Publication Information

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3865, 3871, 3910, 3920, 3923, 3926, 3942, 3986, 4005, 4015, 4051, 4064, 4081, 4104, 4130, 4142, 4158, 4169, 4182, 4231, 4252, 4262, 4301, 4316, 4325], 'Supramolecular': [41, 72, 98, 116, 134, 199], 'Structure': [42, 73, 99, 117, 135, 200], 'Materials,': [44, 75, 101, 119, 137, 202], 'Department': [45, 52, 76, 102, 120, 138, 148, 203], 'Chemistry,': [47, 54, 78, 104, 122, 140, 150, 205], 'Jilin': [48, 79, 87, 105, 123, 141, 206], 'University,': [49, 62, 80, 88, 106, 124, 142, 158, 207], 'Changchun': [50, 81, 89, 107, 125, 143, 208], '130012': [51, 82, 108, 126, 144, 209], 'College': [55, 151], 'Arts': [57, 153], 'Sciences,': [59, 155], 'Northeast': [60, 156], 'Agricultural': [61, 157], 'Harbin': [63, 159], '150030': [64, 160], ',': [65, 91, 109, 127, 145, 161, 186, 3665], 'Man†': [67], 'The': [83, 330, 390, 414, 472, 630, 846, 1088, 1213, 1338, 1476, 1517, 1555, 1626, 1732, 1745, 1759, 2380, 2475, 2564, 2631, 2850, 2877, 2945, 2970, 3016, 3120, 3145, 3176, 3251, 3264, 3428, 3471, 3501, 3530, 3962, 4013, 4187, 4248], 'First': [84], 'Hospital': [85], '130021': [90], 'Bai': [93], 'Liu': [111, 129], 'Fu': [147], 'Hu': [163], 'Institute': [164, 213], 'Polymer': [166, 215], 'Optoelectronic': [167, 216], 'Materials': [168, 176, 217, 225], 'Devices,': [170, 178, 219, 227], 'Luminescent': [175, 224], 'South': [179, 228], 'China': [180, 229], 'University': [181, 230], 'Technology,': [183, 232], 'Guangzhou': [184, 233], '510640': [185, 234], '*Corresponding': [189], 'author:': [190], 'E-mail': [191], 'Address:': [192], '[email': [193], 'protected]': [194], 'https://doi.org/10.31635/ccschem.021.202000627': [235], 'SectionsSupplemental': [236], 'MaterialAboutAbstractPDF': [237], 'ToolsAdd': [238], 'to': [239, 404, 419, 524, 541, 723, 756, 762, 792, 829, 892, 949, 971, 1058, 1072, 1075, 1085, 1105, 1119, 1184, 1249, 1270, 1280, 1288, 1323, 1334, 1497, 1562, 1635, 1677, 1721, 1894, 1924, 2082, 2112, 2266, 2289, 2317, 2572, 2864, 2905, 2909, 2978, 3134, 3154, 3162, 3224, 3478, 3634, 3970, 4109, 4136, 4154, 4165, 4286, 4305, 4329], 'favoritesDownload': [240], 'CitationsTrack': [241], 'Citations': [242], 'ShareFacebookTwitterLinked': [243], 'InEmail': [244], 'light-emitting': [246, 562, 1235], 'diodes': [247, 563], '(OLEDs),': [248], 'which': [249, 425, 609, 827, 884, 935, 996, 1029, 1082, 1155, 1359, 1508, 1570, 2348, 2514, 2783, 2887, 3068, 3258, 3846, 3881, 3944, 4044, 4133, 4311, 4335], 'have': [250, 507, 565, 975, 1012, 1039], 'been': [251, 508, 550, 1040, 3091], 'recently': [252, 1513], 'utilized': [253], 'in': [254, 293, 427, 469, 484, 522, 533, 559, 568, 679, 719, 742, 760, 767, 775, 805, 842, 944, 992, 1016, 1070, 1102, 1135, 1170, 1209, 1436, 1440, 1450, 1502, 1683, 2332, 2347, 2364, 2401, 2446, 2449, 2619, 2627, 2705, 2733, 2747, 2774, 2793, 2871, 2933, 2941, 2962, 3036, 3086, 3247, 3282, 3359, 3376, 3387, 3413, 3437, 3442, 3451, 3482, 3488, 3542, 3557, 3586, 3627, 3637, 3652, 3658, 3689, 3710, 3749, 3771, 3813, 3835, 3883, 3895, 3901, 3916, 3932, 3950, 3965, 3989, 4019, 4107, 4111, 4189, 4207, 4233, 4267, 4290], 'some': [255, 2910, 4155], 'flat-panel': [256, 578], 'display': [257], 'screens': [258], 'such': [259, 494, 4215], 'as': [260, 321, 495, 511, 556, 575, 601, 790, 1294, 1304, 1566, 1568, 1608, 1610, 1763, 2376, 2517, 2637, 2639, 2779, 2842, 2844, 3106, 3234, 3245, 3592, 3612, 3614, 3656, 3899, 4030, 4216, 4265], 'mobile': [261], 'phones': [262], 'televisions,': [264], 'show': [265, 1181, 2412], 'many': [266], 'merits,': [267], 'including': [268, 3679], 'light': [269, 590, 666], 'weight,': [270], 'high': [271, 301, 593, 758, 838, 852, 869, 988, 1107, 1133, 1161, 1165, 1189, 1272, 1433, 1567, 1609, 2441, 3080, 3839, 3892, 3940, 3963, 4217], 'flexibility,': [272], 'energy': [273, 3030, 3051, 3124, 3266, 3289, 3405], 'preservation,': [274], 'so': [276], 'forth,': [277], 'are': [279, 303, 393, 530, 610, 749, 967, 1553, 1629, 2570, 3034, 3389, 3440, 3449], 'considered': [280, 1069, 1225], 'the': [281, 322, 363, 395, 405, 420, 437, 462, 480, 534, 569, 576, 625, 639, 658, 665, 673, 684, 691, 698, 708, 717, 720, 735, 738, 764, 768, 773, 781, 794, 810, 843, 931, 945, 993, 1018, 1031, 1059, 1073, 1080, 1086, 1098, 1126, 1158, 1182, 1200, 1251, 1254, 1305, 1325, 1335, 1348, 1362, 1365, 1369, 1373, 1384, 1393, 1396, 1400, 1405, 1410, 1416, 1419, 1426, 1446, 1468, 1498, 1503, 1512, 1578, 1590, 1605, 1631, 1643, 1648, 1655, 1658, 1661, 1666, 1897, 1913, 2085, 2101, 2270, 2294, 2300, 2305, 2312, 2319, 2335, 2368, 2377, 2413, 2450, 2457, 2487, 2518, 2557, 2574, 2628, 2640, 2650, 2663, 2671, 2678, 2682, 2688, 2695, 2706, 2728, 2734, 2740, 2748, 2754, 2762, 2794, 2819, 2830, 2833, 2854, 2872, 2883, 2893, 2899, 2906, 2914, 2919, 2934, 2942, 2949, 2968, 2973, 2996, 3005, 3020, 3028, 3071, 3101, 3111, 3197, 3202, 3225, 3241, 3248, 3261, 3270, 3293, 3385, 3390, 3410, 3446, 3461, 3468, 3485, 3494, 3519, 3523, 3537, 3543, 3558, 3583, 3593, 3604, 3620, 3628, 3646, 3653, 3666, 3690, 3705, 3731, 3736, 3783, 3791, 3796, 3800, 3807, 3853, 3872, 3876, 3887, 3902, 3917, 3924, 3933, 3948, 3971, 4000, 4049, 4067, 4077, 4082, 4137, 4149, 4159, 4174, 4227, 4273, 4287, 4291, 4295, 4299, 4323], 'next-generation': [282, 577], 'displays': [283, 579, 1462, 1523], 'solid-state': [285, 581, 1021], 'lightings.': [286], 'Blue-emitting': [287], 'materials': [288, 506, 1096, 1101, 1142, 1179, 1268, 1691], 'that': [289, 966, 1066, 1383, 1576, 2538, 2988, 