Title: Heterogeneous Catalysis of CO<sub>2</sub> Conversion to Methanol on Copper Surfaces
Abstract: Angewandte Chemie International EditionVolume 53, Issue 45 p. 12022-12024 Highlight Heterogeneous Catalysis of CO2 Conversion to Methanol on Copper Surfaces† Prof. Dr. Malte Behrens, Corresponding Author Prof. Dr. Malte Behrens [email protected] Faculty of Chemistry and Center for Nanointegration Duisburg-Essen (CENIDE), Universität Duisburg-Essen, Universitätststr. 7 (Germany)Faculty of Chemistry and Center for Nanointegration Duisburg-Essen (CENIDE), Universität Duisburg-Essen, Universitätststr. 7 (Germany)Search for more papers by this author Prof. Dr. Malte Behrens, Corresponding Author Prof. Dr. Malte Behrens [email protected] Faculty of Chemistry and Center for Nanointegration Duisburg-Essen (CENIDE), Universität Duisburg-Essen, Universitätststr. 7 (Germany)Faculty of Chemistry and Center for Nanointegration Duisburg-Essen (CENIDE), Universität Duisburg-Essen, Universitätststr. 7 (Germany)Search for more papers by this author First published: 14 October 2014 https://doi.org/10.1002/anie.201409282Citations: 117 † I thank Robert Schlögl and Felix Studt for fruitful discussions. Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onEmailFacebookTwitterLinkedInRedditWechat Graphical Abstract Combined experimental and theoretical approaches resulted in a better understanding of the hydrogenation of CO2 to methanol on copper-based catalysts. These results highlight the important role of the reducible oxide promoter for CO2 activation. References 1 1aM. Bertau, H. Offermanns, L. Plass, F. Schimdt, H.-J. Wernicke, Methanol: The Basic Chemical and Energy Feedstock of the Future, Springer, Heidelberg, 2013; 1bG. A. Olah, Angew. Chem. Int. Ed. 2013, 52, 104; Angew. Chem. 2013, 125, 112. 2R. Schlögl, Green 2012, 2, 235. 3J. Graciani, K. Mudiyanselage, F. Xu, A. E. Baber, J. Evans, S. D. Senanayake, D. J. Stacchiola, P. Liu, J. Hrbek, J. Fernández Sanz, J. A. Rodriguez, Science 2014, 345, 546. 4Y. Yang, C. A. Mims, D. H. Mei, C. H. F. Peden, C. T. Campbell, J. Catal. 2013, 298, 10. 5T. Fujitani, I. Nakamura, T. Uchijima, J. Nakamura, Surf. Sci. 1997, 383, 285. 6L. Martínez-Suárez, J. Frenzel, D. Marx, B. Meyer, Phys. Rev. Lett. 2013, 110, 086108. 7S. Kuld, C. Conradsen, P. G. Moses, I. Chorkendorff, J. Sehested, Angew. Chem. Int. Ed. 2014, 53, 5941; Angew. Chem. 2014, 126, 6051. 8V. Schott, H. Oberhofer, A. Birkner, M. Xu, Y. Wang, M. Muhler, K. Reuter, C. Wöll, Angew. Chem. Int. Ed. 2013, 52, 11925; Angew. Chem. 2013, 125, 12143. 9M. G. Willinger, W. Zhang, O. Bondarchuk, S. Shaikhutdinov, H. J. Freund, R. Schlögl, Angew. Chem. Int. Ed. 2014, 53, 5998; Angew. Chem. 2014, 126, 6108. 10 10aR. Naumann d'Alnoncourt, M. Kurtz, H. Wilmer, E. Löffler, V. Hagen, J. Shen, M. Muhler, J. Catal. 2003, 220, 249; 10bN. Y. Topsøe, H. Topsøe, Top. Catal. 1999, 8, 267. 11F. Studt, F. Abild-Pedersen, J. B. Varley, J. K. Nørskov, Catal. Lett. 2013, 143, 71. 12 12aF. Studt, I. Sharafutdinov, F. Abild-Pedersen, C. F. Elkjær, J. S. Hummelshøj, S. Dahl, I. Chorkendorff, J. K. Nørskov, Nat. Chem. 2014, 6, 320; 12bG. Prieto, J. Zečević, H. Friedrich, K. P. De Jong, P. E. De Jongh, Nat. Mater. 2013, 12, 34; 12cO. Martin, J. Pérez-Ramírez, Catal. Sci. Technol. 2013, 3, 3343. Citing Literature Volume53, Issue45November 3, 2014Pages 12022-12024 ReferencesRelatedInformation
Publication Year: 2014
Publication Date: 2014-10-14
Language: en
Type: article
Indexed In: ['crossref', 'pubmed']
Access and Citation
Cited By Count: 126
AI Researcher Chatbot
Get quick answers to your questions about the article from our AI researcher chatbot