3972], 'C–H': [3975], 'Bond': [3976, 4764], 'Activation': [3977, 4382, 4861], 'Provides': [3979], 'Evidence': [3980, 4203], 'Terminal': [3983, 4048], 'Nitride.Nat.': [3985], 'Chem.2010,': [3986], '2,': [3987], '723–729.': [3988], '25.': [3991], 'Arnold': [3992], 'Jones': [3995], 'Odoh': [3998, 4092], 'O.;': [4000, 4094, 4275], 'Schreckenbach': [4001], 'Magnani': [4003], 'Love': [4005], 'B.Strongly': [4007], 'Coupled': [4008], 'Binuclear': [4009], 'Uranium–Oxo': [4010], 'Rearrangement': [4015], 'Silylation.Nat.': [4018], 'Chem.2012,': [4019], '4,': [4020], '221–227.': [4021], '26.': [4024], 'King': [4025, 4057], 'F.': [4029, 4277, 4830], 'Nitride': [4050], 'Complex.Science2012,': [4051], '337,': [4052], '717–720.': [4053], '27.': [4056], 'T.Isolation': [4075], 'Characterization': [4077, 4839], 'Uranium(VI)–Nitride': [4080], 'Triple': [4081], 'Bond.Nat.': [4082], 'Chem.2013,': [4083], '5,': [4084], '482–488.': [4085], '28.': [4088], 'Anderson': [4089], 'N.': [4090, 4518], 'H.;': [4091, 4790], 'Yao': [4095], 'Y.;': [4096], 'Williams': [4097], 'Schaefer': [4100], 'Kiernicki': [4103], 'Goshert': [4109], 'M.': [4110, 4150, 4346, 4376], 'D.;': [4111, 4787, 4904, 4987], 'Fanwick': [4112], 'Schelter': [4115], 'Bart': [4124], 'C.Harnessing': [4125], 'Redox': [4126], 'Activity': [4127], 'Tris(imido)': [4133], 'Compounds.Nat.': [4134], 'Chem.2014,': [4135], '6,': [4136], '919–926.': [4137], '29.': [4140], 'Zhang': [4141], 'Hou': [4143], 'Ding': [4147], 'Walter': [4149], 'D.Influence': [4151], 'Orbitals': [4155], 'Organoactinides:': [4162], 'Studies': [4166, 4427], 'Metallacyclopropene.J.': [4170], 'Soc.2016,': [4173, 4934], '138,': [4174, 4935], '5130–5142.': [4175], '30.': [4178], 'Tonner': [4181, 4192, 4533, 4556, 4573, 4601], 'R.Divalent': [4182], 'Compounds.Pure': [4184], 'Appl.': [4185], 'Chem.2009,': [4186], '81,': [4187], '597–614.': [4188], '31.': [4191], 'G.C(NHC)2:': [4195], 'Divalent': [4196, 4279, 4546, 4766], 'Compounds': [4198, 4658], 'N-Heterocyclic': [4200], 'Ligands-Theoretical': [4202], 'Class': [4206], 'Promising': [4210], 'Properties.Angew.': [4212], 'Ed.2007,': [4215], '46,': [4216], '8695–8698.': [4217], '32.': [4220], 'Dyker': [4221, 4292], 'C.': [4222, 4257, 4293, 4349, 4370], 'Lavallo': [4224, 4290], 'V.;': [4225, 4291], 'Donnadieu': [4226, 4295, 4322], 'Bertrand': [4228, 4297, 4326, 4446], 'G.Synthesis': [4229, 4298, 4327], 'Extremely': [4232], 'Bent': [4233], 'Acyclic': [4234, 4423], 'Allene': [4235], '(A': [4236], '“Carbodicarbene”):': [4237], 'Strong': [4239], 'Donor': [4240], 'Ligand.Angew.': [4241], 'Ed.2008,': [4244, 4268, 4284, 4312], '47,': [4245, 4269, 4285, 