3093, 3189, 3214, 3232, 3479, 3722, 3829, 3851, 3999, 4110, 4201, 4315], 'can': [290, 635, 1558, 1599], 'be': [291, 636, 1068, 1120, 1223, 1247, 1281, 1601, 3155, 3222, 3255, 4306, 4330], 'applied': [292, 510], 'nondoped': [294, 331, 399, 410, 776, 847, 896, 946, 979, 1518, 1591, 1638], 'OLEDs': [295, 401, 745, 761, 1038, 1136, 1204, 1640], 'with': [296, 337, 436, 822, 856, 915, 987, 1003, 1143, 1453, 1484, 1511, 1531, 1751, 1904, 2092, 2371, 2404, 2486, 2674, 2691, 2720, 3285, 3362, 3550, 3753, 3821, 3886, 3947, 3991, 4066, 4101, 4144, 4258], 'little': [297, 3715], 'efficiency': [298, 348, 358, 384, 618, 661, 668, 678, 687, 759, 902, 1108, 1130, 1207, 1620, 3394, 3894], 'roll-offs': [299, 385, 1131, 1208, 1621], 'at': [300, 367, 371, 784, 1132, 1188, 1442, 1528, 1736, 2293, 2469, 2511, 3400, 3547, 3573, 3624, 4098, 4126], 'brightness': [302, 340, 373, 870, 1110, 1134, 1548, 1606], 'great': [305], 'importance.': [306], 'Here,': [307], 'highly': [309, 2716, 3638, 3896, 3934], 'efficient,': [310], 'blue-emitting': [311, 848, 1267], 'material,': [312], '9-phenyl-10-(4-(pyren-1-yl)phenyl)-9H-pyreno[4,5-d]imidazole': [313, 1342], '(PyPI-Py),': [314, 1343], 'is': [315, 365, 417, 459, 620, 657, 683, 1030, 1050, 1079, 1193, 1301, 1321, 1381, 1509, 1571, 1607, 1669, 3407, 3419, 3847, 3882, 4312], 'achieved': [316, 898, 1157], 'using': [317, 1043, 2367, 4025], 'pyrene[4,5-d]imidazole': [318, 983, 1336, 1388, 2935], 'pyrene': [320, 555, 598, 695, 747, 782, 1022, 1315, 1320, 1390, 1413, 1585, 1644, 1652, 2562, 2689, 2777, 2900, 2924, 2943, 2983, 3230, 4162, 4202], 'weak': [323, 1283, 1296, 1306, 1330, 2756, 2781, 3236], 'electron': [324, 327, 1297], 'donor': [325, 1174], 'acceptor,': [328], 'respectively.': [329, 2474, 2496], 'blue': [332, 400, 412, 589, 607, 927, 1203, 1234, 1525, 1592, 1639], 'OLED': [333, 628, 849, 897, 928, 980, 1519], 'exhibits': [334, 1432], 'excellent': [335, 491, 585, 1684], 'performance': [336, 407, 416, 774], 'maximum': [339, 346, 355, 438, 900, 910, 999, 1539, 1547, 1564, 4095, 4128], '75,687': [342, 1550], 'cd': [343, 351, 378, 873, 906, 942, 1543, 1551, 1614], 'm−2,': [344, 379, 1615], 'current': [347, 901], '13.38': [350, 1542], 'A−1,': [352], 'external': [356], 'quantum': [357, 617, 677, 1434, 3393], '(ηext)': [359, 619], '8.52%.': [361], 'Moreover,': [362, 1458], 'ηext': [364, 634, 736, 853, 911, 951, 1000, 1025, 1078, 1187, 1201, 1557, 1594], 'maintained': [366], '8.35%': [368, 1596], '8.05%': [370, 1598], '10,000': [375, 1611], '50,000': [377, 1613], 'respectively,': [380, 1616, 3160, 3281], 'displaying': [381, 1617], 'extremely': [382, 1618], 'small': [383, 3050], '2.0%': [387, 1623], '5.5%.': [389, 1625], 'device': [391, 1627, 1685, 3262, 3973], 'characteristics': [392, 1628], 'among': [394, 1630], 'highest': [396, 1556, 1632, 2632], 'values': [397, 1026, 1633, 2479, 2489, 3386, 3949, 4050], 'for': [398, 409, 553, 606, 613, 624, 672, 697, 1035, 1054, 1061, 1196, 1232, 1266, 1589, 1637, 1742, 1846, 1885, 2015, 2023, 2073, 2230, 2238, 2576, 2768, 2813, 2957, 2967, 3032, 3110, 3704, 3755, 3789, 4194, 4198], 'correspond': [403], 'best': [406], 'obtained': [408, 997, 1309, 3291], 'pyrene-based': [411, 481, 798, 1044, 1210], 'OLEDs.': [413], 'superior': [415, 2552], 'attributed': [418, 3223], 'proper': [421], 'donor–acceptor': [422], 'design': [423, 1230, 2786], 'strategy': [424, 1231], 'results': [426, 483, 962, 3296], 'quasi-equivalent': [429, 3863, 3907], 'hybrid': [430, 1144], 'local': [431, 1145, 1420], 'charge-transfer': [433, 1374], 'excited': [434, 1149, 1421, 1663, 2834, 2846, 2873, 3025, 3116, 3654, 3737, 3787, 3832], 'state': [435, 722, 995, 1150, 1386, 1423, 1448, 1664, 1676, 2736, 2796, 2835, 2874, 3655, 3692, 3788, 3833, 3913, 3919], 'generation': [439, 713, 1417], 'an': [441, 925, 1263, 1472, 1485, 2506, 2560, 3107, 3228, 3911], '82%': [442], 'fraction': [443], 'singlet': [445, 1168, 1397, 2841, 2991, 3022, 3786], 'excitons.': [446], 'Download': [447, 449, 2428, 2430, 2595, 2597, 2822, 2824, 3757, 3759, 3776, 3778, 4084, 4086], 'figure': [448, 2429, 2596, 2823, 3758, 3777, 4085], 'PowerPoint': [450, 2431, 2598, 2825, 3760, 3779, 4087], 'Introduction': [451], 'Pyrene,': [452], 'consisting': [453, 3909], 'four': [455], 'fused': [456], 'benzene': [457], 'rings,': [458], 'one': [460, 3831], 'most': [463, 1099], 'widely': [464, 509], 'investigated': [465, 789, 1100], 'polycyclic': [466, 2436], 'aromatic': [467, 882, 2437], 'hydrocarbons': [468], 'recent': [470, 546, 1103, 1140], 'decades.1,2': [471], 'rigid': [473, 543, 692], 'planar': [474, 4145], 'structure': [475, 783, 1461, 3465, 3556, 3729], 'flat': [477], 'π-system': [478], 'component': [482], 'favorable': [485, 2565], 'π-electron': [486], 'flow,': [487], 'flexible': [488], 'self-assembly,': [489], 'photoelectric': [492], 'properties,': [493, 4214], 'bright': [496], 'emission,': [497, 591], 'efficient': [498, 588, 926, 1469], 'excimer': [499], 'formation,': [500], 'special-stacking': [502], 'topological': [503], 'configuration.3–7': [504], 'Pyrene-based': [505], 'biological': [512], 'probes': [513], 'fluorescent': [515, 1037, 1094], 'sensors': [516], 'because': [517, 1237, 2555, 2912, 3008, 3459, 3870, 4157], 'their': [519, 542, 802, 2405, 2603, 3190, 3286], 'tunable': [520], 'fluorescence': [521, 718, 3081, 4074], 'response': [523], 'environmental': [525], 'alteration.8–10': [526], 'Pyrene[4,5-d]imidazole-based': [527], 'organic': [528], 'dyes': [529], 'also': [531, 976, 1083, 1152, 1180, 2362, 