Title: The Ammonia-Synthesis Catalyst of the Next Generation: Barium-Promoted Oxide-Supported Ruthenium
Abstract: Angewandte Chemie International EditionVolume 40, Issue 6 p. 1061-1063 Communication The Ammonia-Synthesis Catalyst of the Next Generation: Barium-Promoted Oxide-Supported Ruthenium Hubert Bielawa Dr., Hubert Bielawa Dr. Laboratory of Industrial Chemistry Ruhr University Bochum 44780 Bochum (Germany) Fax: (+49) 234-32-14115Search for more papers by this authorOlaf Hinrichsen Dr., Olaf Hinrichsen Dr. Laboratory of Industrial Chemistry Ruhr University Bochum 44780 Bochum (Germany) Fax: (+49) 234-32-14115Search for more papers by this authorAlexander Birkner Dr., Alexander Birkner Dr. Physical Chemistry I Ruhr University BochumSearch for more papers by this authorMartin Muhler Prof. Dr., Martin Muhler Prof. Dr. [email protected] Laboratory of Industrial Chemistry Ruhr University Bochum 44780 Bochum (Germany) Fax: (+49) 234-32-14115Search for more papers by this author Hubert Bielawa Dr., Hubert Bielawa Dr. Laboratory of Industrial Chemistry Ruhr University Bochum 44780 Bochum (Germany) Fax: (+49) 234-32-14115Search for more papers by this authorOlaf Hinrichsen Dr., Olaf Hinrichsen Dr. Laboratory of Industrial Chemistry Ruhr University Bochum 44780 Bochum (Germany) Fax: (+49) 234-32-14115Search for more papers by this authorAlexander Birkner Dr., Alexander Birkner Dr. Physical Chemistry I Ruhr University BochumSearch for more papers by this authorMartin Muhler Prof. Dr., Martin Muhler Prof. Dr. [email protected] Laboratory of Industrial Chemistry Ruhr University Bochum 44780 Bochum (Germany) Fax: (+49) 234-32-14115Search for more papers by this author First published: 14 March 2001 https://doi.org/10.1002/1521-3773(20010316)40:6<1061::AID-ANIE10610>3.0.CO;2-BCitations: 252Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onEmailFacebookTwitterLinkedInRedditWechat Graphical Abstract A high potential to save energy in the production of ammonia is possible with the ruthenium catalysts developed by a knowledge-based approach using a parallel screening procedure. The high activity of these catalysts is dominated by the B5-type site 1. References 1 A. Mittasch, Adv. Catal. 1950, 2, 81–104. 10.1016/S0360-0564(08)60375-2 Web of Science®Google Scholar 2 Google Scholar 2a K.-I. Aika, K. Tamaru in Ammonia: Catalysis and Manufacture ( ), Springer, Berlin, 1995, pp. 103–148; 10.1007/978-3-642-79197-0_3 Google Scholar 2b O. Hinrichsen, Catal. Today 1999, 53, 177–188, and refs therein. 10.1016/S0920-5861(99)00115-7 CASWeb of Science®Google Scholar 3 Google Scholar 3a A. I. Foster, P. G. James, J. J. McCarroll, S. R. Tennison The British Petroleum, US-A 4 163 775, 1979; Google Scholar 3b J. J. McCarroll, S. R. Tennison, N. P. Wilkinson The British Petroleum, US-A 4 600 571, 1986. Google Scholar 4 Google Scholar 4a G. S. Benner, J. R. Le Blanc, J. M. Lee, H. P. Leftin, P. J. Shires, C. P. van Dijk The M. W. Kellogg Company, US-A 4 568 532, 1986; Google Scholar 4b A. K. Rhodes, Oil Gas J. 1996, 11, 37–41; Google Scholar 4c R. Strait, Nitrogen Methanol 1999, 238, 37–43. Google Scholar 5 Google Scholar 5a Z. Kowalczyk, J. Sentek, S. Jodzis, R. Diduszko, A. Presz, A. Terzyk, Z. Kucharski, J. Suwalski, Carbon 1996, 34, 403–409; 10.1016/0008-6223(95)00199-9 CASWeb of Science®Google Scholar 5b Z. Kowalczyk, S. Jodzis, W. Rarog, J. Zielinski, J. Pielaszek, Appl. Catal. A 1998, 173, 153–160. 