4313], '3206–3209.': [4246], '33.': [4249], 'Fürstner': [4250, 4641], 'Alcarazo': [4252, 4633, 4731], 'Goddard': [4254, 4639, 4727], 'Lehmann': [4256], 'W.Coordination': [4258], 'Ene-1,1-Diamines': [4261], 'Prototype': [4264], '“Carbodicarbene”.Angew.': [4265], '3210–3214.': [4270], '34.': [4273], 'Kaufhold': [4274], 'Hahn': [4276], 'E.Carbodicarbenes:': [4278], 'Compounds.Angew.': [4281], '4057–4061.': [4286], '35.': [4289], 'Properties': [4301, 4330], 'Stable': [4303], 'Five-Membered-Ring': [4304], 'Allenes': [4305], 'Containing': [4306], 'Only': [4307], 'Second-Row': [4308], 'Elements.Angew.': [4309], '5411–5414.': [4314], '36.': [4317], 'Melaimi': [4318], 'Parameswaran': [4320, 4614], 'Persistent,': [4333], 'All-Carbon': [4334], 'Four-Membered-Ring': [4335], 'Allene.Angew.': [4336], 'Ed.2009,': [4339], '48,': [4340], '4792–4795.': [4341], '37.': [4344], 'Goldfogel': [4345, 4375], 'Roberts': [4348, 4369], 'Meek': [4351, 4378], 'J.Intermolecular': [4353], 'Hydroamination': [4354], '1,3-Dienes': [4356], 'Catalyzed': [4357], 'Bis(phosphine)carbodicarbene-Rhodium': [4359], 'Soc.2014,': [4363], '136,': [4364], '6227–6230.': [4365], '38.': [4368], 'Matías': [4372], 'J.Lewis': [4380], 'Acid': [4381], 'Carbodicarbene': [4384, 4455], 'Catalysts': [4385], 'Rh-Catalyzed': [4387], 'Hydroarylation': [4388], 'Dienes.J.': [4390], 'Soc.2015,': [4393], '137,': [4394], '6488–6491.': [4395], '39.': [4398], 'Hsu': [4399, 4415, 4493], 'Y.-C.;': [4400], 'Shen': [4401], 'J.-S.;': [4402], 'Lin': [4403], 'B.-C.;': [4404], 'W.-C.;': [4406, 4469, 4471], 'Chan': [4407], 'Y.-T.;': [4408], 'Ching': [4409], 'W.-M.;': [4410], 'Yap': [4411, 4489], 'C.-P.;': [4416, 4494], 'Ong': [4417, 4497], 'T.-G.Synthesis': [4418], 'Isolation': [4420], 'Tridentate': [4424], 'Bis(pyridine)carbodicarbene': [4425], 'Its': [4429], 'Structural': [4430], 'Implications': [4431], 'Reactivities.Angew.': [4433], 'Ed.2015,': [4436], '54,': [4437], '2420–2424.': [4438], '40.': [4441], 'Pranckevicius': [4442], 'Liu': [4444, 4483], 'Stephen': [4448], 'Carbodicyclopropenylidene:': [4453], 'Based': [4456], 'Solely': [4457], 'Carbon.Angew.': [4459], 'Ed.2016,': [4462], '55,': [4463], '5536–5540.': [4464], '41.': [4467], 'Shih': [4470], 'Jurca': [4472], 'Andrada': [4476, 4905, 4943, 4963], 'Peng': [4479], 'C.-J.;': [4480], 'Chang': [4481], 'C.-C.;': [4482], 'S.-K.;': [4484], 'Y.-P.;': [4486], 'Wen': [4487], 'Y.-S.;': [4488], 'T.