4236, 4256], 'suitable': [532], 'applications': [535], 'dye-sensitized': [537], 'solar': [538], 'cells': [539], 'owing': [540, 1269], 'structure.11,12': [544], 'In': [545, 1139, 1257, 1318, 1377, 2497, 2661, 2711, 2994, 3200, 4088, 4147, 4294], 'years,': [547, 1141], 'there': [548, 1192, 3713], 'has': [549, 599, 3090], 'increasing': [551, 1017, 3662], 'interest': [552], 'developing': [554], 'semiconductor': [558], 'optoelectronics.1,2,13–17': [560], '(OLEDs)': [564], 'greatly': [566, 2860], 'progressed': [567], 'past': [570], 'decades': [571], 'shown': [573, 2331, 2618, 4266], 'potential': [574, 1049, 1183], 'lightings.18–20': [582], 'Because': [583, 3922], 'thermal': [586, 2442, 2553, 2566, 4221], 'stability,': [587, 4222], 'mobility': [594], 'charge': [596, 706], 'carrier,': [597], 'emerged': [600], 'very': [603, 868], 'appealing': [604], 'chromophore': [605], 'OLEDs,': [608, 777], 'urgently': [611], 'needed': [612], 'full-color': [614], 'displays.21–25': [615], 'External': [616], 'crucial': [622], 'parameter': [623], 'characterization': [626, 2329, 2415], 'performance.': [629, 1686, 3263, 3974], 'theoretical': [631, 1032, 1477, 3138, 3249, 3889], 'value': [632, 912, 952], 'calculated': [637, 2722, 3268, 4284, 4304, 4328], 'by': [638, 752, 1310, 1346, 1726, 1756, 1919, 2107, 2389, 3127, 3137, 3196, 3424, 3536, 4024], 'following': [640], 'equation:': [641], 'η': [642, 645, 648, 651], 'ext': [643], '=': [644, 1790, 1797, 1804, 1814, 1821, 1832, 1941, 1948, 1955, 1978, 2129, 2136, 2149, 2157, 2170, 2178, 2185, 3060], 'r': [646], '×': [647, 650, 653, 3367, 4308, 4319, 4332], 'out': [649, 2268], 'PL': [652, 3357, 3374, 3431, 3538, 3706, 3743, 3765, 3893, 4229, 4250], 'γ': [654, 682], 'where': [655], 'ηr': [656], 'exciton': [659, 2992], 'utilization': [660], '(EUE),': [662], 'ηout': [663], 'represents': [664, 2818], 'extraction': [667], '(20–30%),26': [669], 'ηPL': [670, 731, 839, 989, 1019, 1074, 1162, 1273, 1363, 3941, 3964, 4014, 4188, 4218], 'stands': [671], 'intrinsic': [674], 'photoluminescence': [675], '(PL)': [676], 'film,': [680, 4091], 'holes-electrons': [685], 'recombination': [686], '(ideally': [688], '100%).27': [689], 'Although': [690], 'architecture': [693], 'allows': [696], 'formation': [699], 'face-to-face': [701], 'π–π': [702, 795, 834], 'stacking': [703, 796, 835, 1465], 'enhanced': [705, 3598], 'migration,': [707], 'strong': [709, 1240, 1244, 2751, 2954, 3873, 4138], 'tendency': [710, 804], 'toward': [711], 'excimers': [712], 'will': [714, 1391, 1414], 'substantially': [715, 3239], 'quench': [716], 'solid': [721, 994, 1447], 'certain': [725, 2980], 'extent,': [726], 'yielding': [727], 'relatively': [729, 1329, 2755, 4122], 'low': [730, 831, 1206, 1619, 3837], 'further': [733, 1197, 1754, 1917, 2105, 2500, 3534, 3644, 3781], 'limiting': [734], 'resulting': [739, 1366, 1667, 1682, 1746, 2961], 'device.28,29': [740], 'Thus,': [741, 1191], 'prior': [743], 'studies,': [744], 'derivatives': [748], 'mostly': [750, 2668, 2685, 2896], 'fabricated': [751], 'doping': [753], 'technology': [754], 'aiming': [755], 'achieve': [757, 1076], 'avoid': [763, 1250], 'fluorescence-quenching': [765], 'effect': [766, 3643, 4141], 'aggregated': [769], 'state.30–32': [770], 'To': [771, 2601, 2826, 3780], 'improve': [772, 1361], 'rational': [778], 'modifications': [779], 'various': [785], 'positions': [786], 'were': [787, 1151, 1719, 2282, 2355, 2386, 2482, 2614, 2646, 2848, 3002, 3066, 3132, 3152, 3193, 3276, 3609, 4152, 4223, 4283], 'extensively': [788], 'well': [791, 1153, 2638, 2843, 2932, 3613], 'adjust': [793], 'molecules,': [799], 'thereby': [800], 'reducing': [801], 'aggregation': [803, 1474, 4140, 4210], 'condensed': [806], 'media': [807], 'fine-tuning': [809], 'optical': [811, 3288, 3404], 'properties.': [812], 'For': [813, 2298, 3618], 'example,': [814, 3619], 'Cheng': [815], 'et': [816, 876, 922], 'al.33': [817], 'prepared': [818, 878, 2363], 'dipyrenylbenzene-containing': [820], 'compound': [821, 1580, 2337], 'twisted': [824, 1464, 2717], 'molecular': [825, 1662, 2604, 2610, 2634, 2643, 2708, 2718, 3012, 3242, 4209], 'structure,': [826], 'led': [828], 'extent': [832, 2981, 4156], '75%': [841], 'film': [844, 1452, 3380, 3399, 4234, 4255], 'state.': [845, 2630, 3738, 4012], 'displayed': [850, 2445, 3441, 3455, 3979], '5.2%': [855], 'Commission': [857], 'Internationale': [858], 'de': [859], "l'Eclairage": [860], '(CIE)': [861], 'coordinates': [862, 917, 957, 1005], '(0.15,': [864, 959, 1536], '0.11)': [865], '40,400': [872], 'm−2.': [874], 'Huang': [875], 'al.34': [877], 'dumbbell-shaped': [880], 'spirocyclic': [881], 'hydrocarbon,': [883], 'realized': [885], 'large': [887, 2946, 3567, 4123], 'pyrene–pyrene': [888], 'distance': [889], 'up': [891], '10.4': [893], 'Å.': [894], 'Its': [895], '(CE)': [903], '7.4': [905, 1979], 'A−1': [907, 943, 1544], '4.6%': [914], 'CIE': [916, 956, 1004, 1533], '(0.16,': [919], '0.15).': [920], 'Chan': [921], 'al.35': [923], 'demonstrated': [924, 3726], 'based': [929, 981, 1520, 1641, 2310, 3805], 'solution-processable': [932], 'pyrene-1,3-alt-calix': [933], 'arene,': [934], 'exhibited': [936, 2527], 'record': [938], 'CE': [939, 1540], '10.5': [941, 1881, 2069], 'OLED,': [947], 'corresponding': [948, 1339, 1561, 3161, 3287, 3447], '6.4%': [954], '0.24).': [960], 'Such': [961], 'represent': [963, 1097], 'typical': [964, 1481, 2655, 3732, 3854], 'chromophores': [965], 'not': [968], 'inherently': [969], 'prone': [970], 'aggregate.': [972], 'Recently,': [973], 