10.1016/S0926-860X(98)00175-6 CASWeb of Science®Google Scholar 6 Google Scholar 6a S. Dahl, E. Törnqvist, I. Chorkendorff, J. Catal. 2000, 192, 381–390; 10.1006/jcat.2000.2858 CASWeb of Science®Google Scholar 6b S. Dahl, J. Sehested, C. J. H. Jacobsen, E. Törnqvist, I. Chorkendorff, J. Catal. 2000, 192, 391–399; 10.1006/jcat.2000.2857 CASWeb of Science®Google Scholar 6c S. Dahl, A. Logadottir, R. C. Egeberg, J. H. Larsen, I. Chorkendorff, E. Törnqvist, J. K. Nørskov, Phys. Rev. Lett. 1999, 83, 1814–1817; 10.1103/PhysRevLett.83.1814 Web of Science®Google Scholar 6d S. Dahl, P. A. Taylor, E. Törnqvist, I. Chorkendorff, J. Catal. 1998, 178, 679–686; 10.1006/jcat.1998.2168 CASWeb of Science®Google ScholarC. J. H. Jacobsen, S. Dahl, P. L. Hansen, E. Törnqvist, H. Topsøe, D. V. Prip, P. B. Moenshaug, I. Chorkendorff, J. Mol. Catal. A 2000, 163, 19–26. Google Scholar 7 R. van Hardeveld, A. van Montfoort, Surf. Sci. 1966, 4, 396–430. 10.1016/0039-6028(66)90016-1 CASWeb of Science®Google Scholar 8 Google Scholar 8a H. Bielawa, O. Hinrichsen, M. Muhler, J. Catal., submitted; Google Scholar 8b H. Bielawa, PhD Thesis, Ruhr-University Bochum, 2000. Google Scholar 9 F. Rosowski, A. Hornung, O. Hinrichsen, D. Herein, M. Muhler, G. Ertl, Appl. Catal. A 1997, 151, 443–460. 10.1016/S0926-860X(96)00304-3 CASWeb of Science®Google Scholar 10 A. Nielsen, An Investigation of Promoted Iron Catalysts for the Synthesis of Ammonia, 3rd ed., Gjellerup, Copenhagen, 1968. Google Scholar 11 K. Aika, T. Takano, S. Murata, J. Catal. 1992, 136, 126–140. 10.1016/0021-9517(92)90112-U CASWeb of Science®Google Scholar 12 Google Scholar 12a P. Cong, R. D. Doolen, Q. Fan, D. M. Giaquinta, S. Guan, E. W. McFarland, D. M. Poojary, K. Self, H. W. Turner, W. H. Weinberg, Angew. Chem. 1999, 111, 508–512; 10.1002/(SICI)1521-3757(19990215)111:4<507::AID-ANGE507>3.0.CO;2-I Google ScholarAngew. Chem. Int. Ed. 1999, 38, 484–488; 10.1002/(SICI)1521-3773(19990215)38:4<483::AID-ANIE483>3.0.CO;2-# CASWeb of Science®Google Scholar 12b B. Jandeleit, D. J. Schaefer, T. S. Powers, H. W. Turner, W. H. Weinberg, Angew. Chem. 1999, 111, 2648–2689; 10.1002/(SICI)1521-3757(19990903)111:17<2648::AID-ANGE2648>3.0.CO;2-N Google ScholarAngew. Chem. Int. Ed. 1999, 38, 2476–2514. 10.1002/(SICI)1521-3773(19990903)38:17<2476::AID-ANIE2476>3.0.CO;2-S CASPubMedGoogle Scholar 13 M. Muhler, O. Hinrichsen, H. Bielawa, C. J. H. Jacobsen Haldor Topsøe A/S, DK-A 3157237003, 2000. Google Scholar Citing Literature Volume40, Issue6March 16, 2001Pages 1061-1063 ReferencesRelatedInformation
Publication Year: 2001
Publication Date: 2001-03-16
Language: en
Type: article
Indexed In: ['crossref', 'pubmed']
Access and Citation
Cited By Count: 282
AI Researcher Chatbot
Get quick answers to your questions about the article from our AI researcher chatbot