-G.Carbodicarbenes:': [4498], 'Unexpected': [4499], 'π-Accepting': [4500], 'Ability': [4501], 'during': [4502], 'Small': [4505], 'Molecules.J.': [4506], 'Soc.2017,': [4509], '139,': [4510], '12830–12836.': [4511], '42.': [4514], 'Ramirez': [4515], 'Desai': [4517], 'Hansen': [4520], 'McKelvie': [4522], 'N.Hexaphenylcarbodiphosphorane,': [4523], '(C6H5)3PCP(C6H5)3.J.': [4524], 'Soc.1961,': [4527], '83,': [4528], '3539–3540.': [4529], '43.': [4532], 'Öxler': [4535], 'Neumüller': [4537], 'Petz': [4539, 4656], 'G.Carbodiphosphoranes:': [4542], 'Carbon(0).Angew.': [4547], 'Ed.2006,': [4550], '45,': [4551], '8038–8042.': [4552], '44.': [4555], 'G.Divalent': [4559, 4576], 'Part': [4562, 4579], '1:': [4563], 'Parent': [4564], 'Compounds.Chem.': [4565], 'Eur.': [4566, 4592, 4887, 4956, 4979], 'J.2008,': [4567, 4593, 4888], '14,': [4568, 4594], '3260–3272.': [4569], '45.': [4572], '2:': [4580], 'Protonation': [4581], 'Main': [4585, 4663, 4711], 'Group': [4586, 4622, 4664, 4712], 'Transition': [4588], 'Metal': [4589], 'Acids.Chem.': [4591], '3273–3289.': [4595], '46.': [4598], 'Klein': [4603], 'Takagi': [4605], 'Shimizu': [4607], 'Krapp': [4609], 'Pandey': [4611], 'K.': [4612, 4786], 'P.New': [4615], 'Modes': [4617], 'Carbon': [4619], 'Heavier': [4621], '14': [4623], 'Si–Pb.Chem.': [4625], 'Soc.': [4626], 'Rev.2014,': [4627, 4818], '43,': [4628], '5106–5139.': [4629], '47.': [4632], 'Radkowski': [4635], 'Mehler': [4637], 'A.Chiral': [4642], 'Heterobimetallic': [4643], 'Carbodiphosphoranes': [4646], 'Phosphinidene–Carbene': [4648], 'Adducts.Chem.': [4649], 'Commun.2013,': [4650], '49,': [4651], '3140–3142.': [4652], '48.': [4655], 'W.Addition': [4657], 'Carbones,': [4660], 'CL2,': [4661], 'Acids:': [4666], 'Glance': [4669], 'Old': [4671], 'Compounds.Coord.': [4674, 4713], 'Rev.2015,': [4676], '291,': [4677], '1–27.': [4678], '49.': [4681], 'G.Dative': [4683, 4708, 4973], 'Main-Group': [4686], 'Case': [4689], 'More': [4691], 'Arrows!Angew.': [4692], '6040–6046.': [4697], '50.': [4700], 'Hermann': [4703], 'Holzmann': [4705], 'Rev.2017,': [4715], '344,': [4716], '163–204.': [4717], '51.': [4720], 'Inés': [4721], 'Patil': [4723], 'Carreras': [4725], 'Thiel': [4729], 'M.Synthesis,': [4732], 'Structure,': [4733], 'Dihydrido': [4738], 'Borenium': [4739], 'Cation.Angew.': [4740], '8400–8403.': [4745], '52.': [4748], 'Sun': [4753], 'C.Double': [4762], 'Uranium.Nat.': [4769], 'Comm.2018,': [4770], '4997.': [4772], '53.': [4775], 'Oldham': [4776, 4779], 'W.': [4777, 4789, 4812], 'Abney': [4785], 'Smith': [4788], 'Costa': [4791], 'A.Synthesis': [4793], 'N-heterocyclic': [4797], 'Dichloride.Chem.': [4802], 'Commun.2001,': [4803], '1348–1349.': [4804], '54.': [4807], 'Kindra': [4808], 'Evans': [4811], 'J.Magnetic': [4813], 'Susceptibility': [4814], 'Complexes.Chem.': [4817], '114,': [4819], '8865−8882.': [4820], '55.': [4823], 'Lam': [4824], 'Anthon': [4827], 'Heinemann': [4829], 