'we': [974], 'reported': [977, 1013, 1634], 'derivative': [984], "N,N-diphenyl-4'-(9-phenyl-9H-pyreno(4,5-d)imidazol-10-yl)-(1,1'-biphenyl)-4-amine": [985], '(PyPPA).': [986], '45%': [991], '8.47%': [1002], '(0.14,': [1007], '0.13).36': [1008], 'These': [1009, 2434], 'previous': [1010, 1259, 3903], 'studies': [1011], 'significant': [1014, 2703], 'achievements': [1015], 'derivatives.': [1023], 'Furthermore,': [1024, 3088, 3975, 4272], 'exceeding': [1027], '5%,': [1028], 'upper': [1033], 'limit': [1034], 'traditional': [1036, 1674], 'successfully': [1041, 1156, 4224], 'attained': [1042], 'materials.': [1045], 'Exploiting': [1046], "material's": [1048], 'never-ending': [1052], 'mission': [1053], 'scientist.': [1056], 'According': [1057], 'expression': [1060], 'ηext,': [1062], 'another': [1063], 'important': [1064], 'factor': [1065], 'must': [1067], 'addition': [1071], 'higher': [1077, 1574, 2484, 2544, 3021, 4313], 'ηr,': [1081], 'refers': [1084], 'EUE.': [1087], 'phosphorescent': [1089], 'thermally': [1091], 'activated': [1092], 'delayed': [1093], '(TADF)': [1095], 'years': [1104], 'realize': [1106], 'through': [1111, 1647], 'efficacious': [1112], 'triplet': [1113, 2845, 3024], 'harvesting.37–40': [1114], 'However,': [1115, 3484], 'they': [1116, 3724], 'usually': [1117], 'need': [1118], 'doped': [1121], 'into': [1122, 4008], 'appropriate': [1123, 3108], 'hosts,': [1124], 'problem': [1127], 'severe': [1129], 'remains': [1137], 'unresolved.': [1138], 'CT': [1147, 1385, 1490, 2986, 3514, 3525, 3531, 3650, 3855, 3866, 3877, 3927, 4001], '(HLCT)': [1148], 'developed,': [1154], 'merits': [1159], 'output': [1166], 'excitons': [1169], 'series': [1172], '(D)–acceptor': [1175], '(A)': [1176], 'materials.36,41–52': [1177], 'HLCT': [1178, 1482, 1500, 1515, 1680, 3044, 3115, 3912, 4011], 'maintain': [1185], 'stable': [1186, 1524], 'brightness.': [1190], 'still': [1194, 1600], 'room': [1195, 1895, 2083, 3401], 'enhancement': [1198], 'D–A': [1211, 1229, 2752], 'system.': [1212], 'electron-donating': [1214, 2757], '-withdrawing': [1216, 2759], 'strengths': [1217, 2760], 'D': [1219, 1241, 1291, 1307, 1349, 1406, 2763, 2855, 3102], 'A': [1221, 1245, 1331, 1352, 1411, 1538, 1854, 2041, 2765, 2857, 3104, 3237], 'should': [1222, 1246], 'carefully': [1224], 'when': [1226, 1286, 1332, 1604], 'adopting': [1227], 'material': [1236], 'neither': [1238], 'nor': [1242], 'employed': [1248], 'variation': [1252, 3695], 'emission': [1255, 1526, 3587, 3605, 3621, 4096], 'region.': [1256], 'our': [1258, 2785], 'works,': [1260], 'imidazole': [1261], 'was': [1262, 1344, 1734, 1749, 1761, 1883, 1899, 1916, 2071, 2087, 2104, 2264, 2315, 2339, 2361, 2509, 2515, 2541, 2667, 2684, 2859, 2879, 2895, 3209, 3476, 3493, 3533, 3596, 3714, 3803, 3945, 4022, 4045, 4134, 4192, 4235, 4303, 4327, 4336], 'ideal': [1264], 'unit': [1265, 1653, 3099], 'its': [1271, 1459, 2551, 2889, 3719, 4212], 'bipolar': [1275], 'transport': [1276], 'characteristics.36,42–44,53–55': [1277], 'It': [1278], 'tends': [1279], 'electron-withdrawing': [1284], 'substituent': [1285], 'linked': [1287], 'stronger': [1290], 'but': [1292, 2903, 2938, 3632], 'acts': [1293], 'donator': [1298], 'otherwise.42,51': [1299], 'Pyrene[4,5-d]imidazole': [1300], 'thus': [1302, 3256], 'chosen': [1303], 'creating': [1311], 'melt': [1313], 'imidazole.': [1317], 'contrast,': [1319, 2662, 3201], 'expected': [1322, 1382, 2406], 'play': [1324], 'role': [1326, 4206], 'connected': [1333], 'group.': [1337], 'D–π–A': [1340], 'molecule,': [1341, 2652], 'constructed': [1345, 3804], 'linking': [1347, 2697], '(pyrene-imidazole)': [1350], '(pyrene)': [1353], 'moieties': [1354, 2766], 'via': [1355, 2342], 'phenyl': [1357, 2921, 3097], 'bridge,': [1358], 'may': [1360, 3507], 'molecule': [1367, 3007, 3856], 'premise': [1370], 'guaranteeing': [1372], '(CT)': [1375], 'character.': [1376], 'this': [1378], 'case,': [1379], 'it': [1380, 3089], 'between': [1387, 1404, 2727, 2853, 3053, 3100, 3875], 'increase': [1392, 1425], 'ratio': [1394, 3085], 'exciton,': [1398], 'phenylene': [1401, 2886, 2902, 2937], 'π': [1402, 2657], 'bridge': [1403], 'pyrene-imidazole': [1408, 3469], 'enhance': [1415], '(LE)': [1422], 'ηPL.': [1427, 2969], 'As': [1428, 2330, 2444, 2617, 3703, 3811], 'result,': [1430], 'PyPI-Py': [1431, 1522, 1668, 2040, 2281, 2360, 2385, 2467, 2481, 2540, 2569, 2591, 2666, 2713, 2801, 2814, 3033, 3151, 3181, 3206, 3275, 3309, 3342, 3434, 3475, 3506, 3564, 3608, 3676, 3748, 3770, 3816, 3937, 4006, 4018, 4052, 4065, 4232, 4302, 4326], 'efficiencies': [1435], 'both': [1437, 2647, 3194, 3673, 3836, 3951], 'solution': [1438, 1713, 3361], '(82%': [1439], 'hexane': [1441], '10−5': [1443, 3368], 'M)': [1444, 3752], '(52%': [1449], 'neat': [1451, 3378, 3397, 4090, 4254], 'thickness': [1454], '30': [1456, 3383], 'nm).': [1457], 'single-crystal': [1460], 'mode,': [1466], 'suggesting': [1467], 'inhibition': [1470], 'intense': [1473], 'effect.': [1475], 'calculations': [1478, 2600, 2613, 3139], 'indicate': [1479], 'character': [1483, 2301, 3532], 'intensive': [1486], 'intercrossed': [1487], 'coupling': [1488, 3874], 'LE': [1492, 1675, 3516, 3527, 3733, 3868, 3879, 3929, 4003], 'states,': [1493, 3880], 'therefore': [1495], 'leads': [1496], 'predominant': [1499], 'feature': [1501], 'S1': [1504, 2805, 2812, 2958, 3054, 3918, 4037], '→': [1505, 2658, 2811, 2959], 'S0': [1506, 2810, 2960], 'transition,': [1507], 'consistent': [1510], 'proposed': [1514], 'principle.36,48–51': [1516], 'peaks': [1527, 3358, 