Title: Photochemical Fate: The First Step Determines Efficiency of H2 Formation with a Supramolecular Photocatalyst
Abstract: Angewandte Chemie International EditionVolume 49, Issue 23 p. 3981-3984 Communication Photochemical Fate: The First Step Determines Efficiency of H2 Formation with a Supramolecular Photocatalyst† Stefanie Tschierlei, Stefanie Tschierlei Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302 These authors contributed equally to the work.Search for more papers by this authorMichael Karnahl, Michael Karnahl Friedrich-Schiller-Universität Jena, Institut für Anorganische und Analytische Chemie, August-Bebel-Strasse 2, 07743 Jena (Germany) These authors contributed equally to the work.Search for more papers by this authorMartin Presselt Dr., Martin Presselt Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorBenjamin Dietzek Dr., Benjamin Dietzek Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302 Institut für Photonische Techologien e.V. Albert-Einstein-Strasse 9, 07745 Jena (Germany)Search for more papers by this authorJulien Guthmuller Dr., Julien Guthmuller Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorLeticia González Prof. Dr., Leticia González Prof. Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorMichael Schmitt Dr., Michael Schmitt Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorSven Rau Prof. Dr., Sven Rau Prof. Dr. [email protected] Friedrich-Schiller-Universität Jena, Institut für Anorganische und Analytische Chemie, August-Bebel-Strasse 2, 07743 Jena (Germany) Friedrich-Alexander-Universität Erlangen-Nürnberg, Department Chemie und Pharmazie, Institut für Anorganische Chemie, Egerlandstrasse 1, 91058 Erlangen (Germany), Fax: (+49) 9131-852-7367Search for more papers by this authorJürgen Popp Prof. Dr., Jürgen Popp Prof. Dr. [email protected] Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302 Institut für Photonische Techologien e.V. Albert-Einstein-Strasse 9, 07745 Jena (Germany)Search for more papers by this author Stefanie Tschierlei, Stefanie Tschierlei Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302 These authors contributed equally to the work.Search for more papers by this authorMichael Karnahl, Michael Karnahl Friedrich-Schiller-Universität Jena, Institut für Anorganische und Analytische Chemie, August-Bebel-Strasse 2, 07743 Jena (Germany) These authors contributed equally to the work.Search for more papers by this authorMartin Presselt Dr., Martin Presselt Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorBenjamin Dietzek Dr., Benjamin Dietzek Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302 Institut für Photonische Techologien e.V. Albert-Einstein-Strasse 9, 07745 Jena (Germany)Search for more papers by this authorJulien Guthmuller Dr., Julien Guthmuller Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorLeticia González Prof. Dr., Leticia González Prof. Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorMichael Schmitt Dr., Michael Schmitt Dr. Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302Search for more papers by this authorSven Rau Prof. Dr., Sven Rau Prof. Dr. [email protected] Friedrich-Schiller-Universität Jena, Institut für Anorganische und Analytische Chemie, August-Bebel-Strasse 2, 07743 Jena (Germany) Friedrich-Alexander-Universität Erlangen-Nürnberg, Department Chemie und Pharmazie, Institut für Anorganische Chemie, Egerlandstrasse 1, 91058 Erlangen (Germany), Fax: (+49) 9131-852-7367Search for more papers by this authorJürgen Popp Prof. Dr., Jürgen Popp Prof. Dr. [email protected] Friedrich-Schiller-Universität, Institut für Physikalische Chemie, Helmholtzweg 4, 07743 Jena (Germany), Fax: (+49) 3641-948-302 Institut für Photonische Techologien e.V. Albert-Einstein-Strasse 9, 07745 Jena (Germany)Search for more papers by this author First published: 17 May 2010 https://doi.org/10.1002/anie.200906595Citations: 158 † Correspondence regarding the synthesis and catalysis should be addressed to Prof. Dr. Sven Rau and correspondence concerning the Raman spectra should be addressed to Prof. Dr. Jürgen Popp. This research was supported financially by the Thüringer Ministerium für Bildung, Wissenschaft und Kultur (grant no. B 514-09049). J.P. and B.D. acknowledge financial support from the FCI. S.R. and M.K. thank the DFG and the University of Jena. J.G. thanks the Carl-Zeiss Foundation. Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Graphical Abstract The color of the incident light determines the efficiency of the hydrogen evolution mediated by a supramolecular photocatalyst. This finding demonstrates the importance of the Franck–Condon point in artificial photosynthesis systems and should have an impact on their design. References 1V. Balzani, A. Credi, M. Venturi, ChemSusChem 2008, 1, 26– 58. 2N. Armaroli, V. Balzani, Angew. Chem. 2007, 119, 52– 67. 3K. Rangan, S. M. Arachchige, J. R. Brown, K. J. Brewer, Energy Environ. 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Publication Year: 2010
Publication Date: 2010-05-17
Language: en
Type: article
Indexed In: ['crossref', 'pubmed']
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