'O’Connor': [4832], 'Meyer': [4835, 4858], 'K.Structural': [4836], 'Spectroscopic': [4838], 'Charge-Separated': [4842], 'Benzophenone': [4844], 'Ketyl': [4845], 'Radical': [4846], 'Complex.J.': [4847], 'Soc.2008,': [4850], '130,': [4851], '6567−6576.': [4852], '56.': [4855], 'Castro-Rodríguez': [4856], 'I.;': [4857], 'K.Small': [4859], 'Complexes:': [4865], 'Control': [4866], 'Architecture.Chem.': [4871], 'Commun.2006,': [4872], '1353–1368.': [4873], '57.': [4876], 'Pyykkö': [4877], 'Atsumi': [4879], 'M.Molecular': [4880], 'Single-Bond': [4881], 'Covalent': [4882], 'Radii': [4883], 'Elements': [4885], '1–118.Chem.': [4886], '15,': [4889], '186–197.': [4890], '58.': [4893], 'Mohapatra': [4894], 'Kundu': [4896], 'Paesch': [4898], 'Herbst-Irmer': [4901], 'Stalke': [4903], 'Roesky': [4910], 'H.': [4911], 'W.The': [4912], 'Stabilized': [4917], 'Si2H2': [4918], 'May': [4919], 'Be': [4920], 'Equally': [4921], 'Well': [4922], 'Described': [4923], 'Coordinate': [4925], 'Classical': [4929], '10429−10432.': [4936], '59.': [4939], 'Scharf': [4940], 'Gessner': [4948], 'V.': [4949], 'H.The': [4950], 'Situation': [4952], 'Metalated': [4954], 'Ylides.Chem.': [4955], 'J.2017,': [4957], '23,': [4958, 5010], '4422−4434.': [4959], '60.': [4962], 'Casals-Sainz': [4966], 'Martín': [4969], 'Pendás': [4970], 'Á.;': [4971], 'Electron-Sharing': [4975], 'C2F4.Chem.': [4978], 'J.2018,': [4980], '24,': [4981], '9083−9089.': [4982], '61.': [4985], 'Cremer': [4986], 'Kraka': [4988], 'E.Chemical': [4989], 'without': [4991], 'Electron': [4993], 'Density-Does': [4994], 'Difference': [4996], 'Electron-Density': [4997], 'Analysis': [4998], 'Suffice': [4999], 'Description': [5002], 'Bond?Angew.': [5006], 'Ed.1984,': [5009], '627–628.': [5011], 'Previous': [5014], 'articleNext': [5015], 'article': [5016], 'FiguresReferencesRelatedDetails': [5017], 'Issue': [5018], 'AssignmentVolume': [5019], '4Issue': [5020], '6Page:': [5021], '1921-1929Supporting': [5022], 'Copyright': [5024], '&': [5025], 'Permissions©': [5026], '2021': [5027], 'Chinese': [5028], 'SocietyKeywordsuraniumDFT': [5030], 'calculationsuranium-carbon': [5031], 'bondcarbonecarbodiphosphoraneAcknowledgmentsThis': [5033], 'Downloaded': [5107], '1,034': [5108], 'times': [5109], 'PDF': [5110], 'DownloadLoading': [5111], '...': [5112]}, 'cited_by_api_url': 'https://api.openalex.org/works?filter=cites:W3179422784', 'counts_by_year': [{'year': 2024, 'cited_by_count': 1}, {'year': 2023, 'cited_by_count': 5}, {'year': 2022, 'cited_by_count': 4}], 'updated_date': '2025-01-11T02:05:38.910124', 'created_date': '2021-07-19'}
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