3375], '475': [1529], 'nm': [1530, 3549, 3575, 3626, 3636, 4100, 4106, 4172, 4184], 'coordinate': [1534], '0.22).': [1537], 'm−2': [1552], 'achieved.': [1554], 'reach': [1559], '8.52%,': [1560], 'EUE': [1565, 3084], '82%,': [1569], 'almost': [1572], '3.2-fold': [1573], 'than': [1575, 3213, 3850, 4048, 4314], 'model': [1579, 2336], '9,10-diphenyl-9H-pyreno[4,5-d]imidazole': [1581], '(PyPI)': [1582], 'without': [1583, 4241], 'unit.': [1586, 1645, 2563], 'More': [1587], 'importantly,': [1588], 'device,': [1593], 'reached': [1602], 'even': [1603, 3931], 'date': [1636], 'Consequently,': [1646], 'introduction': [1649, 2558], 'onto': [1654], 'PyPI': [1656, 1853, 2279, 2338, 2383, 2425, 2488, 2503, 2526, 2589, 2622, 2672, 2729, 2816, 2884, 2907, 3001, 3185, 3198, 3216, 3273, 3307, 3327, 3436, 3454, 3481, 3540, 3590, 3674, 3709, 3754, 4016, 4040, 4092, 4143, 4195, 4253, 4317], 'segment,': [1657], 'nature': [1659, 2831], 'changed': [1670], 'ideally': [1671], 'from': [1672, 1891, 2079, 2284, 2862, 3269, 3292, 3409, 3421, 3467, 3510], 'preponderant': [1679], 'state,': [1681], 'Experimental': [1687], 'Methods': [1688], 'Synthesis': [1689, 1692, 1851, 2038, 2327], '4-pyren-1-yl-benzaldehyde': [1694, 2054], '1-Bromopyrene': [1695], '(4.90': [1696], 'g,': [1697, 1703, 1729, 1767, 1859, 1880, 1929, 2046, 2057, 2068, 2117], '17.4': [1698], 'mmol),': [1699, 1705, 1861, 1866, 1871, 2048, 2053, 2059], '(4-formylphenyl)boronic': [1700], 'acid': [1701, 1873, 1907, 2061, 2095], '(2.25': [1702], '15.0': [1704], 'dry': [1706], 'toluene': [1707], '(24.0': [1708], 'mL),': [1709, 1875, 2063], 'K2CO3': [1711], 'aqueous': [1712], '(16.0': [1714], 'mL,': [1715, 1864, 1869, 2051], '2.0': [1716], 'mol': [1717, 3369], 'L−1)': [1718], 'added': [1720], 'reaction': [1723, 2346], 'flask': [1724], 'followed': [1725], 'Pd(PPh3)4': [1727], '(1.05': [1728], '0.9': [1730], 'mmol).': [1731], 'mixture': [1733, 1855, 1898, 1908, 2042, 2086, 2096], 'refluxed': [1735, 2356], '90': [1737], '°C': [1738, 1893, 2081, 2492, 2543, 2547], 'under': [1739, 2357, 2592, 4173], 'N2': [1740, 2358], 'atmosphere': [1741], '48': [1743], 'h.': [1744, 1887, 2075], 'crude': [1747, 1914, 2102], 'product': [1748, 1760, 1915, 1927, 2103, 2115], 'extracted': [1750], 'trichloromethane': [1752], 'purified': [1755, 1918, 2106], 'column': [1757, 1920, 2108], 'chromatography.': [1758], 'isolated': [1762], 'white': [1764, 1926, 2114], 'powder': [1765], '(3.70': [1766], 'Yield:': [1768, 1930, 2118], '80%).': [1769], 'Proton': [1770], 'nuclear': [1771, 1983], 'magnetic': [1772, 1984], 'resonance': [1773, 1985], '(1H': [1774], 'NMR)': [1775, 1987], '[500': [1776], 'MHz,': [1777, 1935, 1989, 2123, 2192], 'dimethyl': [1778], 'sulfoxide': [1779], '(DMSO)-d6,': [1780], '25': [1781], '°C,': [1782, 2473, 2495, 2513, 2536], 'δ]:': [1783], '10.19': [1784], '(s,': [1785, 1809], '1H),': [1786, 1793, 1800, 1807, 1817, 1944, 1951, 1959, 2132, 2139, 2160, 2174], '8.43': [1787], '(d,': [1788, 1795, 1802, 1812, 1830, 1939, 1946, 1976, 2127, 2134, 2155, 2176, 2183], 'J': [1789, 1796, 1803, 1813, 1820, 1831, 1940, 1947, 1954, 1977, 2128, 2135, 2148, 2156, 2169, 2177, 2184], '7.9': [1791, 1823, 2137], 'Hz,': [1792, 1799, 1806, 1816, 1824, 1834, 1943, 1950, 1958, 1980, 2131, 2138, 2152, 2159, 2173, 2180, 2187], '8.38': [1794], '7.6': [1798], '8.34': [1801], '7.3': [1805], '8.28': [1808], '2H),': [1810, 1828, 1965, 1971, 2153, 2181], '8.23': [1811], '9.3': [1815], '8.15': [1818], '(dd,': [1819, 2147], '10.0,': [1822], '3H),': [1825, 1962, 1974, 2142, 2166], '8.13–8.08': [1826], '(m,': [1827, 1961, 1964, 1967, 1970, 1973, 2141, 2144, 2162, 2165], '7.91': [1829], '8.1': [1833], '2H).': [1835], 'Matrix-assisted': [1836], 'laser': [1837], 'desorption': [1838], 'ionization': [1839], 'time-of-flight': [1840], '(MALDI-TOF)': [1841], '(mass': [1842, 2011, 2226], 'm/z):': [1843, 2012, 2227], '[M+]': [1844, 2013, 2228], 'calcd': [1845, 2014, 2229], 'C23H14O,': [1847], '306.36;': [1848], 'found,': [1849, 2018, 2233], '307.20.': [1850], 'pyrene-4,5-dione': [1857, 2044, 2354], '(0.50': [1858, 2045], '2.1': [1860, 2047], 'aniline': [1862, 2049], '(5.0': [1863, 1868, 2050], '55.1': [1865, 2052], 'benzaldehyde': [1867, 2375], '49.0': [1870], 'acetic': [1872, 2060], '(15.0': [1874, 2062], 'ammonium': [1877, 2065, 2350], 'acetate': [1878, 2066], '(0.80': [1879, 2056, 2067, 3186], 'mmol)': [1882, 2070], 'stirred': [1884, 2072], '2': [1886, 2074, 2789], 'When': [1888, 2076], 'cooled': [1889, 2077], 'down': [1890, 2078], '120': [1892, 2080], 'temperature,': [1896, 2084], 'subsequently': [1900, 2088], 'filtered': [1901, 2089], 'flushed': [1903, 2091], 'water/acetic': [1906, 2094], '(3:1,': [1909, 2097], '40.0': [1910, 2098], 'mL).': [1911, 2099], 'Then,': [1912, 2100], 'chromatography': [1921, 2109], 'sublimation': [1923, 2111], 'give': [1925, 2113], '(0.65': [1928], '78%).': [1931], '1H': [1932, 2120, 2390], 'NMR': [1933, 2121, 2190, 2393], '(500': [1934, 2122], 'DMSO-d6,': [1936, 2124], 'δ)': [1937, 2125], '8.95': [1938], '7.0': [1942, 1949], '8.32': [1945], '8.24': [1952], '(t,': [1953, 2168], '8.6,': [1956], '8.6': [1957], '8.21–8.17': [1960], '7.83–7.79': [1963], '7.79–7.71': [1966], '4H),': [1968, 2163], '7.69–7.65': [1969], '7.43–7.36': [1972], '7.32': [1975], '1H).': [1981, 2188], 'Carbon': [1982], '(13C': [1986], '(126': [1988, 2191], 'CDCl3,': [1990, 2193], 'δ):': [1991, 2194], '132.20,': [1992], '131.69,': [1993], '130.17,': [1994, 2202], '129.87,': [1995], '129.49,': [1996], '129.22,': [1997], '128.91,': [1998], '128.28,': [1999], '127.97,': [2000], '127.58,': [2001], '126.40,': [2002], '125.29,': [2003], '124.54,': [2004], '124.29,': [2005], '122.85,': [2006], '122.46,': [2007], '119.82,': [2008], '117.98.': [2009], 'MALDI-TOF': [2010, 2225], 'C29H18N2,': [2016], '394.47;': [2017], '395.32.': [2019], 'Anal.': [2020, 2235], 'Calcd': [2021, 2236], '(%)': [2022, 2237], 'C29H18N2:': [2024], 'C,': [2025, 2032, 2240, 2247], '88.30;': [2026], 'H,': [2027, 2034, 2242, 2249], '4.60;': [2028], 'N,': [2029, 2036, 2244, 2251], '7.10.': [2030], 'Found:': [2031, 2246], '88.37;': [2033], '4.58;': [2035], '7.04.': [2037], '(PyP-CHO)': [2055], '2.6': [2058], '(0.77': [2116], '62%).': [2119], '9.02': [2126], '6.7': [2130], '8.40': [2133], '8.38–8.31': [2140], '8.28–8.20': [2143], '7H),': [2145], '8.13': [2146], '8.5,': [2150], '6.1': [2151], '8.06': [2154], '7.8': [2158, 2172], '7.99–7.90': [2161], '7.87–7.82': [2164], '7.80': [2167], '7.8,': [2171], '7.70': [2175], '8.3': [2179], '7.35': [2182], '8.2': [2186], '13C': [2189, 2392], '132.24,': [2195], '131.72,': [2196], '131.47,': [2197], '130.96,': [2198], '130.79,': [2199], '130.61,': [2200], '130.39,': [2201], '130.13,': [2203], '129.41,': [2204], '129.30,': [2205], '128.44,': [2206], '128.00,': [2207], '127.68,': [2208], '127.61,': [2209], '127.45,': [2210], '127.40,': [2211], '126.52,': [2212], '126.09,': [2213], '125.37,': [2214], '125.24,': [2215], '125.07,': [2216], '124.98,': [2217], '124.96,': [2218], '124.87,': [2219], '124.66,': [2220], '124.43,': [2221], '123.64,': [2222], '122.93,': [2223], '118.06.': [2224], 'C45H26N2,': [2231], '594.72;': [2232], '595.35.': [2234], 'C45H26N2:': [2239], '90.88;': [2241], '4.41;': [2243], '4.71.': [2245], '90.75;': [2248], '4.64;': [2250], '4.61.': [2252], 'Theoretical': [2253, 2599], 'calculation': [2254], 'Gaussian': [2255], '09': [2256], '(version': [2257], 'D.01)': [2258], 'package': [2259], 'PowerLeader': [2262], 'cluster': [2263], 'used': [2265, 2316], 'carry': [2267], 'all': [2269, 3725], 'density': [2271], 'functional': [2272], 'theory': [2273], '(DFT)': [2274], 'calculations.': [2275], 'structures': [2277, 2381, 2421], 'selected': [2283], 'optimized': [2285], 'ground-state': [2286], 'geometries': [2287, 2806], 'according': [2288, 4285], 'time-dependent': [2290], 'DFT': [2291, 2612], '(TD-DFT)': [2292], 'level': [2295, 3165, 3172, 3204], 'CAMB3LYP/6-31G(d,p).': [2297], 'examining': [2299], 'electronic': [2303], 'transitions,': [2304, 3517], 'dominant': [2306], '"particle"–"hole"': [2307], 'pair': [2308], 'contributions': [2309], 'TD-M062X/6-31G(d,p)': [2313], 'method': [2314, 3109], 'evaluate': [2318], 'natural': [2320], 'transition': [2321, 2459, 2956, 2987], 'orbitals': [2322, 2635, 2644], '(NTOs).': [2323], 'Results': [2324], 'Discussion': [2326], 'Scheme': [2333, 2417], '1,': [2334], 'conveniently': [2340], 'synthesized': [2341], 'click-like': [2344], 'one-pot': [2345], 'benzaldehyde,': [2349], 'acetate,': [2351], 'aniline,': [2352], 'atmosphere.24': [2359], 'good': [2365, 2402, 3283, 3884, 3972, 4220], 'yield': [2366], 'same': [2369, 4175], 'procedure': [2370], 'PyP-CHO': [2372], 'instead': [2373], 'starting': [2378], 'material.': [2379], 'fully': [2387, 2741], 'characterized': [2388], 'spectroscopies,': [2394], 'mass': [2395], 'spectrometry,': [2396], 'elemental': [2398], 'analysis': [2399, 2524, 2839, 3018], 'accordance': [2403], 'structures.': [2407], 'Supporting': [2408, 3037, 3141, 3600, 3699, 3958, 4034, 4054, 4114, 4268, 4292], 'Information': [2409, 3038, 3142, 3601, 3700, 3959, 4035, 4055, 4115, 4269], 'Figures': [2410, 3039], 'S1–S5': [2411], 'detailed': [2414], 'data.': [2416], '1': [2418, 2580, 3300, 3366], '|': [2419, 2581, 2790, 3301, 3741, 3763, 4060], 'Molecular': [2420], 'synthesis': [2423], 'PyPI-Py.': [2427, 2775, 3500, 3921], 'Thermal': [2432], 'properties': [2433, 2567, 3119, 3427], 'two': [2435, 3490], 'hydrocarbon': [2438], 'skeletons': [2439], 'featured': [2440], 'stability.': [2443], 'Figure': [2447, 2579, 2620, 2788, 3143, 3443, 3602, 3701, 3739, 3761, 3814, 4058, 4116, 4270], '1a,': [2448], 'differential': [2451], 'scanning': [2452], 'calorimetry': [2453], '(DSC)': [2454], 'heating': [2455, 2501], 'cycles,': [2456], 'glass': [2458], 'temperature': [2460, 2520, 2530], '(Tg)': [2461], 'melting': [2463], 'point': [2464], '(Tm)': [2465], 'appeared': [2468], '150': [2470], '317': [2472], 'Tg': [2476], 'Tm': [2478], 'much': [2483], 'compared': [2485], '74': [2491], '215': [2494], 'addition,': [2498, 2712], 'upon': [2499, 2982, 3693], 'beyond': [2504], 'Tg,': [2505], 'exothermal': [2507], 'peak': [2508, 3622, 3680, 4097, 4119], 'detected': [2510], '139': [2512], 'assigned': [2516], 'crystallization': [2519], '(Tc).': [2521], 'From': [2522], 'thermogravimetric': [2523], '(TGA),': [2525], 'decomposition': [2529], '(5%': [2531], 'weight': [2532], 'loss)': [2533], '355': [2535], 'whereas': [2537, 2681, 2892, 3563], '122': [2542], 'reaching': [2545], '477': [2546], '(Figure': [2548, 2737, 2875, 2925, 3014, 3616, 3696, 3996, 4246], '1b),': [2549], 'demonstrating': [2550, 3518], 'stability': [2554], 'additional': [2561, 3229], 'sufficient': [2571], 'meet': [2573], 'requirements': [2575], 'evaporative': [2577], 'manufacture.': [2578], 'DSC': [2582], '(a)': [2583, 2791], 'TGA': [2585], '(b)': [2586, 2804], 'curves': [2587], 'nitrogen': [2593], 'atmosphere.': [2594], 'estimate': [2602], 'configuration': [2605, 2870, 3013], 'distribution': [2607, 3244], 'frontier': [2609, 2707], 'orbitals,': [2611], 'carried': [2615], 'out.': [2616], '2a,': [2621], 'presented': [2623], 'nearly': [2624, 3010], 'coplanar': [2625, 2869], 'geometry': [2626, 2719], 'ground': [2629, 2735, 2795, 3691], 'occupied': [2633], '(HOMOs)': [2636], 'lowest': [2641, 3524], 'unoccupied': [2642], '(LUMOs)': [2645], 'delocalized': [2648, 2770, 2897], 'entire': [2651], 'indicating': [2653, 4200], 'pure': [2656], 'π*': [2659], 'transition.': [2660], 'HOMO': [2664, 2745, 2890, 3123, 3171, 3191], 'distributed': [2669, 3003], 'segment': [2673, 2908], 'residual': [2676], 'substituted': [2679], 'pyrene,': [2680], 'LUMO': [2683, 2743, 3121, 3164, 3203], 'located': [2686], 'group': [2690, 3231], 'sizable': [2692], 'extension': [2693], 'central': [2696], 'phenylene.': [2698], 'This': [2699, 3219, 3641, 3842, 4118], 'finding': [2700], 'suggested': [2701], 'change': [2704], 'orbital': [2709, 2950, 3243], 'distribution.': [2710], 'showed': [2714, 3817, 4093], 'torsion': [2723], 'angle': [2724, 2852, 2917], '55°': [2726, 2863], 'Py': [2731], 'units': [2732, 2858], '2a).': [2738], 'Unlike': [2739, 3582], 'separated': [2742, 2939], 'distributions': [2746, 2799, 2928, 2977], 'molecules': [2749], 'containing': [2750], 'units,': [2753], 'allowed': [2767], 'partially': [2769, 3508], 'HOMOs': [2771], 'LUMOs': [2773], 'Therefore,': [2776, 2927, 3905], 'serves': [2778, 3105], 'A,': [2782], 'accommodates': [2784], 'strategy.': [2787], 'Geometries': [2792], 'HOMO/LUMO': [2798, 3325], 'PyPI.': [2803], 'NTOs': [2808, 2838], '(f': [2817], 'oscillator': [2820], 'strength).': [2821], 'examine': [2827], 'study': [2829], 'PyPI-Py,': [2837, 3790, 4148, 4199], 'states': [2847, 3026, 3045], 'calculated.': [2849], 'twist': [2851, 2916], 'decreased': [2861, 2915], '35°,': [2865], 'inducing': [2866], 'more': [2868], '2b).': [2876], 'hole': [2878, 2974, 2997], 'mainly': [2880], 'spread': [2881], 'over': [2882, 3004], 'resembled': [2888], 'distribution,': [2891], 'particle': [2894, 2976, 2999], 'extended': [2904], 'degree': [2911], 'along': [2918], 'pyrene-imidazole,': [2920], 'ring,': [2922], '2).': [2926, 3015], 'hole–particle': [2930], 'overlapped': [2931], 'somewhat': [2940], 'section.': [2944], 'scale': [2947, 4240], 'overlaps': [2951], 'indicated': [2952, 2984, 3188, 3861], 'LE-type': [2955], 'considerable': [2964], 'radiative-transition': [2965], 'rate': [2966, 4278], 'separation': [2971], 'facilitated': [2989], 'substantial': [2990], 'formation.': [2993], 'comparison,': [2995], 'whole': [3006], 'unchanged': [3011], 'NTO': [3017, 3888], 'correlative': [3029], 'diagram': [3031], 'provided': [3035], 'S6': [3040], 'S7.': [3042], 'High-energy': [3043], 'T3': [3046, 3056], 'T4': [3048, 3058], 'splitting': [3052], 'or': [3057], '(ΔEST': [3059], '0.09': [3061], '0.08': [3063], 'eV,': [3064, 3159, 3280], 'respectively)': [3065], 'observed,': [3067], 'might': [3069, 3914], 'facilitate': [3070], 'reverse': [3072], 'intersystem': [3073], 'crossing': [3074], '(RISC)': [3075], 'process': [3076], 'procure': [3078], 'radiation': [3082], 'OLEDs.41–52': [3087], 'proved': [3092], 'introducing': [3094], 'π-conjugated': [3096], 'ring': [3098], 'effective': [3112], 'modulation': [3113], 'state.36': [3117], 'Electrochemical': [3118, 3304], 'levels': [3125, 3192], 'acquired': [3126], 'cyclic': [3128], 'voltammetry': [3129], '(CV)': [3130], 'measurements': [3131], 'similar': [3133, 3177, 3477], 'those': [3135], 'predicted': [3136], '(': [3140, 3599, 3957, 4033, 4053, 4113], 'S8).': [3144], 'reduction': [3146], 'oxidation': [3148, 3178], 'potentials': [3149, 3179], 'measured': [3153], '−2.20': [3156], '0.79': [3158], '−2.46': [3167], 'eV': [3168, 3211], '−5.45': [3174], 'eV.': [3175], '(0.79': [3182], 'eV)': [3183, 3187, 3208], 'determined': [3195, 3408, 4023], 'segment.': [3199], '(−2.46': [3207], '0.28': [3210, 3338], 'lower': [3212, 4047], '(−2.18': [3217], 'eV).': [3218], 'distinction': [3220], 'could': [3221, 3254], 'incorporation': [3226], 'acted': [3233], 'altered': [3240], 'mentioned': [3246, 3900], 'description.': [3250], 'electron-injection': [3252], 'ability': [3253], 'improved,': [3257], 'favored': [3259], 'enhancing': [3260], 'HOMO–LUMO': [3265], 'gaps': [3267, 3290], 'CV': [3271], '3.24': [3277, 3340], '2.99': [3279, 3352], 'agreement': [3284, 3885], 'UV–vis': [3294], 'spectroscopy': [3295], '(Table': [3297, 4185], '1).': [3298, 4186], 'Table': [3299, 3452, 3960, 4056], 'Optical': [3302, 3426], 'Properties': [3305], 'Compound': [3310], 'λabs': [3311, 3313], '(nm)a': [3312, 3316], '(nm)b': [3314, 3319], 'λem': [3315, 3317], '(FWHM)': [3318, 4129], 'ηPLc': [3320], 'Eg': [3321, 3323], '(eV)d': [3322], '(eV)e': [3324], '(eV)f': [3326], '330,': [3328], '350,': [3329, 3343], '382': [3330], '365,': [3331], '385': [3332, 3344], '383,': [3333], '405,': [3334], '430': [3335], '454': [3336, 4099], '(80)': [3337], '3.20': [3339], '−5.42/−2.18': [3341], '366,': [3345], '390': [3346], '450': [3347, 3574], '462': [3348], '(67)': [3349], '0.52': [3350], '3.06': [3351], '−5.45/−2.46': [3353], 'aUV–vis': [3354], 'absorption': [3355, 3372, 3411, 3457, 3472, 3491, 3503, 3670, 3720, 4071], 'THF': [3360, 3414, 3750, 3990, 4112], 'concentration': [3364], 'L−1.': [3370], 'bUV–vis': [3371], 'thin': [3379, 3398], '(film': [3381], 'thickness:': [3382], 'nm,': [3384, 3571, 4132], 'parentheses': [3388], 'FWHMs).': [3391], 'cPL': [3392], 'temperature.': [3402], 'dThe': [3403], 'bandgap': [3406, 3418], 'edge': [3412, 3498], 'solution.': [3415], 'eThe': [3416], 'electrochemical': [3417], 'estimated': [3420], 'CV.': [3422, 3425], 'fMeasured': [3423], 'UV': [3429, 3745, 3767], 'spectra': [3432, 3492, 3588, 3606, 3671, 3707, 3746, 3768], 'tetrahydrofuran': [3438], '(THF)': [3439], '3,': [3444], 'data': [3448], 'given': [3450, 3812], '1.': [3453], 'complex': [3456], 'profiles': [3458], 'localized': [3462], 'π–π*': [3463], 'vibronic': [3464, 3554, 3727], 'derived': [3466], 'moiety.': [3470], 'spectrum': [3473], 'profile.': [3483, 3581], 'largest': [3486], 'difference': [3487, 3716], 'these': [3489], '30-nm': [3495], 'red-shifted': [3496, 3615], 'onset': [3497], 'longer': [3502], 'band': [3504], 'arise': [3509], 'hybridization': [3512, 3864, 3908, 3925], 'extensive': [3520], 'similarity': [3521], 'excitation': [3528], 'energy.': [3529], 'evidenced': [3535], 'spectra.': [3539], 'emits': [3541], 'violet-blue': [3544], 'region': [3545], 'peaking': [3546, 3572], '383': [3548], 'features': [3551], 'distinct': [3553], 'fine': [3555, 3728], 'polar': [3559, 3639, 3840, 3897, 3935], 'solvent': [3560, 3594, 3630, 3663, 3694, 3898], 'THF,': [3562], 'manifested': [3565], 'red-shift': [3568], '67': [3570, 4183], 'exhibiting': [3577, 3685], 'broad,': [3579], 'structureless': [3580], 'miniscule': [3584], 'changes': [3585, 3688], 'observed': [3591, 3657], 'polarity': [3595, 3664], 'gradually': [3597], 'S9),': [3603], 'continuously': [3610], 'broadened': [3611], '4).': [3617], 'occurred': [3623, 4257], '420': [3625], 'nonpolar': [3629], 'n-hexane': [3631], 'moved': [3633], '480': [3635], 'acetonitrile.': [3640], 'solvatochromic': [3642, 3809], 'confirmed': [3645], 'inherence': [3647], 'constituent': [3651], 'other': [3659], 'reports.42–45': [3660], 'With': [3661], 'overall': [3667, 4046], 'profile': [3668], 'scarcely': [3677], 'changed,': [3678], 'shape,': [3681], 'position,': [3682], 'onset,': [3684], 'few': [3686], 'dipolar': [3687], '4': [3697, 3762], 'S9).': [3702], 'different': [3711, 3772, 4020], 'solvents,': [3712], 'just': [3717], 'like': [3718], 'spectra,': [3721], 'is,': [3723], 'showing': [3730], 'characteristic': [3734], '3': [3740], 'Normalized': [3742, 3764], '(10−5': [3751, 3774], 'comparison.': [3756], 'solvents': [3773, 3801, 3955, 3967], 'M).': [3775], 'investigate': [3782], 'property': [3784], 'Stokes': [3792, 4068], 'shift': [3793, 4069, 4168], '(va–vf)': [3794], 'versus': [3795, 4076], 'orientation': [3797, 4078], 'polarization': [3798, 4079], 'f(ɛ,n)': [3802], 'Lippert–Mataga': [3808, 4062], 'model.56': [3810], '5,': [3815], 'linear': [3819], 'relationship': [3820], 'dipole': [3823, 3844], 'moment': [3824], '14.37': [3826], 'D,': [3827], 'illustrating': [3828], 'only': [3830, 4170], 'existed': [3834], 'solvents.': [3841, 4083], 'moderate': [3843, 4042], 'moment,': [3845], 'actually': [3848], 'smaller': [3849], '4-(N,N-dimethylamino)benzonitrile': [3857], '(DMABN)': [3858], '(≈23': [3859], 'D),56': [3860], 'components': [3869, 3995, 4004, 4245], 'simulation': [3890], 'reports.42,43,50': [3904], 'occur': [3915], 'components,': [3930], 'acetonitrile,': [3936], 'retained': [3938, 4041], '70%,': [3943], 'comparable': [3946], 'low-': [3952], 'moderate-polarity': [3954], '(80–90%)': [3956], 'S1).': [3961, 4057], 'diverse': [3966], 'would': [3968], 'contribute': [3969], 'time-resolved': [3977], 'experiment': [3978], 'single-exponential': [3981], 'decay': [3982, 4230, 4251, 4277], 'short': [3984, 4260], 'lifetime': [3985, 4261], '1.55': [3987], 'ns': [3988], 'no': [3992], 'obvious': [3993], 'delay': [3994, 4244], '6a),': [3997], 'implying': [3998], 'combined': [4007], 'single': [4010], 'solutions': [4021], '0.1': [4026], 'M': [4027], 'quinoline': [4028], 'sulfate': [4029], 'reference': [4032], 'Tables': [4036], 'S2).': [4039], 'ηPL,': [4043], '5': [4059], 'Solvatochromic': [4061], 'models': [4063], '(νa:': [4070], 'wavenumber;': [4072], 'νf:': [4073], 'wavenumber)': [4075], '(f)': [4080], 'bathochromic-shift': [4103], '70': [4105], 'contrast': [4108], 'S10).': [4117], 'had': [4120], 'full': [4124], 'width': [4125], 'half': [4127], '80': [4131], 'ascribed': [4135], 'intermolecular': [4139, 4150], 'structure.24': [4146], 'interactions': [4151], 'suppressed': [4153], 'sterically': [4160], 'hindered': [4161], 'group,': [4163], 'leading': [4164], 'bathochromic': [4167], '12': [4171], 'experimental': [4176], 'conditions': [4177], 'reduced': [4180], 'FWHM': [4181], 'amorphous': [4190], 'films': [4191], '28%': [4193], '52%': [4197], 'played': [4203], 'positive': [4205], 'inhibiting': [4208], 'while': [4211], 'native': [4213], 'maintained.': [4225], 'Additionally,': [4226], 'transient': [4228, 4249], 'completely': [4237], 'within': [4238], 'nanosecond': [4239], 'any': [4242], 'apparent': [4243], '6b).': [4247], '3.12': [4263], 'ns,': [4264], 'S11.': [4271], 'radiative': [4274], 'nonradiative': [4276], 'constants': [4279], '(kr': [4280], 'knr)': [4282], 'equation': [4288], 'listed': [4289], 'Information.': [4293], 'excited-state': [4296], 'dynamics': [4297], 'study,': [4298], 'kr': [4300], '1.59': [4307], '108': [4309, 4320, 4333], 's−1,': [4310, 4334], '(0.89': [4318], 's−1),': [4321], 'knr': [4324], '1.47': [4331], 's': [4337]}, 'cited_by_api_url': 'https://api.openalex.org/works?filter=cites:W3122603190', 'counts_by_year': [{'year': 2024, 'cited_by_count': 15}, {'year': 2023, 'cited_by_count': 17}, {'year': 2022, 'cited_by_count': 14}, {'year': 2021, 'cited_by_count': 4}], 'updated_date': '2024-12-24T18:56:22.594443', 'created_date': '2021-02-01'}